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Book ; Article ; Online: Mitigating NO_x emissions does not help alleviate wintertime particulate pollution in Beijing-Tianjin-Hebei (BTH), China

Li, Xia / Bei, Naifang / Hu, Bo / Wang, Yuan / Liu, Suixin / Wu, Jiarui / Pan, Yuepeng / Wen, Tianxue / Liu, Zirui / Liu, Lang / Wang, Ruonan / Zuo, Min / Shen, Zhenxing / Cao, Junji / Tie, Xuexi / Molina, Luisa T. / Li, Guohui

2020  

Abstract: ... in January 2019 in the BTH reveal that NO_x emissions mitigation does not help lower wintertime nitrate and ... decreased by over 20%. It still remains elusive about contributions of nitrogen oxides (NO_x) emissions ... by NO_x mitigation offsets the HNO₃ loss and enhances sulfate and secondary organic aerosols formation ...

Abstract Stringent mitigation measures have reduced wintertime PM_(2.5) concentrations by 42.2% from 2013 to 2018 in the BTH. The observed nitrate aerosols have not exhibited a significant decreasing trend and constituted a major fraction (about 20%) of the total PM_(2.5), although the surface-measured NO₂ level has decreased by over 20%. It still remains elusive about contributions of nitrogen oxides (NO_x) emissions mitigation to the nitrate and PM_(2.5) level. The WRF-Chem model simulations of a persistent haze episode in January 2019 in the BTH reveal that NO_x emissions mitigation does not help lower wintertime nitrate and PM_(2.5) concentrations under current conditions in the BTH, because the substantial O₃ increase induced by NO_x mitigation offsets the HNO₃ loss and enhances sulfate and secondary organic aerosols formation. Our results are further consolidated by occurrence of the severe PM pollution in the BTH during the COVID-19 outbreak with a significant reduction of NO₂.
Keywords covid19
Publishing date 2020-09-02
Publishing country us
Document type Book ; Article ; Online
Database BASE - Bielefeld Academic Search Engine (life sciences selection)

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