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Article ; Online: Novel design of high elastic solid polymer electrolyte for stable lithium metal batteries.

Li, Qiuhong / Liao, Yalan / Xing, Cong / Shi, Yaru / Liu, Xiaoyu / Li, Wenrong / Zhang, Jiujun / Zhao, Bing / Jiang, Yong

Journal of colloid and interface science

2024 Volume 659, Page(s) 533–541

Abstract: Li metal anodes have high specific capacity and low electrode potential, and have always been considered as one of the most promising anode materials. However, the growth of Li dendrites, unstable solid electrolyte interface layer (SEI), severe side ... ...

Abstract	Li metal anodes have high specific capacity and low electrode potential, and have always been considered as one of the most promising anode materials. However, the growth of Li dendrites, unstable solid electrolyte interface layer (SEI), severe side reactions at the Li/electrolyte interface, and infinite volume expansion of the Li anode seriously hinder the practical application of solid-state Li metal batteries (LMBs). Herein, we report a polyurethane elastomer (TPU) material with high elasticity and interfacial stability as a solid polymer electrolyte (SPE) for LMBs. The synergistic effects of its designed soft chain forging (PEO) and hard chain segments (IPDI) can enhance Li ion conductivity, elastic modulus and flexibility of the SPE to settle the challenges of the Li metal anodes. Moreover, Li
Language	English
Publishing date	2024-01-04
Publishing country	United States
Document type	Journal Article
ZDB-ID	241597-5
ISSN	1095-7103 ; 0021-9797
ISSN (online)	1095-7103
ISSN	0021-9797
DOI	10.1016/j.jcis.2023.12.187
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Article ; Online: A Tb

Wang, Bin / Zheng, Wei / Chen, Jiashang / Wang, Yaru / Duan, Xing / Ma, Shiyu / Kong, Zhe / Xia, Tifeng

Spectrochimica acta. Part A, Molecular and biomolecular spectroscopy

2023 Volume 304, Page(s) 123388

Abstract: We successfully synthesized a stable anionic microporous metal-organic framework (MOF) HDU-1 ([ ... ...

Abstract	We successfully synthesized a stable anionic microporous metal-organic framework (MOF) HDU-1 ([Me
Language	English
Publishing date	2023-09-09
Publishing country	England
Document type	Journal Article
ZDB-ID	210413-1
ISSN	1873-3557 ; 0370-8322 ; 0584-8539 ; 1386-1425
ISSN (online)	1873-3557
ISSN	0370-8322 ; 0584-8539 ; 1386-1425
DOI	10.1016/j.saa.2023.123388
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Article ; Online: Co-pyrolysis of alkali-fused fly ash and corn stover to synthesize biochar composites for remediating lead-contaminated soil.

Ma, Yan / Shang, Xiufang / Zhang, Yaru / Chen, Wei / Gao, Yan / Guo, Jianda / Zheng, Hao / Xing, Baoshan

Environmental research

2024 Volume 252, Issue Pt 2, Page(s) 118938

Abstract: Fly ash (FA) is mainly composed of silica, alumina, and other metal oxide components, and has a positive stabilizing effect on soil heavy metals. Biochar composites produced from FA and corn stover (CS) can improve its remediation performance. Therefore, ...

Abstract	Fly ash (FA) is mainly composed of silica, alumina, and other metal oxide components, and has a positive stabilizing effect on soil heavy metals. Biochar composites produced from FA and corn stover (CS) can improve its remediation performance. Therefore, a batch of biochar composites (alkali-fused FA-CS biochars, ABs), synthesized via co-pyrolysis of CS and alkali-fused FA (AFFA) at different temperatures of 300, 500, and 700 °C (AB300-1, AB500-1, and AB700-1) and CS to AFFA mass ratios of 10:1, 10:2, and 10:5 (AB500-1, AB500-2, and AB500-5), was used to remediate lead (Pb)-contaminated soil. Compared with pristine biochars (BCs), ABs were enriched with oxygen-containing functional groups (Si-O-Si and Si-O) and aromatic structures. The ABs prepared at lower pyrolytic temperature (≤500 °C) and lower ratio of CS to AFFA (10:1) showed higher yield and stability. The contents of Toxicity Characteristic Leaching Procedure (TCLP)-extractable Pb and DTPA-CaCl
Language	English
Publishing date	2024-04-20
Publishing country	Netherlands
Document type	Journal Article
ZDB-ID	205699-9
ISSN	1096-0953 ; 0013-9351
ISSN (online)	1096-0953
ISSN	0013-9351
DOI	10.1016/j.envres.2024.118938
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Article ; Online: Effect of root exudates on the release, surface property, colloidal stability, and phytotoxicity of dissolved black carbon.

Gu, Shiguo / Lian, Fei / Han, Yaru / Wang, Zhenyu / Xing, Baoshan

Ecotoxicology and environmental safety

2022 Volume 239, Page(s) 113687

Abstract: In this study, the release of dissolved black carbon (DBC) from bulk-BC, its surface properties, colloidal stability, and oxidative stress to rice seedlings in the presence and absence of rice root exudates were compared. The bulk-BCs were prepared at ... ...

Abstract	In this study, the release of dissolved black carbon (DBC) from bulk-BC, its surface properties, colloidal stability, and oxidative stress to rice seedlings in the presence and absence of rice root exudates were compared. The bulk-BCs were prepared at 550 °C and derived from wood chips and pig manure, respectively. The release of DBC from bulk-BC was significantly enhanced (20.19-23.63%) by the introduction of root exudates, where low molecular weight organic acids played a dominating role in the dissociation of DBC from carbon skeleton. The surface properties of DBC were greatly modified by root exudates including decreases in the surface area (18.13%) and mineral contents (43.90-69.57%). The O-containing groups and graphitization were also enhanced by 11.46% and 18.65%, respectively. Meanwhile, the presence of root exudates not only reduced the colloidal stability of DBC but also lowered the intensity of free radicals (19.44-22.22%) in DBC. Consequently, the oxidative stress of DBC to rice seedlings was significantly (p < 0.05) alleviated, evidenced by reduced antioxidative enzyme activities (5.67-29.25%) and soluble protein content (15.75-46.79%) in rice plants. These results indicate that the interaction between DBC and root exudates could remarkably modify the surface properties and reactivity of DBC, which has profound implications for understanding the behavior and functions of DBC in the environment.
MeSH term(s)	Animals ; Carbon/metabolism ; Exudates and Transudates ; Oryza/metabolism ; Seedlings ; Soot/toxicity ; Surface Properties ; Swine
Chemical Substances	Soot ; Carbon (7440-44-0)
Language	English
Publishing date	2022-05-25
Publishing country	Netherlands
Document type	Journal Article
ZDB-ID	436536-7
ISSN	1090-2414 ; 0147-6513
ISSN (online)	1090-2414
ISSN	0147-6513
DOI	10.1016/j.ecoenv.2022.113687
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Article ; Online: Novel Insights into the Impact of Nano-Biochar on Composition and Structural Transformation of Mineral/Nano-Biochar Heteroaggregates in the Presence of Root Exudates.

Lian, Fei / Gu, Shiguo / Han, Yaru / Wang, Zhenyu / Xing, Baoshan

Environmental science & technology

2022 Volume 56, Issue 13, Page(s) 9816–9825

Abstract: Multiple lines of existing evidence indicate that natural organic matter (NOM) could protect poorly crystalline Fe(III) (oxyhydr)oxides from Fe(II)-catalyzed mineral transformation. Conversely, we find that nano-sized biochar (nano-BC), a pyrogenic form ... ...

Abstract	Multiple lines of existing evidence indicate that natural organic matter (NOM) could protect poorly crystalline Fe(III) (oxyhydr)oxides from Fe(II)-catalyzed mineral transformation. Conversely, we find that nano-sized biochar (nano-BC), a pyrogenic form of NOM, promotes the phase transformation of ferrihydrite (Fh) in nano-BC/Fh heteroaggregates in the presence of aqueous Fe(II) and rice root exudates. The nano-BC/Fh heteroaggregates are composed of a core-shell like structure where the inner-layered nano-BC is more compacted and plays the dominant role in accelerating the phase transformation of Fh relative to that in the outer sphere. The extent of phase transformation is more regulated by the reversible redox reactions between quinone and hydroquinone in nano-BC than the electron transfer via its condensed aromatic structures. Furthermore, the reductive organic acids in root exudates contribute to the mineral transformation of nano-BC/Fh associations by donating electrons to Fe(III) through nano-BC. Our results suggest that heteroaggregates between nano-BC and Fe minerals are subjected to partial dissociation during their co-transport, and the stably attached nano-BC is favorable to the phase transformation of poorly crystalline Fe minerals (e.g., Fh), which might have profound implications on biogeochemical cycles of carbon and Fe in the prevailing redox environments.
MeSH term(s)	Exudates and Transudates ; Ferric Compounds/chemistry ; Ferrous Compounds ; Minerals/chemistry ; Oxidation-Reduction
Chemical Substances	Ferric Compounds ; Ferrous Compounds ; Minerals
Language	English
Publishing date	2022-06-20
Publishing country	United States
Document type	Journal Article ; Research Support, Non-U.S. Gov't
ISSN	1520-5851
ISSN (online)	1520-5851
DOI	10.1021/acs.est.2c02127
Database	MEDical Literature Analysis and Retrieval System OnLINE

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Article ; Online: Effect of root exudates on the release, surface property, colloidal stability, and phytotoxicity of dissolved black carbon

Shiguo Gu / Fei Lian / Yaru Han / Zhenyu Wang / Baoshan Xing

Ecotoxicology and Environmental Safety, Vol 239, Iss , Pp 113687- (2022)

2022

Abstract	In this study, the release of dissolved black carbon (DBC) from bulk-BC, its surface properties, colloidal stability, and oxidative stress to rice seedlings in the presence and absence of rice root exudates were compared. The bulk-BCs were prepared at 550 °C and derived from wood chips and pig manure, respectively. The release of DBC from bulk-BC was significantly enhanced (20.19–23.63%) by the introduction of root exudates, where low molecular weight organic acids played a dominating role in the dissociation of DBC from carbon skeleton. The surface properties of DBC were greatly modified by root exudates including decreases in the surface area (18.13%) and mineral contents (43.90–69.57%). The O-containing groups and graphitization were also enhanced by 11.46% and 18.65%, respectively. Meanwhile, the presence of root exudates not only reduced the colloidal stability of DBC but also lowered the intensity of free radicals (19.44–22.22%) in DBC. Consequently, the oxidative stress of DBC to rice seedlings was significantly (p < 0.05) alleviated, evidenced by reduced antioxidative enzyme activities (5.67–29.25%) and soluble protein content (15.75–46.79%) in rice plants. These results indicate that the interaction between DBC and root exudates could remarkably modify the surface properties and reactivity of DBC, which has profound implications for understanding the behavior and functions of DBC in the environment.
Keywords	Dissolved black carbon ; Root exudates ; Physicochemical property ; Colloidal stability ; Free radicals ; Phytotoxicity ; Environmental pollution ; TD172-193.5 ; Environmental sciences ; GE1-350
Subject code	580
Language	English
Publishing date	2022-07-01T00:00:00Z
Publisher	Elsevier
Document type	Article ; Online
Database	BASE - Bielefeld Academic Search Engine (life sciences selection)

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Article ; Online: Theoretical insights into the mechanism underlying aflatoxin B

Wang, Xiaolu / Cui, Lin / Liu, Mengting / Qi, Zheng / Luo, Huiying / Huang, Huoqing / Tu, Tao / Qin, Xing / Wang, Yuan / Zhang, Jie / Wang, Yaru / Yao, Bin / Bai, Yingguo / Su, Xiaoyun

Ecotoxicology and environmental safety

2024 Volume 272, Page(s) 116049

Abstract: Global concern exists regarding the contamination of food and animal feed with aflatoxin ... ...

Abstract	Global concern exists regarding the contamination of food and animal feed with aflatoxin B
MeSH term(s)	Humans ; Aflatoxin B1/toxicity ; Aflatoxin B1/chemistry ; Laccase ; Chromatography, Liquid ; Tandem Mass Spectrometry ; Gallic Acid/analogs & derivatives
Chemical Substances	Aflatoxin B1 (9N2N2Y55MH) ; Laccase (EC 1.10.3.2) ; methyl syringate ; Gallic Acid (632XD903SP)
Language	English
Publishing date	2024-02-01
Publishing country	Netherlands
Document type	Journal Article
ZDB-ID	436536-7
ISSN	1090-2414 ; 0147-6513
ISSN (online)	1090-2414
ISSN	0147-6513
DOI	10.1016/j.ecoenv.2024.116049
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Article ; Online: Lipid Nanoparticles Optimized for Targeting and Release of Nucleic Acid.

Jia, Yaru / Wang, Xiuguang / Li, Luwei / Li, Fangzhou / Zhang, Jinchao / Liang, Xing-Jie

Advanced materials (Deerfield Beach, Fla.)

2023 Volume 36, Issue 4, Page(s) e2305300

Abstract: Lipid nanoparticles (LNPs) are currently the most promising clinical nucleic acids drug delivery vehicles. LNPs prevent the degradation of cargo nucleic acids during blood circulation. Upon entry into the cell, specific components of the lipid ... ...

Abstract	Lipid nanoparticles (LNPs) are currently the most promising clinical nucleic acids drug delivery vehicles. LNPs prevent the degradation of cargo nucleic acids during blood circulation. Upon entry into the cell, specific components of the lipid nanoparticles can promote the endosomal escape of nucleic acids. These are the basic properties of lipid nanoparticles as nucleic acid carriers. As LNPs exhibit hepatic aggregation characteristics, enhancing targeting out of the liver is a crucial way to improve LNPs administrated in vivo. Meanwhile, endosomal escape of nucleic acids loaded in LNPs is often considered inadequate, and therefore, much effort is devoted to enhancing the intracellular release efficiency of nucleic acids. Here, different strategies to efficiently deliver nucleic acid delivery from LNPs are concluded and their mechanisms are investigated. In addition, based on the information on LNPs that are in clinical trials or have completed clinical trials, the issues that are necessary to be approached in the clinical translation of LNPs are discussed, which it is hoped will shed light on the development of LNP nucleic acid drugs.
MeSH term(s)	Nucleic Acids ; Lipids ; Nanoparticles ; Liposomes ; RNA, Small Interfering
Chemical Substances	Lipid Nanoparticles ; Nucleic Acids ; Lipids ; Liposomes ; RNA, Small Interfering
Language	English
Publishing date	2023-11-30
Publishing country	Germany
Document type	Journal Article ; Review
ZDB-ID	1474949-X
ISSN	1521-4095 ; 0935-9648
ISSN (online)	1521-4095
ISSN	0935-9648
DOI	10.1002/adma.202305300
Database	MEDical Literature Analysis and Retrieval System OnLINE

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Article ; Online: Exposure Order to Photoaging and Humic Acids Significantly Modifies the Aggregation and Transformation of Nanoplastics in Aqueous Solutions.

Lian, Fei / Han, Yaru / Zhang, Yikang / Li, Jiaqi / Sun, BinBin / Geng, Zexuan / Wang, Zhenyu / Xing, Baoshan

Environmental science & technology

2023 Volume 57, Issue 16, Page(s) 6520–6529

Abstract: The colloidal stability of nanoplastics in aqueous solutions is greatly regulated by photoaging and dissolved organic matter (DOM). However, how the exposure order to sunlight and DOM modifies the environmental behavior of nanoplastics is seldomly ... ...

Abstract	The colloidal stability of nanoplastics in aqueous solutions is greatly regulated by photoaging and dissolved organic matter (DOM). However, how the exposure order to sunlight and DOM modifies the environmental behavior of nanoplastics is seldomly determined. Here, with two different exposure orders, we investigated the impact of molecular-weight (MW)-fractionated humic acids (HAs) derived from biochar and the Suwannee River, respectively, on the aggregation of poly(ethylene terephthalate) nanoplastics (PET-NPs) in mono- and divalent electrolyte solutions. For exposure pattern (i) (photoaging followed by HA coating), photoaged PET-NPs had more oxidized surfaces and exhibited 22-320% higher binding affinity to HAs (especially the higher MW fractions) than the pristine counterparts, which greatly improved the dispersion of PET-NPs. For exposure pattern (ii) (HA coating followed by photoaging), HA-PET assemblies were formed, the dispersion of which increased with increasing irradiation time and was significantly higher than that of the samples in the exposure pattern (i) at the end of the experiment. This high dispersion of photoaged HA-PET assemblies was ascribed to the extra oxidation of PET by reactive oxygen species generated in the PET-HA interfaces during photoaging. These findings highlight the "active nature" of HA-PET assemblies, which provide new insight into the reaction of HA with nanoplastics beyond adsorption in the natural environment.
MeSH term(s)	Humic Substances/analysis ; Microplastics ; Skin Aging ; Rivers ; Dissolved Organic Matter
Chemical Substances	Humic Substances ; Microplastics ; Dissolved Organic Matter
Language	English
Publishing date	2023-04-12
Publishing country	United States
Document type	Journal Article ; Research Support, Non-U.S. Gov't
ISSN	1520-5851
ISSN (online)	1520-5851
DOI	10.1021/acs.est.2c09140
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Article ; Online: Construction of high elastic artificial SEI for air-stable and long-life lithium metal anode.

Zhao, Bing / Xing, Cong / Shi, Yaru / Duan, Qiming / Shen, Chao / Li, Wenrong / Jiang, Yong / Zhang, Jiujun

Journal of colloid and interface science

2023 Volume 642, Page(s) 193–203

Abstract: Compared with other anode materials, Li metal anode has higher capacity density and lower electrode potential, which has been considered as one of the most promising anode materials. However, the unstable solid electrolyte interface (SEI) leads to Li ... ...

Abstract	Compared with other anode materials, Li metal anode has higher capacity density and lower electrode potential, which has been considered as one of the most promising anode materials. However, the unstable solid electrolyte interface (SEI) leads to Li dendrite growth and the infinite volumetric expansion of Li metal, which seriously hinders the stability and cycle life of Li metal batteries (LMBs). Here, a polyurethane elastomer (TPU) material with high elasticity and air stability is used as the artificial SEI of Li metal anode. Its designed synergistic effect of soft chain forging and hard chain segments not only gives TPU artificial SEI layer good electronic insulation, Li ion conductivity, Li dendrite growth inhibition, high elastic modulus and flexibility to adapt to Li volume expansion, but also has a significant air protection effect on the Li metal surface, so that the TPU coated Li foil will not occur obvious oxidation phenomenon after being placed in air for 45 min. The Li symmetric battery modified by TPU achieved a stable and long-term cycle performance of 1300 h at 1 mA/cm
Language	English
Publishing date	2023-03-30
Publishing country	United States
Document type	Journal Article
ZDB-ID	241597-5
ISSN	1095-7103 ; 0021-9797
ISSN (online)	1095-7103
ISSN	0021-9797
DOI	10.1016/j.jcis.2023.03.168
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