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Article: Biogenic secondary organic aerosols: A review on formation mechanism, analytical challenges and environmental impacts

Mahilang, Mithlesh / Deb, Manas Kanti / Pervez, Shamsh

Chemosphere. 2021 Jan., v. 262

2021

Abstract: The review initiates with current state of information on the atmospheric reaction mechanism of biogenic volatile organic compounds (BVOCs) and its fate in the atmosphere. The plants release BVOCs, i.e., isoprene, monoterpenes, and sesquiterpenes, which ... ...

Abstract	The review initiates with current state of information on the atmospheric reaction mechanism of biogenic volatile organic compounds (BVOCs) and its fate in the atmosphere. The plants release BVOCs, i.e., isoprene, monoterpenes, and sesquiterpenes, which form secondary organic aerosols (SOA) upon oxidation. These oxidation reactions are primarily influenced by solar radiations along with other meteorological parameters viz.; temperature and relative humidity, therefore, the chemistry behind SOA formation is different during day than the night time. The review throws light upon the day and nighttime formation mechanism of SOA, recent advancements in the analytical techniques available for the measurements, and its impact on the environment. Studies have revealed that day time SOA formation is dominated by OH and O₃, however, NOx initiated SOA production is dominated during night. The formation mechanism addresses that the gaseous products of VOCs are firstly formed and then partitioned over the pre-existing particles. New particle formation and biomass-derived aerosols are found to be responsible for enhanced SOA formation. 2-Dimensional gas chromatography-mass spectrometer (2D-GC/MS) is observed to be best for the analysis of organic aerosols. Radiative forcing (RF) SOA is observed to be a useful parameter to evaluate the environmental impacts of SOA and reviewed studies have shown mean RF in the ranges of −0.27 to +0.20 W m⁻².
Keywords	environmental impact ; isoprene ; monoterpenoids ; oxidation ; reaction mechanisms ; relative humidity ; sesquiterpenoids ; spectrometers ; temperature ; volatile organic compounds
Language	English
Dates of publication	2021-01
Publishing place	Elsevier Ltd
Document type	Article
Note	NAL-light
ZDB-ID	120089-6
ISSN	1879-1298 ; 0045-6535 ; 0366-7111
ISSN (online)	1879-1298
ISSN	0045-6535 ; 0366-7111
DOI	10.1016/j.chemosphere.2020.127771
Database	NAL-Catalogue (AGRICOLA)

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Article ; Online: Biogenic secondary organic aerosols: A review on formation mechanism, analytical challenges and environmental impacts.

Mahilang, Mithlesh / Deb, Manas Kanti / Pervez, Shamsh

Chemosphere

2020 Volume 262, Page(s) 127771

Abstract	The review initiates with current state of information on the atmospheric reaction mechanism of biogenic volatile organic compounds (BVOCs) and its fate in the atmosphere. The plants release BVOCs, i.e., isoprene, monoterpenes, and sesquiterpenes, which form secondary organic aerosols (SOA) upon oxidation. These oxidation reactions are primarily influenced by solar radiations along with other meteorological parameters viz.; temperature and relative humidity, therefore, the chemistry behind SOA formation is different during day than the night time. The review throws light upon the day and nighttime formation mechanism of SOA, recent advancements in the analytical techniques available for the measurements, and its impact on the environment. Studies have revealed that day time SOA formation is dominated by OH and O
MeSH term(s)	Aerosols/analysis ; Aerosols/chemistry ; Air Pollutants/analysis ; Air Pollutants/chemistry ; Atmosphere/chemistry ; Butadienes/analysis ; Butadienes/chemistry ; Hemiterpenes/analysis ; Hemiterpenes/chemistry ; Monoterpenes/analysis ; Monoterpenes/chemistry ; Oxidation-Reduction ; Temperature ; Volatile Organic Compounds/analysis ; Volatile Organic Compounds/chemistry
Chemical Substances	Aerosols ; Air Pollutants ; Butadienes ; Hemiterpenes ; Monoterpenes ; Volatile Organic Compounds ; isoprene (0A62964IBU)
Language	English
Publishing date	2020-08-07
Publishing country	England
Document type	Journal Article ; Review
ZDB-ID	120089-6
ISSN	1879-1298 ; 0045-6535 ; 0366-7111
ISSN (online)	1879-1298
ISSN	0045-6535 ; 0366-7111
DOI	10.1016/j.chemosphere.2020.127771
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Article: Influence of fireworks emission on aerosol aging process at lower troposphere and associated health risks in an urban region of eastern central India.

Mahilang, Mithlesh / Deb, Manas Kanti / Nirmalkar, Jayant / Pervez, Shamsh

Atmospheric pollution research

2020 Volume 11, Issue 7, Page(s) 1127–1141

Abstract: To study the influence of fireworks in atmospheric aerosols and their effect on health during the extreme firework days, fireworks tracer metals and carbonaceous species in size-distributed aerosols in the lower troposphere at Raipur in eastern central ... ...

Abstract	To study the influence of fireworks in atmospheric aerosols and their effect on health during the extreme firework days, fireworks tracer metals and carbonaceous species in size-distributed aerosols in the lower troposphere at Raipur in eastern central India were investigated during the 2018 Deepawali festival. Aerosol samples were collected, before Deepawali period (BDP, n = 5), during Deepawali period (DDP, n = 5) and after Deepawali period (ADP, n = 5). Bimodal size-distribution with intense fine mode peak was found for Na during DDP. Bimodal distribution with fine mode intense peak was found for K during DDP. The bimodal size distribution of K was found common for other events because of biomass burning emissions, whereas high intense peak during DDP indicated mixed sources from biomass burning and fireworks. During DDP, K and Ca were well correlated (r
Keywords	covid19
Language	English
Publishing date	2020-04-21
Publishing country	Turkey
Document type	Journal Article
ZDB-ID	2645757-X
ISSN	1309-1042
ISSN	1309-1042
DOI	10.1016/j.apr.2020.04.009
Database	MEDical Literature Analysis and Retrieval System OnLINE

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Article: Biogenic secondary organic aerosol formation in an urban area of eastern central India: Seasonal variation, size distribution and source characterization

Mahilang, Mithlesh / Deb, Manas Kanti / Pervez, Shamsh / Tiwari, Swapnil / Jain, Vikas Kumar

Environmental research. 2021 Apr., v. 195

2021

Abstract: Samples of ambient aerosols were collected at an urban site of eastern central India from monsoon to summer 2016–17 for the characterization of biogenic secondary organic aerosols (BSOA). The BSOA tracers derived from isoprene, α/β-pinene and β- ... ...

Abstract	Samples of ambient aerosols were collected at an urban site of eastern central India from monsoon to summer 2016–17 for the characterization of biogenic secondary organic aerosols (BSOA). The BSOA tracers derived from isoprene, α/β-pinene and β-caryophyllene in size-distributed aerosols were studied. Concentrations of total SOAI (Isoprene secondary organic aerosols) were found more abundant than α/β-pinene in summer, while contradictory trends were found in the winter season, where SOAM (monoterpene derived SOA) and SOAS (sesquiterpenes derived SOA) were dominated. Size-distribution study revealed that most of the BSOA were formed in the aerosol phase and dominated in fine mode, except cis-pinonic acid. They were formed in the gaseous phase and partitioned onto the aerosol phase. The alkaline nature of mineral dust particles that triggered the adsorption of gaseous species onto pre-existing particles could be the reason for bimodal size distribution with major coarse mode peak and miner fine mode peak. Temporal variations suggest that the BSOA must be derived from terrestrial vegetation and biomass burning. The isoprene SOC (secondary organic carbon) contributed 0.91%, 1.38%, 0.88% and 1.04% to OC during winter, summer, post-monsoon and monsoon season, respectively. The isoprene SOC in fine mode was found to be higher than the coarse mode.
Keywords	adsorption ; aerosols ; biomass ; dust ; isoprene ; monsoon season ; organic carbon ; research ; seasonal variation ; summer ; urban areas ; vegetation ; winter ; India
Language	English
Dates of publication	2021-04
Publishing place	Elsevier Inc.
Document type	Article
Note	NAL-AP-2-clean
ZDB-ID	205699-9
ISSN	1096-0953 ; 0013-9351
ISSN (online)	1096-0953
ISSN	0013-9351
DOI	10.1016/j.envres.2021.110802
Database	NAL-Catalogue (AGRICOLA)

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Article ; Online: Biogenic secondary organic aerosol formation in an urban area of eastern central India: Seasonal variation, size distribution and source characterization.

Mahilang, Mithlesh / Deb, Manas Kanti / Pervez, Shamsh / Tiwari, Swapnil / Jain, Vikas Kumar

Environmental research

2021 Volume 195, Page(s) 110802

Abstract: Samples of ambient aerosols were collected at an urban site of eastern central India from monsoon to summer 2016-17 for the characterization of biogenic secondary organic aerosols (BSOA). The BSOA tracers derived from isoprene, α/β-pinene and β- ... ...

Abstract	Samples of ambient aerosols were collected at an urban site of eastern central India from monsoon to summer 2016-17 for the characterization of biogenic secondary organic aerosols (BSOA). The BSOA tracers derived from isoprene, α/β-pinene and β-caryophyllene in size-distributed aerosols were studied. Concentrations of total SOAI (Isoprene secondary organic aerosols) were found more abundant than α/β-pinene in summer, while contradictory trends were found in the winter season, where SOAM (monoterpene derived SOA) and SOAS (sesquiterpenes derived SOA) were dominated. Size-distribution study revealed that most of the BSOA were formed in the aerosol phase and dominated in fine mode, except cis-pinonic acid. They were formed in the gaseous phase and partitioned onto the aerosol phase. The alkaline nature of mineral dust particles that triggered the adsorption of gaseous species onto pre-existing particles could be the reason for bimodal size distribution with major coarse mode peak and miner fine mode peak. Temporal variations suggest that the BSOA must be derived from terrestrial vegetation and biomass burning. The isoprene SOC (secondary organic carbon) contributed 0.91%, 1.38%, 0.88% and 1.04% to OC during winter, summer, post-monsoon and monsoon season, respectively. The isoprene SOC in fine mode was found to be higher than the coarse mode.
MeSH term(s)	Aerosols/analysis ; Air Pollutants/analysis ; Environmental Monitoring ; India ; Particulate Matter/analysis ; Seasons
Chemical Substances	Aerosols ; Air Pollutants ; Particulate Matter
Language	English
Publishing date	2021-01-28
Publishing country	Netherlands
Document type	Journal Article ; Research Support, Non-U.S. Gov't
ZDB-ID	205699-9
ISSN	1096-0953 ; 0013-9351
ISSN (online)	1096-0953
ISSN	0013-9351
DOI	10.1016/j.envres.2021.110802
Database	MEDical Literature Analysis and Retrieval System OnLINE

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Article ; Online: A KBr-impregnated paper substrate as a sample probe for the enhanced ATR-FTIR signal strength of anionic and non-ionic surfactants in an aqueous medium.

Kurrey, Ramsingh / Deb, Manas Kanti / Shrivas, Kamlesh / Nirmalkar, Jayant / Sen, Bhupendra Kumar / Mahilang, Mithlesh / Jain, Vikas Kumar

RSC advances

2020 Volume 10, Issue 66, Page(s) 40428–40441

Abstract: Herein, we report a KBr-impregnated paper substrate as a sample probe to enhance the attenuated total reflection-Fourier transform infrared (ATR-FTIR) signal strength of anionic surfactants (AS) and non-ionic surfactants (NS) in an aqueous solution. The ... ...

Abstract	Herein, we report a KBr-impregnated paper substrate as a sample probe to enhance the attenuated total reflection-Fourier transform infrared (ATR-FTIR) signal strength of anionic surfactants (AS) and non-ionic surfactants (NS) in an aqueous solution. The mechanism for the sensing of AS and NS is based on the strong interaction of surfactants with the silicate groups (SiO
Language	English
Publishing date	2020-11-07
Publishing country	England
Document type	Journal Article
ISSN	2046-2069
ISSN (online)	2046-2069
DOI	10.1039/d0ra07286a
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Article: Analytical approach on surface active agents in the environment and challenges

Kurrey, Ramsingh / Mahilang, Mithlesh / Deb, Manas Kanti / Shrivas, Kamlesh

Trends in environmental analytical chemistry. 2019 Jan., v. 21

2019

Abstract: Surface active agents (SAAs) are a class of compounds, which is used in variety of products such as detergents, fabric softeners, soaps, paints, adhesives, inks and anti-fogs. After the use of these products containing surfactants are disposed in water ... ...

Abstract	Surface active agents (SAAs) are a class of compounds, which is used in variety of products such as detergents, fabric softeners, soaps, paints, adhesives, inks and anti-fogs. After the use of these products containing surfactants are disposed in water reservoirs. The separation and determination of surfactants from complex matrices become challenging for analytical chemists. The fundamentals on separation, preconcentration and analysis of surfactants employing different analytical instrumental techniques for qualitative and quantitative determination of surfactants in environmental samples are discussed. In addition, this compiled work enhanced our knowledge in learning about pathway mechanisms and the degree of their environmental loads. We also discussed the different aspects of method validation in the framework of quality control (QC) and quality assurance (QA). This review provides information on levels of SAAs in various environmental samples including soil, sediments, sewage wastewater, river wastewater and aerosols worldwide.
Keywords	adhesives ; aerosols ; analytical methods ; detergents ; fabrics ; paints ; quality control ; quantitative analysis ; rivers ; sediments ; sewage ; soaps ; soil ; surfactants ; wastewater ; water reservoirs
Language	English
Dates of publication	2019-01
Publishing place	Elsevier B.V.
Document type	Article
ISSN	2214-1588
DOI	10.1016/j.teac.2019.e00061
Database	NAL-Catalogue (AGRICOLA)

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Article ; Online: A direct DRS-FTIR probe for rapid detection and quantification of fluoroquinolone antibiotics in poultry egg-yolk.

Kurrey, Ramsingh / Mahilang, Mithlesh / Kanti Deb, Manas / Nirmalkar, Jayant / Shrivas, Kamlesh / Pervez, Shamsh / Kumar Rai, Manish / Rai, Joyce

Food chemistry

2018 Volume 270, Page(s) 459–466

Abstract: We report a novel diffuse reflectance-Fourier transforms infrared (DRS-FTIR) spectral monitoring of fluoroquinolone antibiotics such as ciprofloxacin (CIP) and norfloxacin (NOR) for their quantification in poultry egg-yolks. To the best of our knowledge, ...

Abstract	We report a novel diffuse reflectance-Fourier transforms infrared (DRS-FTIR) spectral monitoring of fluoroquinolone antibiotics such as ciprofloxacin (CIP) and norfloxacin (NOR) for their quantification in poultry egg-yolks. To the best of our knowledge, this is the first report to describe the rapid quantitative determination of fluoroquinolone antibiotics in poultry egg samples using DRS-FTIR. The characteristic absorption peaks obtained at 1627 and 1026 cm
MeSH term(s)	Animals ; Anti-Bacterial Agents/analysis ; Anti-Bacterial Agents/biosynthesis ; Egg Yolk/classification ; Fluoroquinolones/analysis ; Food Analysis ; Food Contamination/analysis ; Poultry ; Spectroscopy, Fourier Transform Infrared/methods
Chemical Substances	Anti-Bacterial Agents ; Fluoroquinolones
Language	English
Publishing date	2018-07-19
Publishing country	England
Document type	Journal Article
ZDB-ID	243123-3
ISSN	1873-7072 ; 0308-8146
ISSN (online)	1873-7072
ISSN	0308-8146
DOI	10.1016/j.foodchem.2018.07.129
Database	MEDical Literature Analysis and Retrieval System OnLINE

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Article: A direct DRS-FTIR probe for rapid detection and quantification of fluoroquinolone antibiotics in poultry egg-yolk

Kurrey, Ramsingh / Mahilang, Mithlesh / Kanti Deb, Manas / Nirmalkar, Jayant / Shrivas, Kamlesh / Pervez, Shamsh / Kumar Rai, Manish / Rai, Joyce

Food chemistry. 2019 Jan. 01, v. 270

2019

Abstract	We report a novel diffuse reflectance-Fourier transforms infrared (DRS-FTIR) spectral monitoring of fluoroquinolone antibiotics such as ciprofloxacin (CIP) and norfloxacin (NOR) for their quantification in poultry egg-yolks. To the best of our knowledge, this is the first report to describe the rapid quantitative determination of fluoroquinolone antibiotics in poultry egg samples using DRS-FTIR. The characteristic absorption peaks obtained at 1627 and 1026 cm−1 were used for optimization and determination of CIP and NOR, respectively. The linearity range obtained for the determination of CIP and NOR in egg samples was 0.05–0.50 ng mL−1 with limit of detection and limit of quantification of 0.032 and 1.551 ng mL−1 and 0.028 and 0.194 ng mL−1, respectively. Good recoveries were obtained in the range of 83.1–102.3% from poultry eggs samples using DRS-FTIR method. The advantages of the DRS-FTIR method are its simplicity, sensitivity and suitability for high-throughput analysis towards the food samples.
Keywords	absorption ; antibiotics ; ciprofloxacin ; detection limit ; egg yolk ; eggs ; monitoring ; norfloxacin ; poultry ; quantitative analysis ; rapid methods
Language	English
Dates of publication	2019-0101
Size	p. 459-466.
Publishing place	Elsevier Ltd
Document type	Article
ZDB-ID	243123-3
ISSN	1873-7072 ; 0308-8146
ISSN (online)	1873-7072
ISSN	0308-8146
DOI	10.1016/j.foodchem.2018.07.129
Database	NAL-Catalogue (AGRICOLA)

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