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Article ; Online: H

Humphreys, Susan / von Ungern-Sternberg, Britta Sylvia / Skowno, Justin / Williams, Tara / Taylor, Julia / Taverner, Fiona / Gibbons, Kristen / Burgoyne, Laura / Sommerfield, David / Stephens, Philip / Hallett, Ben / Vijayasekaran, Shyan / Slee, Nicola / Burns, Hannah / Sowa, Marcin / Davidson, Andrew / Schibler, Andreas

BMJ open

2019 Volume 9, Issue 10, Page(s) e031873

Abstract: Introduction: Hypoxaemia during anaesthesia for tubeless upper airway surgery in children with abnormal airways is common due to the complexity of balancing adequate depth of anaesthesia with maintenance of spontaneous breathing and providing an ... ...

Abstract	Introduction: Hypoxaemia during anaesthesia for tubeless upper airway surgery in children with abnormal airways is common due to the complexity of balancing adequate depth of anaesthesia with maintenance of spontaneous breathing and providing an uninterrupted field of view of the upper airway for the surgeon. High-flow nasal oxygenation (HIGH-FLOW) can prolong safe apnoea time and be used in children with abnormal airways but to date has not been compared with the alternative technique of low-flow nasal oxygenation (LOW-FLOW). The aim is to investigate if use of HIGH-FLOW can reduce the number of hypoxaemic events requiring rescue oxygenation compared with LOW-FLOW. METHODS AND ANALYSIS: Ethics and dissemination: Ethical approval has been obtained by Children's Health Queensland Human Research Ethics Committee (HREC/18/QRCH/130). The trial commenced recruitment in 2018. The primary manuscript will be submitted for publication in a peer-reviewed journal. Trial registration number: The HAMSTER is registered with the Australia and New Zealand Clinical TrialsRegistry: ACTRN12618000949280.
MeSH term(s)	Adolescent ; Anesthesia, General ; Child ; Child, Preschool ; Female ; Humans ; Hypoxia/prevention & control ; Infant ; Infant, Newborn ; Male ; Multicenter Studies as Topic ; Noninvasive Ventilation/methods ; Oxygen Inhalation Therapy/methods ; Randomized Controlled Trials as Topic ; Respiratory System/surgery
Language	English
Publishing date	2019-10-14
Publishing country	England
Document type	Clinical Trial Protocol ; Journal Article ; Research Support, Non-U.S. Gov't
ZDB-ID	2599832-8
ISSN	2044-6055 ; 2044-6055
ISSN (online)	2044-6055
ISSN	2044-6055
DOI	10.1136/bmjopen-2019-031873
Database	MEDical Literature Analysis and Retrieval System OnLINE

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Article ; Online: H

Taylor, Jordan W / Harman, W Hill

Chemical communications (Cambridge, England)

2020 Volume 56, Issue 89, Page(s) 13804–13807

Abstract: The water reactivity of the boroauride complex ([Au( ... ...

Abstract	The water reactivity of the boroauride complex ([Au(B
Language	English
Publishing date	2020-10-20
Publishing country	England
Document type	Journal Article
ZDB-ID	1472881-3
ISSN	1364-548X ; 1359-7345 ; 0009-241X
ISSN (online)	1364-548X
ISSN	1359-7345 ; 0009-241X
DOI	10.1039/d0cc05261b
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Article ; Online: Insights into H

Taylor, Megan F / Black, Michael A / Hampton, Mark B / Ledgerwood, Elizabeth C

Free radical research

2023 Volume 56, Issue 9-10, Page(s) 666–676

Abstract: Hydrogen peroxide (H ...

Abstract	Hydrogen peroxide (H
MeSH term(s)	Animals ; Humans ; Hydrogen Peroxide/pharmacology ; Jurkat Cells ; Signal Transduction ; Oxidants/pharmacology ; Oxidative Stress ; Gene Expression ; Mammals
Chemical Substances	Hydrogen Peroxide (BBX060AN9V) ; Oxidants
Language	English
Publishing date	2023-01-11
Publishing country	England
Document type	Journal Article
ZDB-ID	1194130-3
ISSN	1029-2470 ; 1071-5762
ISSN (online)	1029-2470
ISSN	1071-5762
DOI	10.1080/10715762.2023.2165073
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Article ; Online: Chemical shielding of H

Communications chemistry

2021 Volume 4, Issue 1, Page(s) 135

Abstract: ... within a fullerene cage. Here we determine the location of an H ...

Abstract	Molecular surgery provides the opportunity to study relatively large molecules encapsulated within a fullerene cage. Here we determine the location of an H
Language	English
Publishing date	2021-09-22
Publishing country	England
Document type	Journal Article
ZDB-ID	2929562-2
ISSN	2399-3669 ; 2399-3669
ISSN (online)	2399-3669
ISSN	2399-3669
DOI	10.1038/s42004-021-00569-0
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Article ; Online: γ C-H Functionalization of Amines via Triple H-Atom Transfer of a Vinyl Sulfonyl Radical Chaperone.

Herbort, James H / Bednar, Taylor N / Chen, Andrew D / RajanBabu, T V / Nagib, David A

Journal of the American Chemical Society

2022 Volume 144, Issue 29, Page(s) 13366–13373

Abstract: ... from their aliphatic precursors. The strategy employs a triple H-atom transfer (HAT) cascade, entailing (i) cobalt ... catalyzed metal-HAT (MHAT), (ii) carbon-to-carbon 1,6-HAT, and (iii) Co-H regeneration via MHAT. A new class ...

Abstract	A selective, remote desaturation has been developed to rapidly access homoallyl amines from their aliphatic precursors. The strategy employs a triple H-atom transfer (HAT) cascade, entailing (i) cobalt-catalyzed metal-HAT (MHAT), (ii) carbon-to-carbon 1,6-HAT, and (iii) Co-H regeneration via MHAT. A new class of sulfonyl radical chaperone (to rapidly access and direct remote, radical reactivity) enables remote desaturation of diverse amines, amino acids, and peptides with excellent site-, chemo-, and regioselectivity. The key, enabling C-to-C HAT step in this cascade was computationally designed to satisfy both thermodynamic (bond strength) and kinetic (polarity) requirements, and it has been probed via regioselectivity, isomerization, and competition experiments. We have also interrupted this radical transfer dehydrogenation to achieve γ-selective C-Cl, C-CN, and C-N bond formations.
MeSH term(s)	Amines/chemistry ; Amino Acids ; Carbon/chemistry ; Kinetics
Chemical Substances	Amines ; Amino Acids ; Carbon (7440-44-0)
Language	English
Publishing date	2022-07-12
Publishing country	United States
Document type	Journal Article ; Research Support, N.I.H., Extramural
ZDB-ID	3155-0
ISSN	1520-5126 ; 0002-7863
ISSN (online)	1520-5126
ISSN	0002-7863
DOI	10.1021/jacs.2c05266
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Article ; Online: Dietary Intake of Athletes at the World Masters Athletics Championships as Assessed by Single 24 h Recall.

Leonhardt, Taylor P M / Bristol, Ainsley / McLaurin, Natalie / Forbes, Scott C / Tanaka, Hirofumi / Frings-Meuthen, Petra / Pesta, Dominik / Rittweger, Jörn / Chilibeck, Philip D

Nutrients

2024 Volume 16, Issue 4

Abstract: ... 1) events provided 24 h dietary recalls while participating in the games. Carbohydrate intake was ...

Abstract	Proper dietary intake is important for masters athletes because of the physiological changes that occur with aging and the unique nutritional needs when competing at high levels. We evaluated the dietary intake of masters athletes competing at the World Masters Athletics Championships (outdoor games, Tampere, Finland, 2022, and indoor games, Torun, Poland, 2023). A total of 43 athletes (16 females and 27 males, mean age 59.2 ± 10.3 y, height 168 ± 8 cm, and body mass 62.3 ± 10.8 kg) participating in endurance (n = 21), sprint (n = 16), jumping (2), multi-component (e.g., decathlon; n = 3), and throwing (n = 1) events provided 24 h dietary recalls while participating in the games. Carbohydrate intake was below the recommended levels for endurance athletes. Protein intake was below the recommended levels for masters athletes, except for female athletes involved in power events (i.e., sprinters and jumpers). Other nutrient intakes that were below the recommended levels included vitamins D and E, calcium, potassium, vitamin A (except for female endurance athletes), folate (except for female power athletes), vitamin C for female endurance athletes, vitamin K and fiber for males, and zinc for endurance athletes. We conclude that while competing at world championships, many athletes are not consuming the recommended levels of carbohydrates, protein, and micronutrients. Athletes attending these games would benefit from increased nutritional support.
MeSH term(s)	Male ; Humans ; Female ; Middle Aged ; Aged ; Energy Intake ; Dietary Carbohydrates ; Sports/physiology ; Athletes ; Eating ; Dietary Proteins
Chemical Substances	Dietary Carbohydrates ; Dietary Proteins
Language	English
Publishing date	2024-02-19
Publishing country	Switzerland
Document type	Journal Article
ZDB-ID	2518386-2
ISSN	2072-6643 ; 2072-6643
ISSN (online)	2072-6643
ISSN	2072-6643
DOI	10.3390/nu16040564
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Article ; Online: Factor H Autoantibodies and Complement-Mediated Diseases.

Zhang, Yuzhou / Ghiringhelli Borsa, Nicolo / Shao, Dingwu / Dopler, Arthur / Jones, Michael B / Meyer, Nicole C / Pitcher, Gabriella R / Taylor, Amanda O / Nester, Carla M / Schmidt, Christoph Q / Smith, Richard J H

Frontiers in immunology

2020 Volume 11, Page(s) 607211

Abstract: Factor H (FH), a member of the regulators-of-complement-activation (RCA) family of proteins ...

Abstract	Factor H (FH), a member of the regulators-of-complement-activation (RCA) family of proteins, circulates in human plasma at concentrations of 180-420 mg/L where it controls the alternative pathway (AP) of complement in the fluid phase and on cell surfaces. When the regulatory function of FH is impaired, complement-mediated tissue injury and inflammation occur, leading to diseases such as atypical hemolytic uremic syndrome (a thrombotic microangiopathy or TMA), C3 glomerulopathy (C3G) and monoclonal gammopathy of renal significance (MGRS). A pathophysiological cause of compromised FH function is the development of autoantibodies to various domains of the FH protein. FH autoantibodies (FHAAs) are identified in 10.9% of patients with aHUS, 3.2% of patients with C3G, and rarely in patients with MGRS. The phenotypic variability of FHAA-mediated disease reflects both the complexity of FH and the epitope specificity of FHAA for select regions of the native protein. In this paper, we have characterized FHAA epitopes in a large cohort of patients diagnosed with TMA, C3G or MGRS. We explore the epitopes recognized by FHAAs in these diseases and the association of FHAAs with the genetic deletion of both copies of the
MeSH term(s)	Adolescent ; Adult ; Aged ; Aged, 80 and over ; Atypical Hemolytic Uremic Syndrome/blood ; Atypical Hemolytic Uremic Syndrome/epidemiology ; Atypical Hemolytic Uremic Syndrome/genetics ; Atypical Hemolytic Uremic Syndrome/immunology ; Autoantibodies/blood ; Biomarkers/blood ; Child ; Child, Preschool ; Complement C3b Inactivator Proteins/genetics ; Complement Factor H/immunology ; Epitopes ; Female ; Gene Deletion ; Genetic Predisposition to Disease ; Glomerulonephritis/blood ; Glomerulonephritis/epidemiology ; Glomerulonephritis/genetics ; Glomerulonephritis/immunology ; Humans ; Infant ; Male ; Middle Aged ; Paraproteinemias/blood ; Paraproteinemias/epidemiology ; Paraproteinemias/genetics ; Paraproteinemias/immunology ; Phenotype ; Prevalence ; Retrospective Studies ; United States/epidemiology ; Young Adult
Chemical Substances	Autoantibodies ; Biomarkers ; CFH protein, human ; CFHR1 protein, human ; Complement C3b Inactivator Proteins ; Epitopes ; Complement Factor H (80295-65-4)
Language	English
Publishing date	2020-12-15
Publishing country	Switzerland
Document type	Journal Article ; Research Support, N.I.H., Extramural
ZDB-ID	2606827-8
ISSN	1664-3224 ; 1664-3224
ISSN (online)	1664-3224
ISSN	1664-3224
DOI	10.3389/fimmu.2020.607211
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Article: γ C–H Functionalization of Amines via Triple H-Atom Transfer of a Vinyl Sulfonyl Radical Chaperone

Herbort, James H. / Bednar, Taylor N. / Chen, Andrew D. / RajanBabu, T. V. / Nagib, David A.

Journal of the American Chemical Society. 2022 July 12, v. 144, no. 29

2022

Abstract	A selective, remote desaturation has been developed to rapidly access homoallyl amines from their aliphatic precursors. The strategy employs a triple H-atom transfer (HAT) cascade, entailing (i) cobalt-catalyzed metal-HAT (MHAT), (ii) carbon-to-carbon 1,6-HAT, and (iii) Co–H regeneration via MHAT. A new class of sulfonyl radical chaperone (to rapidly access and direct remote, radical reactivity) enables remote desaturation of diverse amines, amino acids, and peptides with excellent site-, chemo-, and regioselectivity. The key, enabling C-to-C HAT step in this cascade was computationally designed to satisfy both thermodynamic (bond strength) and kinetic (polarity) requirements, and it has been probed via regioselectivity, isomerization, and competition experiments. We have also interrupted this radical transfer dehydrogenation to achieve γ-selective C–Cl, C–CN, and C–N bond formations.
Keywords	carbon-hydrogen bond activation ; dehydrogenation ; isomerization ; peptides ; regioselectivity ; thermodynamics
Language	English
Dates of publication	2022-0712
Size	p. 13366-13373.
Publishing place	American Chemical Society
Document type	Article
ZDB-ID	3155-0
ISSN	1520-5126 ; 0002-7863
ISSN (online)	1520-5126
ISSN	0002-7863
DOI	10.1021/jacs.2c05266
Database	NAL-Catalogue (AGRICOLA)

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Article ; Online: Observation of tt[over ¯]H Production.

Sirunyan, A M / Tumasyan, A / Adam, W / Ambrogi, F / Asilar, E / Bergauer, T / Brandstetter, J / Dragicevic, M / Erö, J / Escalante Del Valle, A / Flechl, M / Frühwirth, R / Ghete, V M / Hrubec, J / Jeitler, M / Krammer, N / Krätschmer, I / Liko, D / Madlener, T /

Mikulec, I / Rad, N / Rohringer, H / Schieck, J / Schöfbeck, R / Spanring, M / Spitzbart, D / Taurok, A / Waltenberger, W / Wittmann, J / Wulz, C-E / Zarucki, M / Chekhovsky, V / Mossolov, V / Suarez Gonzalez, J / De Wolf, E A / Di Croce, D / Janssen, X / Lauwers, J / Pieters, M / Van De Klundert, M / Van Haevermaet, H / Van Mechelen, P / Van Remortel, N / Abu Zeid, S / Blekman, F / D'Hondt, J / De Bruyn, I / De Clercq, J / Deroover, K / Flouris, G / Lontkovskyi, D / Lowette, S / Marchesini, I / Moortgat, S / Moreels, L / Python, Q / Skovpen, K / Tavernier, S / Van Doninck, W / Van Mulders, P / Van Parijs, I / Beghin, D / Bilin, B / Brun, H / Clerbaux, B / De Lentdecker, G / Delannoy, H / Dorney, B / Fasanella, G / Favart, L / Goldouzian, R / Grebenyuk, A / Kalsi, A K / Lenzi, T / Luetic, J / Postiau, N / Starling, E / Thomas, L / Vander Velde, C / Vanlaer, P / Vannerom, D / Wang, Q / Cornelis, T / Dobur, D / Fagot, A / Gul, M / Khvastunov, I / Poyraz, D / Roskas, C / Trocino, D / Tytgat, M / Verbeke, W / Vermassen, B / Vit, M / Zaganidis, N / Bakhshiansohi, H / Bondu, O / Brochet, S / Bruno, G / Caputo, C / David, P / Delaere, C / Delcourt, M / Francois, B / Giammanco, A / Krintiras, G / Lemaitre, V / Magitteri, A / Mertens, A / Musich, M / Piotrzkowski, K / Saggio, A / Vidal Marono, M / Wertz, S / Zobec, J / Alves, F L / Alves, G A / Brito, L / Correa Martins Junior, M / Correia Silva, G / Hensel, C / Moraes, A / Pol, M E / Rebello Teles, P / Belchior Batista Das Chagas, E / Carvalho, W / Chinellato, J / Coelho, E / Da Costa, E M / Da Silveira, G G / De Jesus Damiao, D / De Oliveira Martins, C / Fonseca De Souza, S / Malbouisson, H / Matos Figueiredo, D / Melo De Almeida, M / Mora Herrera, C / Mundim, L / Nogima, H / Prado Da Silva, W L / Sanchez Rosas, L J / Santoro, A / Sznajder, A / Thiel, M / Tonelli Manganote, E J / Torres Da Silva De Araujo, F / Vilela Pereira, A / Ahuja, S / Bernardes, C A / Calligaris, L / Fernandez Perez Tomei, T R / Gregores, E M / Mercadante, P G / Novaes, S F / Padula, Sandra S / Romero Abad, D / Aleksandrov, A / Hadjiiska, R / Iaydjiev, P / Marinov, A / Misheva, M / Rodozov, M / Shopova, M / Sultanov, G / Dimitrov, A / Litov, L / Pavlov, B / Petkov, P / Fang, W / Gao, X / Yuan, L / Ahmad, M / Bian, J G / Chen, G M / Chen, H S / Chen, M / Chen, Y / Jiang, C H / Leggat, D / Liao, H / Liu, Z / Romeo, F / Shaheen, S M / Spiezia, A / Tao, J / Wang, C / Wang, Z / Yazgan, E / Zhang, H / Zhao, J / Ban, Y / Chen, G / Levin, A / Li, J / Li, L / Li, Q / Mao, Y / Qian, S J / Wang, D / Xu, Z / Wang, Y / Avila, C / Cabrera, A / Carrillo Montoya, C A / Chaparro Sierra, L F / Florez, C / González Hernández, C F / Segura Delgado, M A / Courbon, B / Godinovic, N / Lelas, D / Puljak, I / Sculac, T / Antunovic, Z / Kovac, M / Brigljevic, V / Ferencek, D / Kadija, K / Mesic, B / Starodumov, A / Susa, T / Ather, M W / Attikis, A / Kolosova, M / Mavromanolakis, G / Mousa, J / Nicolaou, C / Ptochos, F / Razis, P A / Rykaczewski, H / Finger, M / Ayala, E / Carrera Jarrin, E / Abdalla, H / Abdelalim, A A / Mohamed, A / Bhowmik, S / Carvalho Antunes De Oliveira, A / Dewanjee, R K / Ehataht, K / Kadastik, M / Raidal, M / Veelken, C / Eerola, P / Kirschenmann, H / Pekkanen, J / Voutilainen, M / Havukainen, J / Heikkilä, J K / Järvinen, T / Karimäki, V / Kinnunen, R / Lampén, T / Lassila-Perini, K / Laurila, S / Lehti, S / Lindén, T / Luukka, P / Mäenpää, T / Siikonen, H / Tuominen, E / Tuominiemi, J / Tuuva, T / Besancon, M / Couderc, F / Dejardin, M / Denegri, D / Faure, J L / Ferri, F / Ganjour, S / Givernaud, A / Gras, P / Hamel de Monchenault, G / Jarry, P / Leloup, C / Locci, E / Malcles, J / Negro, G / Rander, J / Rosowsky, A / Sahin, M Ö / Titov, M / Abdulsalam, A / Amendola, C / Antropov, I / Beaudette, F / Busson, P / Charlot, C / Granier de Cassagnac, R / Kucher, I / Lobanov, A / Martin Blanco, J / Nguyen, M / Ochando, C / Ortona, G / Pigard, P / Salerno, R / Sauvan, J B / Sirois, Y / Stahl Leiton, A G / Zabi, A / Zghiche, A / Agram, J-L / Andrea, J / Bloch, D / Brom, J-M / Chabert, E C / Cherepanov, V / Collard, C / Conte, E / Fontaine, J-C / Gelé, D / Goerlach, U / Jansová, M / Le Bihan, A-C / Tonon, N / Van Hove, P / Gadrat, S / Beauceron, S / Bernet, C / Boudoul, G / Chanon, N / Chierici, R / Contardo, D / Depasse, P / El Mamouni, H / Fay, J / Finco, L / Gascon, S / Gouzevitch, M / Grenier, G / Ille, B / Lagarde, F / Laktineh, I B / Lattaud, H / Lethuillier, M / Mirabito, L / Pequegnot, A L / Perries, S / Popov, A / Sordini, V / Vander Donckt, M / Viret, S / Zhang, S / Khvedelidze, A / Tsamalaidze, Z / Autermann, C / Feld, L / Kiesel, M K / Klein, K / Lipinski, M / Preuten, M / Rauch, M P / Schomakers, C / Schulz, J / Teroerde, M / Wittmer, B / Zhukov, V / Albert, A / Duchardt, D / Endres, M / Erdmann, M / Esch, T / Fischer, R / Ghosh, S / Güth, A / Hebbeker, T / Heidemann, C / Hoepfner, K / Keller, H / Knutzen, S / Mastrolorenzo, L / Merschmeyer, M / Meyer, A / Millet, P / Mukherjee, S / Pook, T / Radziej, M / Rath, Y / Reithler, H / Rieger, M / Scheuch, F / Schmidt, A / Teyssier, D / Flügge, G / Hlushchenko, O / Kress, T / Künsken, A / Müller, T / Nehrkorn, A / Nowack, A / Pistone, C / Pooth, O / Roy, D / Sert, H / Stahl, A / Aldaya Martin, M / Arndt, T / Asawatangtrakuldee, C / Babounikau, I / Beernaert, K / Behnke, O / Behrens, U / Bermúdez Martínez, A / Bertsche, D / Bin Anuar, A A / Borras, K / Botta, V / Campbell, A / Connor, P / Contreras-Campana, C / Costanza, F / Danilov, V / De Wit, A / Defranchis, M M / Diez Pardos, C / Domínguez Damiani, D / Eckerlin, G / Eichhorn, T / Elwood, A / Eren, E / Gallo, E / Geiser, A / Grados Luyando, J M / Grohsjean, A / Gunnellini, P / Guthoff, M / Haranko, M / Harb, A / Hauk, J / Jung, H / Kasemann, M / Keaveney, J / Kleinwort, C / Knolle, J / Krücker, D / Lange, W / Lelek, A / Lenz, T / Lipka, K / Lohmann, W / Mankel, R / Melzer-Pellmann, I-A / Meyer, A B / Meyer, M / Missiroli, M / Mittag, G / Mnich, J / Myronenko, V / Pflitsch, S K / Pitzl, D / Raspereza, A / Saibel, A / Savitskyi, M / Saxena, P / Schütze, P / Schwanenberger, C / Shevchenko, R / Singh, A / Tholen, H / Turkot, O / Vagnerini, A / Van Onsem, G P / Walsh, R / Wen, Y / Wichmann, K / Wissing, C / Zenaiev, O / Aggleton, R / Bein, S / Benato, L / Benecke, A / Blobel, V / Centis Vignali, M / Dreyer, T / Garutti, E / Gonzalez, D / Haller, J / Hinzmann, A / Karavdina, A / Kasieczka, G / Klanner, R / Kogler, R / Kovalchuk, N / Kurz, S / Kutzner, V / Lange, J / Marconi, D / Multhaup, J / Niedziela, M / Nowatschin, D / Perieanu, A / Reimers, A / Rieger, O / Scharf, C / Schleper, P / Schumann, S / Schwandt, J / Sonneveld, J / Stadie, H / Steinbrück, G / Stober, F M / Stöver, M / Troendle, D / Vanhoefer, A / Vormwald, B / Akbiyik, M / Barth, C / Baselga, M / Baur, S / Butz, E / Caspart, R / Chwalek, T / Colombo, F / De Boer, W / Dierlamm, A / El Morabit, K / Faltermann, N / Freund, B / Giffels, M / Harrendorf, M A / Hartmann, F / Heindl, S M / Husemann, U / Kassel, F / Katkov, I / Keicher, P / Kudella, S / Mildner, H / Mitra, S / Mozer, M U / Müller, Th / Plagge, M / Quast, G / Rabbertz, K / Schröder, M / Shvetsov, I / Sieber, G / Simonis, H J / Ulrich, R / Wayand, S / Waßmer, M / Weber, M / Weiler, T / Williamson, S / Wöhrmann, C / Wolf, R / Anagnostou, G / Daskalakis, G / Geralis, T / Kyriakis, A / Loukas, D / Paspalaki, G / Topsis-Giotis, I / Karathanasis, G / Kesisoglou, S / Kontaxakis, P / Panagiotou, A / Papavergou, I / Saoulidou, N / Tziaferi, E / Vellidis, K / Kousouris, K / Papakrivopoulos, I / Tsipolitis, G / Evangelou, I / Foudas, C / Gianneios, P / Katsoulis, P / Kokkas, P / Mallios, S / Manthos, N / Papadopoulos, I / Paradas, E / Strologas, J / Triantis, F A / Tsitsonis, D / Bartók, M / Csanad, M / Filipovic, N / Major, P / Nagy, M I / Pasztor, G / Surányi, O / Veres, G I / Bencze, G / Hajdu, C / Horvath, D / Hunyadi, Á / Sikler, F / Veszpremi, V / Vesztergombi, G / Vámi, T Á / Beni, N / Czellar, S 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Physical review letters

2018 Volume 120, Issue 23, Page(s) 231801

Abstract: The observation of Higgs boson production in association with a top quark-antiquark pair is reported, based on a combined analysis of proton-proton collision data at center-of-mass energies of sqrt[s]=7, 8, and 13 TeV, corresponding to integrated ... ...

Abstract	The observation of Higgs boson production in association with a top quark-antiquark pair is reported, based on a combined analysis of proton-proton collision data at center-of-mass energies of sqrt[s]=7, 8, and 13 TeV, corresponding to integrated luminosities of up to 5.1, 19.7, and 35.9 fb^{-1}, respectively. The data were collected with the CMS detector at the CERN LHC. The results of statistically independent searches for Higgs bosons produced in conjunction with a top quark-antiquark pair and decaying to pairs of W bosons, Z bosons, photons, τ leptons, or bottom quark jets are combined to maximize sensitivity. An excess of events is observed, with a significance of 5.2 standard deviations, over the expectation from the background-only hypothesis. The corresponding expected significance from the standard model for a Higgs boson mass of 125.09 GeV is 4.2 standard deviations. The combined best fit signal strength normalized to the standard model prediction is 1.26_{-0.26}^{+0.31}.
Language	English
Publishing date	2018-06-08
Publishing country	United States
Document type	Journal Article
ZDB-ID	208853-8
ISSN	1079-7114 ; 0031-9007
ISSN (online)	1079-7114
ISSN	0031-9007
DOI	10.1103/PhysRevLett.120.231801
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Article ; Online: Allylic C-H functionalization

Nelson, Taylor A F / Hollerbach, Michael R / Blakey, Simon B

Dalton transactions (Cambridge, England : 2003)

2020 Volume 49, Issue 40, Page(s) 13928–13935

Abstract: Allylic C-H functionalization catalysed by group 9 Cp* transition-metal complexes has recently ... gained significant attention. These reactions have expanded allylic C-H functionalization to include di ... several catalytic C-N, C-O, and C-C bond forming allylic C-H functionalization reactions have been reported ...

Abstract	Allylic C-H functionalization catalysed by group 9 Cp* transition-metal complexes has recently gained significant attention. These reactions have expanded allylic C-H functionalization to include di- and trisubstituted olefins, and a broad range of coupling partners. More specifically, several catalytic C-N, C-O, and C-C bond forming allylic C-H functionalization reactions have been reported, proceeding via MCp*-π-allyl intermediates. Herein we present an overview of these reactions by mechanistic paradigm. We also place this information in context of recent advances, as well as, limitations that remain for this class of reactions.
Language	English
Publishing date	2020-09-10
Publishing country	England
Document type	Journal Article
ZDB-ID	1472887-4
ISSN	1477-9234 ; 1364-5447 ; 0300-9246 ; 1477-9226
ISSN (online)	1477-9234 ; 1364-5447
ISSN	0300-9246 ; 1477-9226
DOI	10.1039/d0dt02313b
Database	MEDical Literature Analysis and Retrieval System OnLINE

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