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Article: Piscidin-1, an antimicrobial peptide from fish (hybrid striped bass morone saxatilis x M. chrysops), induces apoptotic and necrotic activity in HT1080 cells.

Lin, Heng-Ju / Huang, Tsui-Chin / Muthusamy, Sasikala / Lee, Jheng-Fong / Duann, Yeh-Fang / Lin, Cheng-Hui

2012 Volume 29, Issue 5, Page(s) 327–332

Abstract: Piscidin-1, a 22-residue cationic peptide isolated from mast cells of a hybrid striped bass, has potent antimicrobial activities against both gram-positive and -negative bacteria. To date, there is no report of its antitumor activity on any tumor cell ... ...

Abstract	Piscidin-1, a 22-residue cationic peptide isolated from mast cells of a hybrid striped bass, has potent antimicrobial activities against both gram-positive and -negative bacteria. To date, there is no report of its antitumor activity on any tumor cell lines. In this study, we examined the antitumor activity of a synthetic piscidin-1 peptide against several human cancer cell lines using an MTS assay and soft-agar colony-formation assay. We found that a low dose of piscidin induces both apoptosis and necrosis in HT1080 cells, as shown by annexin-V/propidium iodide and acridine orange/ethidium bromide staining, and triggers a necrotic cell death pathway in a short period with high-dose treatment. The destruction of cell membranes by piscidin-1 was demonstrated by transmission electron microscopy. Furthermore, piscidin-1 also inhibits the migration of HT1080 cells in a dose-dependent manner. This study provides the first evidence of the anticancer activity of the antimicrobial peptide, piscidin-1, with potential implications for the treatment of cancer.
MeSH term(s)	Animals ; Antimicrobial Cationic Peptides/genetics ; Antimicrobial Cationic Peptides/metabolism ; Antimicrobial Cationic Peptides/pharmacology ; Antineoplastic Agents/metabolism ; Antineoplastic Agents/pharmacology ; Bass/genetics ; Bass/metabolism ; Cell Line, Tumor ; Fish Proteins/genetics ; Fish Proteins/metabolism ; Fish Proteins/pharmacology ; Gene Expression Regulation ; Humans ; Real-Time Polymerase Chain Reaction ; Reverse Transcriptase Polymerase Chain Reaction
Chemical Substances	Antimicrobial Cationic Peptides ; Antineoplastic Agents ; Fish Proteins ; moronecidin protein, Morone saxatilis
Language	English
Publishing date	2012-05
Publishing country	Japan
Document type	Journal Article ; Research Support, Non-U.S. Gov't
ZDB-ID	2038883-4
ISSN	0289-0003
ISSN	0289-0003
DOI	10.2108/zsj.29.327
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Article: A high retinol dietary intake increases its apical absorption by the proximal small intestine of juvenile sunshine bass (Morone chrysops x M. saxatilis).

Buddington, Randal K / Buddington, Karyl K / Deng, Dong-Fang / Hemre, Gro-Ingunn / Wilson, Robert P

The Journal of nutrition

2002 Volume 132, Issue 9, Page(s) 2713–2716

Abstract: The relationship between dietary intake and systemic availability of retinol is likely to be complex because although retinol is an essential nutrient, it is toxic at high levels. The present study determined whether rates of transapical retinol ... ...

Abstract	The relationship between dietary intake and systemic availability of retinol is likely to be complex because although retinol is an essential nutrient, it is toxic at high levels. The present study determined whether rates of transapical retinol absorption are modulated so that availability is increased at low dietary levels, but decreased when dietary intake is excessive. Juvenile hybrid striped bass were fed for 6 wk diets with 568 (below), 1657 (approximating the requirement) and 40,244 (excessive) micro g/kg dry diet of trans retinol. Proximal small intestine segments were used to measure rates of retinol absorption and tissue concentrations. Initial and final body mass did not differ among groups; deficiency and toxicity symptoms were not observed. Uptake of tracer retinol was inhibited by unlabeled retinol, indicating the presence of saturable, carrier-mediated absorption. Increasing dietary levels of retinol increased the rates of absorption measured at 0.05 mmol/L [8.04 +/- 0.65; 15.2 +/- 1.53; 25.1 +/- 3.4 pmol/(mg. min) for below, approximating and exceeding the retinol requirement; P < 0.0001]; this resulted in higher tissue concentrations of all-trans retinol (0.21 +/- 0.03, 0.49 +/- 0.21 and 338 +/- 89 pmol/g; P < 0.0001) and dehydro-retinol (0.11 +/- 0.04, 0.91 +/- 0.04, and 454 +/- 109 pmol/g; P < 0.001). These findings suggest that the systemic availability of various dietary levels of retinol is modulated after transapical absorption.
MeSH term(s)	Animals ; Bass/growth & development ; Bass/metabolism ; Biological Availability ; Dose-Response Relationship, Drug ; Intestinal Absorption/drug effects ; Intestine, Small/metabolism ; Random Allocation ; Vitamin A/administration & dosage ; Vitamin A/pharmacokinetics ; Vitamin A/pharmacology
Chemical Substances	Vitamin A (11103-57-4)
Language	English
Publishing date	2002-09
Publishing country	United States
Document type	Journal Article
ZDB-ID	218373-0
ISSN	1541-6100 ; 0022-3166
ISSN (online)	1541-6100
ISSN	0022-3166
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Article ; Online: Enhanced catalytic activity of Ce(1-x)M(x)O2 (M = Ti, Zr, and Hf) solid solution with controlled morphologies.

Chen, Wei-Ta / Chen, Kuei-Bo / Wang, Ming-Fang / Weng, Sheng-Feng / Lee, Chi-Shen / Lin, M C

Chemical communications (Cambridge, England)

2010 Volume 46, Issue 19, Page(s) 3286–3288

Abstract: Ce(1-x)M(x)O(2) (M = Ti, Zr, and Hf) nanomaterials with controlled morphology and composition were ...

Abstract	Ce(1-x)M(x)O(2) (M = Ti, Zr, and Hf) nanomaterials with controlled morphology and composition were synthesized by a two-step route for the first time. These nanomaterials exhibit high activities for hydrogen reduction and ethanol reforming reactions, and therefore, they may be useful for applications in catalysis and solid oxide fuel cells.
Language	English
Publishing date	2010-05-21
Publishing country	England
Document type	Journal Article
ZDB-ID	1472881-3
ISSN	1364-548X ; 1359-7345 ; 0009-241X
ISSN (online)	1364-548X
ISSN	1359-7345 ; 0009-241X
DOI	10.1039/b923217f
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Article ; Online: Synthesis and phase width of quaternary selenides Pb4In(x)M(6-x)Se13 (M = Bi, x = 2.1-2.8; Sb, x = 2).

Wang, Ming-Fang / Huang, Wen-Hen / Lee, Chi-Shen

Inorganic chemistry

2009 Volume 48, Issue 14, Page(s) 6402–6408

Abstract: Quaternary selenides of Pb(4)In(x)M(6-x)Se(13) (M = Bi, x = 2.1-2.8; Sb, x = 2) were synthesized ... by solid-state methods, and their structures were determined from X-ray diffraction of single crystals ...

Abstract	Quaternary selenides of Pb(4)In(x)M(6-x)Se(13) (M = Bi, x = 2.1-2.8; Sb, x = 2) were synthesized by solid-state methods, and their structures were determined from X-ray diffraction of single crystals. These compounds are isostructural with Pb(4)In(2)Bi(4)S(13) and crystallize in orthorhombic space group Pbam (No. 55) with Z = 4; the structure features a three-dimensional framework consisting of Z-shaped ribbon units and corner-sharing infinite one-dimensional [InSe(4)](infinity) chains running parallel to the c-axis, which are connected by Pb atoms to form a three-dimensional structure. Calculations of the band structure and measurements of Seebeck coefficient, electrical conductivity, and diffuse reflectance spectra confirm that these compounds are semiconductors with a narrow band gap. All compounds show semiconducting properties; the Seebeck coefficient of Pb(4)In(2.5)Bi(3.5)Se(13) is -180 microV/K at 295 K.
Language	English
Publishing date	2009-07-20
Publishing country	United States
Document type	Journal Article
ZDB-ID	1484438-2
ISSN	1520-510X ; 0020-1669
ISSN (online)	1520-510X
ISSN	0020-1669
DOI	10.1021/ic8023875
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Article ; Online: Atypical X-linked agammaglobulinaemia caused by a novel BTK mutation in a selective immunoglobulin M deficiency patient.

Lim, Lee-Moay / Chang, Jer-Ming / Wang, I-Fang / Chang, Wei-Chiao / Hwang, Daw-Yang / Chen, Hung-Chun

BMC pediatrics

2013 Volume 13, Page(s) 150

Abstract: Background: X-linked agammaglobulinaemia (XLA) is the most common inherited humoural ... who presented with selective immunoglobulin M (IgM) immunodeficiency and nephropathy. He was diagnosed ...

Abstract	Background: X-linked agammaglobulinaemia (XLA) is the most common inherited humoural immunodeficiency disorder. Mutations in the gene coding for Bruton's tyrosine kinase (BTK) have been identified as the cause of XLA. Most affected patients exhibit a marked reduction of serum immunoglobulins, mature B cells, and an increased susceptibility to recurrent bacterial infections. However, the diagnosis of XLA can be a challenge in certain patients who have near-normal levels of serum immunoglobulin. Furthermore, reports on XLA with renal involvement are scant. Case presentation: We report an atypical XLA patient who presented with selective immunoglobulin M (IgM) immunodeficiency and nephropathy. He was diagnosed with selective IgM immunodeficiency, based on his normal serum immunoglobulin G (IgG) and immunoglobulin A (IgA) levels but undetectable serum IgM level. Intravenous immunoglobulin was initiated due to increased infections and persistent proteinuria but no improvement in proteinuria was found. A lupus-like nephritis was detected in his kidney biopsy and the proteinuria subsided after receiving a mycophenolate mofetil regimen. Although he had a history of recurrent bacterial infections since childhood, XLA was not diagnosed until B-lymphocyte surface antigen studies and a genetic analysis were conducted. Conclusions: We suggest that B-lymphocyte surface antigen studies and a BTK mutation analysis should be performed in familial patients with selective IgM deficiency to rule out atypical XLA.
MeSH term(s)	Agammaglobulinemia/diagnosis ; Agammaglobulinemia/genetics ; Antigens, Differentiation, B-Lymphocyte/analysis ; Child ; Genetic Diseases, X-Linked/genetics ; Humans ; Immunoglobulin M/deficiency ; Immunoglobulin M/genetics ; Male ; Mycophenolic Acid/analogs & derivatives ; Mycophenolic Acid/therapeutic use ; Nephritis/drug therapy ; Nephritis/etiology ; Proteinuria/etiology
Chemical Substances	Antigens, Differentiation, B-Lymphocyte ; Immunoglobulin M ; Mycophenolic Acid (HU9DX48N0T)
Language	English
Publishing date	2013-09-27
Publishing country	England
Document type	Case Reports ; Journal Article
ZDB-ID	2041342-7
ISSN	1471-2431 ; 1471-2431
ISSN (online)	1471-2431
ISSN	1471-2431
DOI	10.1186/1471-2431-13-150
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Article ; Online: The Origin of Capacity Fade in the Li2MnO3·LiMO2 (M = Li, Ni, Co, Mn) Microsphere Positive Electrode: An Operando Neutron Diffraction and Transmission X-ray Microscopy Study.

Chen, Chih-Jung / Pang, Wei Kong / Mori, Tatsuhiro / Peterson, Vanessa K / Sharma, Neeraj / Lee, Po-Han / Wu, She-Huang / Wang, Chun-Chieh / Song, Yen-Fang / Liu, Ru-Shi

Journal of the American Chemical Society

2016 Volume 138, Issue 28, Page(s) 8824–8833

Abstract: The mechanism of capacity fade of the Li2MnO3·LiMO2 (M = Li, Ni, Co, Mn) composite positive ... transmission X-ray microscopy methods, enabling the phase, crystallographic, and morphological evolution ... of 73(1) wt % R3̅m LiMO2 with the remaining 27(1) wt % C2/m Li2MnO3 likely existing as an intergrowth ...

Abstract	The mechanism of capacity fade of the Li2MnO3·LiMO2 (M = Li, Ni, Co, Mn) composite positive electrode within a full cell was investigated using a combination of operando neutron powder diffraction and transmission X-ray microscopy methods, enabling the phase, crystallographic, and morphological evolution of the material during electrochemical cycling to be understood. The electrode was shown to initially consist of 73(1) wt % R3̅m LiMO2 with the remaining 27(1) wt % C2/m Li2MnO3 likely existing as an intergrowth. Cracking in the Li2MnO3·LiMO2 electrode particle under operando microscopy observation was revealed to be initiated by the solid-solution reaction of the LiMO2 phase on charge to 4.55 V vs Li(+)/Li and intensified during further charge to 4.7 V vs Li(+)/Li during the concurrent two-phase reaction of the LiMO2 phase, involving the largest lattice change of any phase, and oxygen evolution from the Li2MnO3 phase. Notably, significant healing of the generated cracks in the Li2MnO3·LiMO2 electrode particle occurred during subsequent lithiation on discharge, with this rehealing being principally associated with the solid-solution reaction of the LiMO2 phase. This work reveals that while it is the reduction of lattice size of electrode phases during charge that results in cracking of the Li2MnO3·LiMO2 electrode particle, with the extent of cracking correlated to the magnitude of the size change, crack healing is possible in the reverse solid-solution reaction occurring during discharge. Importantly, it is the phase separation during the two-phase reaction of the LiMO2 phase that prevents the complete healing of the electrode particle, leading to pulverization over extended cycling. This work points to the minimization of behavior leading to phase separation, such as two-phase and oxygen evolution, as a key strategy in preventing capacity fade of the electrode.
Language	English
Publishing date	2016-07-20
Publishing country	United States
Document type	Journal Article
ZDB-ID	3155-0
ISSN	1520-5126 ; 0002-7863
ISSN (online)	1520-5126
ISSN	0002-7863
DOI	10.1021/jacs.6b03932
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Article: Full-Spectral Fine-Tuning Visible Emissions from Cation Hybrid Cs1âmFAmPbX3 (X = Cl, Br, and I, 0 â¤ m â¤ 1) Quantum Dots

Chen, Daqin / Chen Xiao / Wan Zhongyi / Fang Gaoliang

ACS applied materials . 2017 June 21, v. 9, no. 24

2017

Abstract: ... of monodisperse, cubic structure CsâââFAâPbXâ (X = Cl, Br, and I or their mixtures Cl/Br and Br/I, 0 â ... m â¤ 1) hybrid perovskite quantum dots (QDs). Impressively, cation substitution of Csâº by FAâº ...

Abstract	Full-color visible emissions are particularly crucial for applications in displays and lightings. In this work, we developed a facile room-temperature ligand-assisted supersaturated recrystallization synthesis of monodisperse, cubic structure CsâââFAâPbXâ (X = Cl, Br, and I or their mixtures Cl/Br and Br/I, 0 â¤ m â¤ 1) hybrid perovskite quantum dots (QDs). Impressively, cation substitution of Csâº by FAâº was beneficial in finely tuning the band gap and in exciton recombination kinetics, improving the structural stability, and raising the absolute quantum yields up to 85%. With further assistance of anion replacement, full-spectral visible emissions in the wavelength range of 450â750 nm; narrow full width at half-maxima, and a wide color gamut, encompassing 130% of National Television System Committee television color standard, were achieved. Finally, CsâââFAâPbXâ-polymer films retaining multicolor luminescence are prepared and a prototype white light-emitting diode device was constructed using green Csâ.âFAâ.âPbBrâ and red Csâ.âFAâ.âBrâ.âIâ.â QDs as color converters, certainly suggesting their potential applications in the optoelectronics field.
Keywords	ambient temperature ; bromine ; cations ; cesium ; color ; crystallization ; emissions ; iodine ; luminescence ; quantum dots ; television ; wavelengths
Language	English
Dates of publication	2017-0621
Size	p. 20671-20678.
Publishing place	American Chemical Society
Document type	Article
ISSN	1944-8252
DOI	10.1021/acsami.7b05429
Database	NAL-Catalogue (AGRICOLA)

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Article ; Online: Density functional study of closed-shell attraction on X(ML)3 + (X = O, S, Se; M = Au, Ag, Cu) systems.

Fang, Hua / Wang, Shu-Guang

Journal of molecular modeling

2007 Volume 13, Issue 1, Page(s) 255–265

Abstract: ... ML)(3) (+)(X = O, S, Se; M = Au, Ag, Cu). Using a scalar-relativistic density functional approach ... With the help of quantum mechanical calculations, we have examined the series of central system X ...

Abstract	With the help of quantum mechanical calculations, we have examined the series of central system X(ML)(3) (+)(X = O, S, Se; M = Au, Ag, Cu). Using a scalar-relativistic density functional approach, we studied the geometry structures, Mulliken populations and charges of the systems. Structure parameters of the experimental systems are reproduced well with Xalpha method. The metallophilic interaction energy is analyzed and decomposed. For the systems with different central atoms and different metal atoms, the nature of the metallophilic attraction interaction is analyzed.
MeSH term(s)	Chemistry/methods ; Computer Simulation ; Copper/chemistry ; Electrons ; Gold/chemistry ; Models, Chemical ; Models, Molecular ; Models, Theoretical ; Oxygen/chemistry ; Selenium/chemistry ; Silver/chemistry ; Sulfur/chemistry ; Thermodynamics
Chemical Substances	Silver (3M4G523W1G) ; Sulfur (70FD1KFU70) ; Gold (7440-57-5) ; Copper (789U1901C5) ; Selenium (H6241UJ22B) ; Oxygen (S88TT14065)
Language	English
Publishing date	2007-01
Publishing country	Germany
Document type	Journal Article ; Research Support, Non-U.S. Gov't
ZDB-ID	1284729-x
ISSN	0948-5023 ; 1610-2940
ISSN (online)	0948-5023
ISSN	1610-2940
DOI	10.1007/s00894-006-0156-5
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Article: The Origin of Capacity Fade in the Li2MnO3Â·LiMO2 (M = Li, Ni, Co, Mn) Microsphere Positive Electrode: An Operando Neutron Diffraction and Transmission X-ray Microscopy Study

Chen, Chih-Jung / Lee Po-Han / Liu Ru-Shi / Mori Tatsuhiro / Pang Wei Kong / Peterson Vanessa K / Sharma Neeraj / Song Yen-Fang / Wang Chun-Chieh / Wu She-huang

Journal of the American Chemical Society. 2016 July 20, v. 138, no. 28

2016

Abstract: The mechanism of capacity fade of the LiâMnOâÂ·LiMOâ (M = Li, Ni, Co, Mn) composite positive ... transmission X-ray microscopy methods, enabling the phase, crystallographic, and morphological evolution ... of 73(1) wt % R3Ìm LiMOâ with the remaining 27(1) wt % C2/m LiâMnOâ likely existing ...

Abstract	The mechanism of capacity fade of the LiâMnOâÂ·LiMOâ (M = Li, Ni, Co, Mn) composite positive electrode within a full cell was investigated using a combination of operando neutron powder diffraction and transmission X-ray microscopy methods, enabling the phase, crystallographic, and morphological evolution of the material during electrochemical cycling to be understood. The electrode was shown to initially consist of 73(1) wt % R3Ìm LiMOâ with the remaining 27(1) wt % C2/m LiâMnOâ likely existing as an intergrowth. Cracking in the LiâMnOâÂ·LiMOâ electrode particle under operando microscopy observation was revealed to be initiated by the solid-solution reaction of the LiMOâ phase on charge to 4.55 V vs Liâº/Li and intensified during further charge to 4.7 V vs Liâº/Li during the concurrent two-phase reaction of the LiMOâ phase, involving the largest lattice change of any phase, and oxygen evolution from the LiâMnOâ phase. Notably, significant healing of the generated cracks in the LiâMnOâÂ·LiMOâ electrode particle occurred during subsequent lithiation on discharge, with this rehealing being principally associated with the solid-solution reaction of the LiMOâ phase. This work reveals that while it is the reduction of lattice size of electrode phases during charge that results in cracking of the LiâMnOâÂ·LiMOâ electrode particle, with the extent of cracking correlated to the magnitude of the size change, crack healing is possible in the reverse solid-solution reaction occurring during discharge. Importantly, it is the phase separation during the two-phase reaction of the LiMOâ phase that prevents the complete healing of the electrode particle, leading to pulverization over extended cycling. This work points to the minimization of behavior leading to phase separation, such as two-phase and oxygen evolution, as a key strategy in preventing capacity fade of the electrode.
Keywords	cobalt ; cracking ; electrochemistry ; electrodes ; lithium ; manganese ; microscopy ; nickel ; oxygen production ; separation ; X-radiation
Language	English
Dates of publication	2016-0720
Size	p. 8824-8833.
Publishing place	American Chemical Society
Document type	Article
ZDB-ID	3155-0
ISSN	1520-5126 ; 0002-7863
ISSN (online)	1520-5126
ISSN	0002-7863
DOI	10.1021%2Fjacs.6b03932
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Article ; Online: DFT studies on nonlinear optical properties of neutral nest-shaped heterothiometallic [MOS3Py5Cu3X] (M=Mo, W; X=F, Cl, Br, I) clusters.

Tang, Guo-dong / Jiang, Zheng-jing / Li, Rong-qing / Zhang, Jin-fang / Zhang, Yu / Zhang, Chi

Spectrochimica acta. Part A, Molecular and biomolecular spectroscopy

2009 Volume 74, Issue 1, Page(s) 228–232

Abstract: ... compounds [MOS(3)Py(5)Cu(3)X] (M=Mo, W; X=F, Cl, Br, I) with the high first static hyperpolarizabilities ... increases from F to I atom. The LUMO orbitals of clusters [MoOS(3)Py(5)Cu(3)X] are comprised of Mo, O and S ... atoms while the LUMO orbitals of clusters [WOS(3)Py(5)Cu(3)X] composed of W atom and pyridine ring ...

Abstract	Theoretical calculations were carried out on some neutral nest-shaped heterothiometallic cluster compounds [MOS(3)Py(5)Cu(3)X] (M=Mo, W; X=F, Cl, Br, I) with the high first static hyperpolarizabilities beta values. The geometries of these cluster compounds were optimized by the restricted DFT method at B3LYP level with LanL2DZ base set without any constrains. In order to understand the relationship between the first static hyperpolarizabilities and the compositions of these clusters, the frontier orbital compositions and energy gaps between the HOMO and LUMO orbitals were calculated and analysed. In these clusters the HOMO orbitals are mainly composed of halogen atoms and the first static hyperpolarizability increases from F to I atom. The LUMO orbitals of clusters [MoOS(3)Py(5)Cu(3)X] are comprised of Mo, O and S atoms while the LUMO orbitals of clusters [WOS(3)Py(5)Cu(3)X] composed of W atom and pyridine ring. The energy gaps between the HOMO and LUMO orbitals of the clusters [MoOS(3)Py(5)Cu(3)X] are smaller than those of the clusters [WOS(3)Py(5)Cu(3)X]. As a result the first static hyperpolarizability values of the clusters [MoOS(3)Py(5)Cu(3)X] are higher than those of the clusters [WOS(3)Py(5)Cu(3)X].
MeSH term(s)	Absorptiometry, Photon ; Copper/chemistry ; Halogens/chemistry ; Metals/chemistry ; Models, Molecular ; Models, Theoretical ; Molecular Conformation ; Molybdenum/chemistry ; Optics and Photonics ; Pyridines/chemistry ; Sulfur Compounds/chemistry
Chemical Substances	Halogens ; Metals ; Pyridines ; Sulfur Compounds ; Copper (789U1901C5) ; Molybdenum (81AH48963U)
Language	English
Publishing date	2009-09-15
Publishing country	England
Document type	Journal Article ; Research Support, Non-U.S. Gov't
ZDB-ID	210413-1
ISSN	1873-3557 ; 0370-8322 ; 0584-8539 ; 1386-1425
ISSN (online)	1873-3557
ISSN	0370-8322 ; 0584-8539 ; 1386-1425
DOI	10.1016/j.saa.2009.06.035
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