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Article ; Online: Synergistic catalytic conversion and chemisorption of polysulfides from Fe/Fe3C/FeN0.0324 nanocubes modified separator for advanced Li-S batteries

Wan, Pengfei / Dong, Siyang / Xiong, Jing / Jin, Xuanyang / Lu, Shengjun / Zhang, Yufei / Fan, Haosen

Journal of Colloid And Interface Science. 2023 Nov., v. 650 p.582-592

2023

Abstract: Lithium sulfur batteries (LSBs) have been considered as one of the most promising options for next generation high-performance batteries. However, the heavy shuttle effect and inferior redox conversion during the charge/discharge processes of the ... ...

Abstract	Lithium sulfur batteries (LSBs) have been considered as one of the most promising options for next generation high-performance batteries. However, the heavy shuttle effect and inferior redox conversion during the charge/discharge processes of the batteries have greatly hindered their further applications. In this study, to address these disadvantages of LSBs, Fe/Fe₃C/FeN₀.₀₃₂₄ heterostructured nanocubes were designed and prepared through high temperature carbonization process using Prussian blue precursor. Then the Fe/Fe₃C/FeN₀.₀₃₂₄ nanocubes were used to modify the commercial polypropylene (PP) separator, which can greatly catalyze the redox transformation of polysulfides and provide sufficient active sites for chemisorption. As result, the modified separator endowed LSBs with excellent rate capacity and cycle stability, delivering a high-capacity of 1025 mAh/g at 0.5 C with nearly 100% coulombic efficiency. It also displayed a superb cycling performance with a per-cycle capacity attenuation rate of 0.09% after 300 cycles. When the current density increased to 1 C with the S loading of 1.73 mg cm⁻², Fe/Fe₃C/FeN₀.₀₃₂₄-PP separator presented a satisfactory capacity decay rate of 0.05% per cycle after 1000 cycles. Besides, it also presented outstanding electrochemical performance even at high sulfur loading of 4.5 mg cm⁻². This work has provided a new avenue for the design of nanomaterials with synergistic effect of catalytic conversion and chemisorption of polysulfides for the promotion of high-performance Li-S batteries.
Keywords	carbonization ; electrochemistry ; lithium ; nanomaterials ; polypropylenes ; redox reactions ; sulfur ; synergism ; temperature ; Lithium sulfur batteries ; Fe/Fe3C/FeN0.0324 nanocubes ; Separator ; Polysulfide adsorption ; Catalytic conversion
Language	English
Dates of publication	2023-11
Size	p. 582-592.
Publishing place	Elsevier Inc.
Document type	Article ; Online
ZDB-ID	241597-5
ISSN	1095-7103 ; 0021-9797
ISSN (online)	1095-7103
ISSN	0021-9797
DOI	10.1016/j.jcis.2023.07.022
Database	NAL-Catalogue (AGRICOLA)

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Article ; Online: Synergistic enhancement of chemisorption and catalytic conversion in lithium-sulfur batteries via Co

Wan, Pengfei / Peng, Xiaoli / Dong, Siyang / Liu, Xinyun / Lu, Shengjun / Zhang, Yufei / Fan, Haosen

Journal of colloid and interface science

2023 Volume 657, Page(s) 757–766

Abstract: Lithium-sulfur batteries (LSBs) show considerable potential in next-generation high performance batteries, but the heavy shuttle effect and sluggish redox kinetics of polysulfide hinder their further applications. In this paper, to address these ... ...

Abstract	Lithium-sulfur batteries (LSBs) show considerable potential in next-generation high performance batteries, but the heavy shuttle effect and sluggish redox kinetics of polysulfide hinder their further applications. In this paper, to address these shortcomings of LSBs, Co
Language	English
Publishing date	2023-12-05
Publishing country	United States
Document type	Journal Article
ZDB-ID	241597-5
ISSN	1095-7103 ; 0021-9797
ISSN (online)	1095-7103
ISSN	0021-9797
DOI	10.1016/j.jcis.2023.12.013
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Article ; Online: Construction of 2D sandwich-like Na

Sun, Rui / Dong, Siyang / Guo, Xincheng / Xia, Peng / Lu, Shengjun / Zhang, Yufei / Fan, Haosen

Journal of colloid and interface science

2023 Volume 655, Page(s) 226–233

Abstract: Aqueous zinc ion batteries (AZIBs) have attained enormous attention in the last few years. The cathode materials of aqueous zinc ion batteries play a vital effect in their electrochemical and battery properties. In this manuscript, Sandwich-like MXene@ ... ...

Abstract	Aqueous zinc ion batteries (AZIBs) have attained enormous attention in the last few years. The cathode materials of aqueous zinc ion batteries play a vital effect in their electrochemical and battery properties. In this manuscript, Sandwich-like MXene@Na
Language	English
Publishing date	2023-11-04
Publishing country	United States
Document type	Journal Article
ZDB-ID	241597-5
ISSN	1095-7103 ; 0021-9797
ISSN (online)	1095-7103
ISSN	0021-9797
DOI	10.1016/j.jcis.2023.11.020
Database	MEDical Literature Analysis and Retrieval System OnLINE

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Article ; Online: Synergistic catalytic conversion and chemisorption of polysulfides from Fe/Fe

Wan, Pengfei / Dong, Siyang / Xiong, Jing / Jin, Xuanyang / Lu, Shengjun / Zhang, Yufei / Fan, Haosen

Journal of colloid and interface science

2023 Volume 650, Issue Pt A, Page(s) 582–592

Abstract	Lithium sulfur batteries (LSBs) have been considered as one of the most promising options for next generation high-performance batteries. However, the heavy shuttle effect and inferior redox conversion during the charge/discharge processes of the batteries have greatly hindered their further applications. In this study, to address these disadvantages of LSBs, Fe/Fe
Language	English
Publishing date	2023-07-06
Publishing country	United States
Document type	Journal Article
ZDB-ID	241597-5
ISSN	1095-7103 ; 0021-9797
ISSN (online)	1095-7103
ISSN	0021-9797
DOI	10.1016/j.jcis.2023.07.022
Database	MEDical Literature Analysis and Retrieval System OnLINE

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Article ; Online: Co-intercalation strategy of constructing partial cation substitution of ammonium vanadate {(NH

Sun, Rui / Dong, Siyang / Xu, Feng / Li, Zhiyong / Wang, Caihong / Lu, Shengjun / Fan, Haosen

Dalton transactions (Cambridge, England : 2003)

2022 Volume 51, Issue 19, Page(s) 7607–7612

Abstract: Recently, aqueous zinc-ion batteries have become a hot research topic in the field of grid-scale application, which can be attributed to their low-cost, aqueous electrolyte and dominant theoretical reversible capacity. Nevertheless, the lack of suitable ... ...

Abstract	Recently, aqueous zinc-ion batteries have become a hot research topic in the field of grid-scale application, which can be attributed to their low-cost, aqueous electrolyte and dominant theoretical reversible capacity. Nevertheless, the lack of suitable cathode materials greatly hinders the development of aqueous zinc-ion batteries. In this work, we adopt a simple one-step synthesis strategy to prepare (NH
Language	English
Publishing date	2022-05-17
Publishing country	England
Document type	Journal Article
ZDB-ID	1472887-4
ISSN	1477-9234 ; 1364-5447 ; 0300-9246 ; 1477-9226
ISSN (online)	1477-9234 ; 1364-5447
ISSN	0300-9246 ; 1477-9226
DOI	10.1039/d2dt00665k
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Article ; Online: Defect engineering of molybdenum disulfide nanosheets boosting super Zn

Sun, Rui / Dong, Siyang / Yang, Jiekai / Xiong, Jing / Wang, Caihong / Lu, Shengjun / Zhang, Yufei / Fan, Haosen

Chemical communications (Cambridge, England)

2023 Volume 59, Issue 13, Page(s) 1845–1848

Abstract: In this work, peony-like structured ... ...

Abstract	In this work, peony-like structured MoS
Language	English
Publishing date	2023-02-09
Publishing country	England
Document type	Journal Article
ZDB-ID	1472881-3
ISSN	1364-548X ; 1359-7345 ; 0009-241X
ISSN (online)	1364-548X
ISSN	1359-7345 ; 0009-241X
DOI	10.1039/d2cc05888j
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Article ; Online: MOF derived cobalt-nickel bimetallic phosphide (CoNiP) modified separator to enhance the polysulfide adsorption-catalysis for superior lithium-sulfur batteries.

Zhu, Hangyi / Dong, Siyang / Xiong, Jing / Wan, Pengfei / Jin, Xuanyang / Lu, Shengjun / Zhang, Yufei / Fan, Haosen

Journal of colloid and interface science

2023 Volume 641, Page(s) 942–949

Abstract: Lithium-sulfur batteries (LSBs) have aroused great research interest due to their high theoretical capacity and high energy density. To further develop lithium-sulfur batteries, it has become more and more important to put more efforts in promoting the ... ...

Abstract	Lithium-sulfur batteries (LSBs) have aroused great research interest due to their high theoretical capacity and high energy density. To further develop lithium-sulfur batteries, it has become more and more important to put more efforts in promoting the adsorption and rapid catalytic conversion of lithium polysulfides (LiPSs). Herein, Ni/Co bimetallic phosphides were encapsulated into nitrogen-doped dual carbon conductive network (NiCoP@NC) by annealing and phosphorizing Ni-ZIF-67 precursor at high temperature. Due to their numerous co-adsorption/catalytic sites and high conductivity of carbon skeleton, the encapsulated Ni/Co phosphides particles could significantly enhance the anchoring and catalytic conversion of LiPSs and provide ultrafast channels for Li
Language	English
Publishing date	2023-03-16
Publishing country	United States
Document type	Journal Article
ZDB-ID	241597-5
ISSN	1095-7103 ; 0021-9797
ISSN (online)	1095-7103
ISSN	0021-9797
DOI	10.1016/j.jcis.2023.03.083
Database	MEDical Literature Analysis and Retrieval System OnLINE

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Article: Roles of the fibroblast growth factor signal transduction system in tissue injury repair.

Chen, Keyang / Rao, Zhiheng / Dong, Siyang / Chen, Yajing / Wang, Xulan / Luo, Yongde / Gong, Fanghua / Li, Xiaokun

Burns & trauma

2022 Volume 10, Page(s) tkac005

Abstract: Following injury, tissue autonomously initiates a complex repair process, resulting in either partial recovery or regeneration of tissue architecture and function in most organisms. Both the repair and regeneration processes are highly coordinated by a ... ...

Abstract	Following injury, tissue autonomously initiates a complex repair process, resulting in either partial recovery or regeneration of tissue architecture and function in most organisms. Both the repair and regeneration processes are highly coordinated by a hierarchy of interplay among signal transduction pathways initiated by different growth factors, cytokines and other signaling molecules under normal conditions. However, under chronic traumatic or pathological conditions, the reparative or regenerative process of most tissues in different organs can lose control to different extents, leading to random, incomplete or even flawed cell and tissue reconstitution and thus often partial restoration of the original structure and function, accompanied by the development of fibrosis, scarring or even pathogenesis that could cause organ failure and death of the organism. Ample evidence suggests that the various combinatorial fibroblast growth factor (FGF) and receptor signal transduction systems play prominent roles in injury repair and the remodeling of adult tissues in addition to embryonic development and regulation of metabolic homeostasis. In this review, we attempt to provide a brief update on our current understanding of the roles, the underlying mechanisms and clinical application of FGFs in tissue injury repair.
Language	English
Publishing date	2022-03-23
Publishing country	England
Document type	Journal Article ; Review
ZDB-ID	2775996-9
ISSN	2321-3876 ; 2321-3868
ISSN (online)	2321-3876
ISSN	2321-3868
DOI	10.1093/burnst/tkac005
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Article: Lake dynamics and its relationship to climate change on the Tibetan Plateau over the last four decades

Dong, Siyang / Fei Peng / Quangang You / Jian Guo / Xian Xue

Regional environmental change. 2018 Feb., v. 18, no. 2

2018

Abstract: The high sensitivity of the Tibetan Plateau (TP) to global warming is ascribed not only to its high altitude and low temperature but also to the change in the components of water cycling, such as glaciers’ retreat, permafrost degradation, and lakes’ ... ...

Abstract	The high sensitivity of the Tibetan Plateau (TP) to global warming is ascribed not only to its high altitude and low temperature but also to the change in the components of water cycling, such as glaciers’ retreat, permafrost degradation, and lakes’ shrinkage or expansion. Among the components, change in lakes attracts more attention as lakes are crucial for local water management and are easier to monitor. But, how water cycling components respond to global change remains unclear, although they are crucial in understanding the regional environmental change. Lakes, glaciers, and permafrost data derived from meteorological records and remote sensing images were used to detect the change of the water environment on the TP from 1971 to 2013. The climate on TP changed toward a warm-humid condition in the last four decades. Three-quarters of the lakes were significantly expanded over the TP, and the summed area of all the lakes increased by 6061 km² from 1975 to 2010. Panel regression showed that annual average air temperature (T), annual precipitation (P), and reference crop evapotranspiration (ET ₒ) regulate the change in lake surface area (LSA) on the entire TP. The change in LSA is more related to the change in P than in the other two factors, even in the catchment where lakes are recharged by water from glacier melting and permafrost degradation, especially in extremely arid and arid climate zones. Elevation and size affected the sensitivity of lakes to climate change with lakes in a high-elevation area more sensitive to T and small lakes more sensitive to T, P, and ET ₒ . Warming-induced glacier’s retreat led to the significant lake expansion, while permafrost degradation might be responsible for the lake shrinkage in the seasonally frozen ground area due to the related cryogenic waterproof layer downward. Our results about the responses of lakes to climate change in different catchments were in accordance with the findings of previous studies about several typical lakes, which implied that overall response of all the lakes to climate change could be obtained by examining several typical lakes in the catchment level.
Keywords	air temperature ; altitude ; arid zones ; atmospheric precipitation ; evapotranspiration ; glaciers ; global warming ; lakes ; melting ; meteorological data ; permafrost ; remote sensing ; shrinkage ; surface area ; water management ; watersheds ; China
Language	English
Dates of publication	2018-02
Size	p. 477-487.
Publishing place	Springer Berlin Heidelberg
Document type	Article
ZDB-ID	1464515-4
ISSN	1436-3798
ISSN	1436-3798
DOI	10.1007/s10113-017-1211-8
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Article ; Online: FGF4 Promotes Skin Wound Repair through p38 MAPK and GSK3β-Mediated Stabilization of Slug.

Sun, Jian / Zhou, Jie / Zhou, Jianhui / Xu, Wenxin / Du, Yali / Jia, Zhenyu / Shen, Yingjie / Lin, Xiaohua / Wang, Xulan / Bao, Yuxuan / Rao, Zhiheng / Dong, Siyang / Luo, Yongde / Cong, Weitao / Jin, Litai / Li, Xiaokun

The Journal of investigative dermatology

2022 Volume 143, Issue 6, Page(s) 1073–1084.e8

Abstract: Cutaneous wound healing is an orderly and intricate process that restores the barrier function and integrity of injured skin. Re-epithelialization, which involves the proliferation and migration of keratinocytes to cover the denuded surface, is essential ...

Abstract	Cutaneous wound healing is an orderly and intricate process that restores the barrier function and integrity of injured skin. Re-epithelialization, which involves the proliferation and migration of keratinocytes to cover the denuded surface, is essential for successful wound closure. There are many members of the FGF family, of which the paracrine-acting FGF1 and FGF7 subfamily members have been identified as positive regulators of wound repair. However, the role and underlying mechanisms of some other paracrine FGFs in wound repair still remain obscure. In this report, we found that paracrine FGF4 localized predominantly to the epidermal keratinocytes and was markedly upregulated at the wound edges in response to re-epithelialization in human and mouse wound models. Blockade of FGF4 resulted in delayed re-epithelialization of human ex vivo skin wounds, whereas recombinant FGF4 treatment promoted re-epithelialization and wound repair. Mechanistically, recombinant FGF4 promotes p38 MAPK‒GSK3β‒mediated stabilization of Slug by reducing its ubiquitination, which triggers epithelial-to-mesenchymal transition and promotes the migration and proliferation of keratinocytes and thus wound re-epithelialization. Our findings uncover FGF4 as an important regulator of wound healing, highlighting a promising therapeutic avenue for skin injury.
MeSH term(s)	Mice ; Animals ; Humans ; Gastropoda ; Glycogen Synthase Kinase 3 beta ; Wound Healing/physiology ; Skin/injuries ; Keratinocytes/physiology ; Re-Epithelialization ; Disease Models, Animal ; Cell Movement ; Fibroblast Growth Factor 4
Chemical Substances	Glycogen Synthase Kinase 3 beta (EC 2.7.11.1) ; FGF4 protein, human ; Fibroblast Growth Factor 4
Language	English
Publishing date	2022-12-13
Publishing country	United States
Document type	Journal Article ; Research Support, Non-U.S. Gov't
ZDB-ID	80136-7
ISSN	1523-1747 ; 0022-202X
ISSN (online)	1523-1747
ISSN	0022-202X
DOI	10.1016/j.jid.2022.11.015
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