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  1. Article ; Online: A Secondary Al-CO₂ Battery Enabled by Aluminum Iodide as a Homogeneous Redox Mediator

    Fetrow, Christopher / Carugati, Cameron / Yu, Xingwen / Zhou, Xiao-Dong / Wei, Shuya

    ACS Applied Materials & Interfaces. 2023 Mar. 03, v. 15, no. 10 p.12908-12914

    2023  

    Abstract: As an emerging energy storage concept, Al-CO₂ batteries have not yet been demonstrated as a rechargeable system that can deliver a high discharge voltage and a high capacity. In this work, we present a homogeneous redox mediator to access a rechargeable ... ...

    Abstract As an emerging energy storage concept, Al-CO₂ batteries have not yet been demonstrated as a rechargeable system that can deliver a high discharge voltage and a high capacity. In this work, we present a homogeneous redox mediator to access a rechargeable Al-CO₂ battery with an ultralow overpotential of 0.05 V. In addition, the resulting rechargeable Al-CO₂ cell can maintain a high discharge voltage of 1.12 V and delivers a high capacity of 9394 mAh/gcₐᵣbₒₙ. Nuclear magnetic resonance (NMR) analysis indicates that the discharge product is aluminum oxalate which can facilitate the reversible operation of Al-CO₂ batteries. The rechargeable Al-CO₂ battery system demonstrated here holds great promise as a low-cost and high-energy alternative for future grid energy storage applications. Meanwhile, the Al-CO₂ battery system could facilitate capture and concentration of atmospheric CO₂, ultimately benefiting both the energy and environmental sectors of society.
    Keywords aluminum ; batteries ; carbon dioxide ; electric potential difference ; iodides ; nuclear magnetic resonance spectroscopy ; oxalates ; Al−CO2 battery ; homogeneous catalyst ; redox mediator ; Al NMR ; electrolyte additive
    Language English
    Dates of publication 2023-0303
    Size p. 12908-12914.
    Publishing place American Chemical Society
    Document type Article ; Online
    ISSN 1944-8252
    DOI 10.1021/acsami.2c18323
    Database NAL-Catalogue (AGRICOLA)

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  2. Article ; Online: A Secondary Al-CO

    Fetrow, Christopher / Carugati, Cameron / Yu, Xingwen / Zhou, Xiao-Dong / Wei, Shuya

    ACS applied materials & interfaces

    2023  Volume 15, Issue 10, Page(s) 12908–12914

    Abstract: As an emerging energy storage concept, Al- ... ...

    Abstract As an emerging energy storage concept, Al-CO
    Language English
    Publishing date 2023-03-03
    Publishing country United States
    Document type Journal Article
    ISSN 1944-8252
    ISSN (online) 1944-8252
    DOI 10.1021/acsami.2c18323
    Database MEDical Literature Analysis and Retrieval System OnLINE

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    Order via subito

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  3. Article ; Online: Omecamtiv Mecarbil Enhances the Duty Ratio of Human β-Cardiac Myosin Resulting in Increased Calcium Sensitivity and Slowed Force Development in Cardiac Muscle.

    Swenson, Anja M / Tang, Wanjian / Blair, Cheavar A / Fetrow, Christopher M / Unrath, William C / Previs, Michael J / Campbell, Kenneth S / Yengo, Christopher M

    The Journal of biological chemistry

    2017  Volume 292, Issue 9, Page(s) 3768–3778

    Abstract: The small molecule drug omecamtiv mecarbil (OM) specifically targets cardiac muscle myosin and is known to enhance cardiac muscle performance, yet its impact on human cardiac myosin motor function is unclear. We expressed and purified human β-cardiac ... ...

    Abstract The small molecule drug omecamtiv mecarbil (OM) specifically targets cardiac muscle myosin and is known to enhance cardiac muscle performance, yet its impact on human cardiac myosin motor function is unclear. We expressed and purified human β-cardiac myosin subfragment 1 (M2β-S1) containing a C-terminal Avi tag. We demonstrate that the maximum actin-activated ATPase activity of M2β-S1 is slowed more than 4-fold in the presence of OM, whereas the actin concentration required for half-maximal ATPase was reduced dramatically (30-fold). We find OM does not change the overall actin affinity. Transient kinetic experiments suggest that there are two kinetic pathways in the presence of OM. The dominant pathway results in a slow transition between actomyosin·ADP states and increases the time myosin is strongly bound to actin. However, OM also traps a population of myosin heads in a weak actin affinity state with slow product release. We demonstrate that OM can reduce the actin sliding velocity more than 100-fold in the
    MeSH term(s) Actins/chemistry ; Actomyosin/chemistry ; Adenosine Diphosphate/chemistry ; Animals ; Calcium/chemistry ; Dose-Response Relationship, Drug ; Humans ; Kinetics ; Mass Spectrometry ; Mice ; Myocardium/metabolism ; Myosins/chemistry ; Protein Domains ; Recombinant Proteins/chemistry ; Stress, Mechanical ; Urea/analogs & derivatives ; Urea/chemistry ; Ventricular Myosins/chemistry
    Chemical Substances Actins ; Recombinant Proteins ; omecamtiv mecarbil (2M19539ERK) ; Adenosine Diphosphate (61D2G4IYVH) ; Urea (8W8T17847W) ; Actomyosin (9013-26-7) ; Ventricular Myosins (EC 3.6.1.-) ; Myosins (EC 3.6.4.1) ; Calcium (SY7Q814VUP)
    Language English
    Publishing date 2017-01-12
    Publishing country United States
    Document type Journal Article ; Research Support, N.I.H., Extramural ; Research Support, Non-U.S. Gov't
    ZDB-ID 2997-x
    ISSN 1083-351X ; 0021-9258
    ISSN (online) 1083-351X
    ISSN 0021-9258
    DOI 10.1074/jbc.M116.748780
    Database MEDical Literature Analysis and Retrieval System OnLINE

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