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Article ; Online: Nitrate Radicals Suppress Biogenic New Particle Formation from Monoterpene Oxidation.

Li, Dandan / Huang, Wei / Wang, Dongyu / Wang, Mingyi / Thornton, Joel A / Caudillo, Lucía / Rörup, Birte / Marten, Ruby / Scholz, Wiebke / Finkenzeller, Henning / Marie, Guillaume / Baltensperger, Urs / Bell, David M / Brasseur, Zoé / Curtius, Joachim / Dada, Lubna / Duplissy, Jonathan / Gong, Xianda / Hansel, Armin /

He, Xu-Cheng / Hofbauer, Victoria / Junninen, Heikki / Krechmer, Jordan E / Kürten, Andreas / Lamkaddam, Houssni / Lehtipalo, Katrianne / Lopez, Brandon / Ma, Yingge / Mahfouz, Naser G A / Manninen, Hanna E / Mentler, Bernhard / Perrier, Sebastien / Petäjä, Tuukka / Pfeifer, Joschka / Philippov, Maxim / Schervish, Meredith / Schobesberger, Siegfried / Shen, Jiali / Surdu, Mihnea / Tomaz, Sophie / Volkamer, Rainer / Wang, Xinke / Weber, Stefan K / Welti, André / Worsnop, Douglas R / Wu, Yusheng / Yan, Chao / Zauner-Wieczorek, Marcel / Kulmala, Markku / Kirkby, Jasper / Donahue, Neil M / George, Christian / El-Haddad, Imad / Bianchi, Federico / Riva, Matthieu

Environmental science & technology

2024 Volume 58, Issue 3, Page(s) 1601–1614

Abstract: Highly oxygenated organic molecules (HOMs) are a major source of new particles that affect the Earth's climate. HOM production from the oxidation of volatile organic compounds (VOCs) occurs during both the day and night and can lead to new particle ... ...

Abstract	Highly oxygenated organic molecules (HOMs) are a major source of new particles that affect the Earth's climate. HOM production from the oxidation of volatile organic compounds (VOCs) occurs during both the day and night and can lead to new particle formation (NPF). However, NPF involving organic vapors has been reported much more often during the daytime than during nighttime. Here, we show that the nitrate radicals (NO
MeSH term(s)	Monoterpenes/chemistry ; Nitrates/chemistry ; Aerosols/analysis ; Air Pollutants ; Volatile Organic Compounds/chemistry ; Ozone ; Bicyclic Monoterpenes
Chemical Substances	Monoterpenes ; alpha-pinene (JPF3YI7O34) ; Nitrates ; Aerosols ; Air Pollutants ; Volatile Organic Compounds ; Ozone (66H7ZZK23N) ; Bicyclic Monoterpenes
Language	English
Publishing date	2024-01-07
Publishing country	United States
Document type	Journal Article
ISSN	1520-5851
ISSN (online)	1520-5851
DOI	10.1021/acs.est.3c07958
Database	MEDical Literature Analysis and Retrieval System OnLINE

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Article ; Online: Assessing the importance of nitric acid and ammonia for particle growth in the polluted boundary layer.

Marten, Ruby / Xiao, Mao / Wang, Mingyi / Kong, Weimeng / He, Xu-Cheng / Stolzenburg, Dominik / Pfeifer, Joschka / Marie, Guillaume / Wang, Dongyu S / Elser, Miriam / Baccarini, Andrea / Lee, Chuan Ping / Amorim, Antonio / Baalbaki, Rima / Bell, David M / Bertozzi, Barbara / Caudillo, Lucía / Dada, Lubna / Duplissy, Jonathan /

Finkenzeller, Henning / Heinritzi, Martin / Lampimäki, Markus / Lehtipalo, Katrianne / Manninen, Hanna E / Mentler, Bernhard / Onnela, Antti / Petäjä, Tuukka / Philippov, Maxim / Rörup, Birte / Scholz, Wiebke / Shen, Jiali / Tham, Yee Jun / Tomé, António / Wagner, Andrea C / Weber, Stefan K / Zauner-Wieczorek, Marcel / Curtius, Joachim / Kulmala, Markku / Volkamer, Rainer / Worsnop, Douglas R / Dommen, Josef / Flagan, Richard C / Kirkby, Jasper / McPherson Donahue, Neil / Lamkaddam, Houssni / Baltensperger, Urs / El Haddad, Imad

Environmental science: atmospheres

2024 Volume 4, Issue 2, Page(s) 265–274

Abstract: Aerosols formed and grown by gas-to-particle processes are a major contributor to smog and haze in megacities, despite the competition between growth and loss rates. Rapid growth rates from ammonium nitrate formation have the potential to sustain ... ...

Abstract	Aerosols formed and grown by gas-to-particle processes are a major contributor to smog and haze in megacities, despite the competition between growth and loss rates. Rapid growth rates from ammonium nitrate formation have the potential to sustain particle number in typical urban polluted conditions. This process requires supersaturation of gas-phase ammonia and nitric acid with respect to ammonium nitrate saturation ratios. Urban environments are inhomogeneous. In the troposphere, vertical mixing is fast, and aerosols may experience rapidly changing temperatures. In areas close to sources of pollution, gas-phase concentrations can also be highly variable. In this work we present results from nucleation experiments at -10 °C and 5 °C in the CLOUD chamber at CERN. We verify, using a kinetic model, how long supersaturation is likely to be sustained under urban conditions with temperature and concentration inhomogeneities, and the impact it may have on the particle size distribution. We show that rapid and strong temperature changes of 1 °C min
Language	English
Publishing date	2024-01-25
Publishing country	England
Document type	Journal Article
ISSN	2634-3606
ISSN (online)	2634-3606
DOI	10.1039/d3ea00001j
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Book ; Online: Origin of water-soluble organic aerosols at the Maïdo high-altitude observatory, Réunion Island in the tropical Indian Ocean

Simu, Sharmine Akter / Miyazaki, Yuzo / Tachibana, Eri / Finkenzeller, Henning / Brioude, Jérôme / Colomb, Aurélie / Magand, Olivier / Verreyken, Bert / Evan, Stephanie / Volkamer, Rainer / Stavrakou, Trissevgeni

eISSN: 1680-7324

2021

Abstract: The tropical and subtropical Indian Ocean (IO) is expected to be a significant source of water-soluble organic aerosols (WSOAs), which are important factors relevant to cloud condensation nuclei and ice nuclei of aerosol particles. Current atmospheric ... ...

Abstract	The tropical and subtropical Indian Ocean (IO) is expected to be a significant source of water-soluble organic aerosols (WSOAs), which are important factors relevant to cloud condensation nuclei and ice nuclei of aerosol particles. Current atmospheric numerical models significantly underestimate the budget of organic aerosols and their precursors, especially over tropical oceans. This is primarily due to poor knowledge of sources and the paucity of observations of these parameters considering spatial and temporal variation over the tropical open ocean. To evaluate the contribution of sources to WSOA as well as their formation processes, submicrometer aerosol sampling was conducted at the high-altitude Maïdo observatory (21.1° S, 55.4° E, 2,160 m a.s.l), located on the remote island of La Réunion in the southwest IO. The aerosol samples were continuously collected during local daytime and nighttime, which corresponded to the ambient conditions of the marine boundary layer (MBL) and free troposphere (FT), respectively, from March 15 to May 24, 2018. Chemical analysis showed that organic matter was the dominant component of submicrometer water-soluble aerosol (~45 ± 17 %) during the wet season (March 15–April 23), whereas sulfate dominated (~77 ± 17 %) during the dry season (April 24–May 24). Measurements of the stable carbon isotope ratio of water-soluble organic carbon (WSOC) suggested that marine sources contributed significantly to the observed WSOC mass in both the MBL and the FT in the wet season, whereas a mixture of marine and terrestrial sources contributed to WSOC in the dry season. The distinct seasonal changes in the dominant source of WSOC were also supported by Lagrangian trajectory analysis. Positive matrix factorization analysis suggested that marine secondary OA dominantly contributed to the observed WSOC mass (~70 %) during the wet season, whereas mixtures of marine and terrestrial sources contributed during the dry season in both MBL and FT. Overall, this study demonstrates that the effect of marine secondary sources is likely important up to the FT in the wet season, which may be responsible for cloud formation as well as direct radiative forcing over oceanic regions.
Subject code	550 ; 551
Language	English
Publishing date	2021-06-01
Publishing country	de
Document type	Book ; Online
Database	BASE - Bielefeld Academic Search Engine (life sciences selection)

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Book ; Online: Measurement of iodine species and sulfuric acid using bromide chemical ionization mass spectrometers

Wang, Mingyi / He, Xu-Cheng / Finkenzeller, Henning / Iyer, Siddharth / Chen, Dexian / Shen, Jiali / Simon, Mario / Hofbauer, Victoria / Kirkby, Jasper / Curtius, Joachim / Maier, Norbert / Kurtén, Theo / Worsnop, Douglas R. / Kulmala, Markku / Rissanen, Matti / Volkamer, Rainer / Tham, Yee Jun / Donahue, Neil M. / Sipilä, Mikko

eISSN: 1867-8548

2021

Abstract: Iodine species are important in the marine atmosphere for oxidation and new-particle formation. Understanding iodine chemistry and iodine new-particle formation requires high time resolution, high sensitivity, and simultaneous measurements of many iodine ...

Abstract	Iodine species are important in the marine atmosphere for oxidation and new-particle formation. Understanding iodine chemistry and iodine new-particle formation requires high time resolution, high sensitivity, and simultaneous measurements of many iodine species. Here, we describe the application of a bromide chemical ionization mass spectrometer (Br-CIMS) to this task. During the iodine oxidation experiments in the Cosmics Leaving OUtdoor Droplets (CLOUD) chamber, we have measured gas-phase iodine species and sulfuric acid using two Br-CIMS, one coupled to a Multi-scheme chemical IONization inlet (Br-MION-CIMS) and the other to a Filter Inlet for Gasses and AEROsols inlet (Br-FIGAERO-CIMS). From offline calibrations and intercomparisons with other instruments, we have quantified the sensitivities of the Br-MION-CIMS to HOI, I 2 , and H 2 SO 4 and obtained detection limits of 5.8 × 10 6 , 3.8 × 10 5 , and 2.0 × 10 5 molec. cm −3 , respectively, for a 2 min integration time. From binding energy calculations, we estimate the detection limit for HIO 3 to be 1.2 × 10 5 molec. cm −3 , based on an assumption of maximum sensitivity. Detection limits in the Br-FIGAERO-CIMS are around 1 order of magnitude higher than those in the Br-MION-CIMS; for example, the detection limits for HOI and HIO 3 are 3.3 × 10 7 and 5.1 × 10 6 molec. cm −3 , respectively. Our comparisons of the performance of the MION inlet and the FIGAERO inlet show that bromide chemical ionization mass spectrometers using either atmospheric pressure or reduced pressure interfaces are well-matched to measuring iodine species and sulfuric acid in marine environments.
Subject code	333 ; 511
Language	English
Publishing date	2021-06-07
Publishing country	de
Document type	Book ; Online
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Article ; Online: NO at low concentration can enhance the formation of highly oxygenated biogenic molecules in the atmosphere.

Nie, Wei / Yan, Chao / Yang, Liwen / Roldin, Pontus / Liu, Yuliang / Vogel, Alexander L / Molteni, Ugo / Stolzenburg, Dominik / Finkenzeller, Henning / Amorim, Antonio / Bianchi, Federico / Curtius, Joachim / Dada, Lubna / Draper, Danielle C / Duplissy, Jonathan / Hansel, Armin / He, Xu-Cheng / Hofbauer, Victoria / Jokinen, Tuija /

Kim, Changhyuk / Lehtipalo, Katrianne / Nichman, Leonid / Mauldin, Roy L / Makhmutov, Vladimir / Mentler, Bernhard / Mizelli-Ojdanic, Andrea / Petäjä, Tuukka / Quéléver, Lauriane L J / Schallhart, Simon / Simon, Mario / Tauber, Christian / Tomé, António / Volkamer, Rainer / Wagner, Andrea C / Wagner, Robert / Wang, Mingyi / Ye, Penglin / Li, Haiyan / Huang, Wei / Qi, Ximeng / Lou, Sijia / Liu, Tengyu / Chi, Xuguang / Dommen, Josef / Baltensperger, Urs / El Haddad, Imad / Kirkby, Jasper / Worsnop, Douglas / Kulmala, Markku / Donahue, Neil M / Ehn, Mikael / Ding, Aijun

Nature communications

2023 Volume 14, Issue 1, Page(s) 3347

Abstract: The interaction between nitrogen monoxide (NO) and organic peroxy radicals ( ... ...

Abstract	The interaction between nitrogen monoxide (NO) and organic peroxy radicals (RO
MeSH term(s)	Nitric Oxide ; Atmosphere ; Monoterpenes ; Oxidation-Reduction ; Aerosols
Chemical Substances	Nitric Oxide (31C4KY9ESH) ; Monoterpenes ; Aerosols
Language	English
Publishing date	2023-06-08
Publishing country	England
Document type	Journal Article
ZDB-ID	2553671-0
ISSN	2041-1723 ; 2041-1723
ISSN (online)	2041-1723
ISSN	2041-1723
DOI	10.1038/s41467-023-39066-4
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Article ; Online: Role of sesquiterpenes in biogenic new particle formation.

Dada, Lubna / Stolzenburg, Dominik / Simon, Mario / Fischer, Lukas / Heinritzi, Martin / Wang, Mingyi / Xiao, Mao / Vogel, Alexander L / Ahonen, Lauri / Amorim, Antonio / Baalbaki, Rima / Baccarini, Andrea / Baltensperger, Urs / Bianchi, Federico / Daellenbach, Kaspar R / DeVivo, Jenna / Dias, Antonio / Dommen, Josef / Duplissy, Jonathan /

Finkenzeller, Henning / Hansel, Armin / He, Xu-Cheng / Hofbauer, Victoria / Hoyle, Christopher R / Kangasluoma, Juha / Kim, Changhyuk / Kürten, Andreas / Kvashnin, Aleksander / Mauldin, Roy / Makhmutov, Vladimir / Marten, Ruby / Mentler, Bernhard / Nie, Wei / Petäjä, Tuukka / Quéléver, Lauriane L J / Saathoff, Harald / Tauber, Christian / Tome, Antonio / Molteni, Ugo / Volkamer, Rainer / Wagner, Robert / Wagner, Andrea C / Wimmer, Daniela / Winkler, Paul M / Yan, Chao / Zha, Qiaozhi / Rissanen, Matti / Gordon, Hamish / Curtius, Joachim / Worsnop, Douglas R / Lehtipalo, Katrianne / Donahue, Neil M / Kirkby, Jasper / El Haddad, Imad / Kulmala, Markku

Science advances

2023 Volume 9, Issue 36, Page(s) eadi5297

Abstract: Biogenic vapors form new particles in the atmosphere, affecting global climate. The contributions of monoterpenes and isoprene to new particle formation (NPF) have been extensively studied. However, sesquiterpenes have received little attention despite a ...

Abstract	Biogenic vapors form new particles in the atmosphere, affecting global climate. The contributions of monoterpenes and isoprene to new particle formation (NPF) have been extensively studied. However, sesquiterpenes have received little attention despite a potentially important role due to their high molecular weight. Via chamber experiments performed under atmospheric conditions, we report biogenic NPF resulting from the oxidation of pure mixtures of β-caryophyllene, α-pinene, and isoprene, which produces oxygenated compounds over a wide range of volatilities. We find that a class of vapors termed ultralow-volatility organic compounds (ULVOCs) are highly efficient nucleators and quantitatively determine NPF efficiency. When compared with a mixture of isoprene and monoterpene alone, adding only 2% sesquiterpene increases the ULVOC yield and doubles the formation rate. Thus, sesquiterpene emissions need to be included in assessments of global aerosol concentrations in pristine climates where biogenic NPF is expected to be a major source of cloud condensation nuclei.
Language	English
Publishing date	2023-09-08
Publishing country	United States
Document type	Journal Article
ZDB-ID	2810933-8
ISSN	2375-2548 ; 2375-2548
ISSN (online)	2375-2548
ISSN	2375-2548
DOI	10.1126/sciadv.adi5297
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Article ; Online: Molecular Understanding of the Enhancement in Organic Aerosol Mass at High Relative Humidity.

Surdu, Mihnea / Lamkaddam, Houssni / Wang, Dongyu S / Bell, David M / Xiao, Mao / Lee, Chuan Ping / Li, Dandan / Caudillo, Lucía / Marie, Guillaume / Scholz, Wiebke / Wang, Mingyi / Lopez, Brandon / Piedehierro, Ana A / Ataei, Farnoush / Baalbaki, Rima / Bertozzi, Barbara / Bogert, Pia / Brasseur, Zoé / Dada, Lubna /

Duplissy, Jonathan / Finkenzeller, Henning / He, Xu-Cheng / Höhler, Kristina / Korhonen, Kimmo / Krechmer, Jordan E / Lehtipalo, Katrianne / Mahfouz, Naser G A / Manninen, Hanna E / Marten, Ruby / Massabò, Dario / Mauldin, Roy / Petäjä, Tuukka / Pfeifer, Joschka / Philippov, Maxim / Rörup, Birte / Simon, Mario / Shen, Jiali / Umo, Nsikanabasi Silas / Vogel, Franziska / Weber, Stefan K / Zauner-Wieczorek, Marcel / Volkamer, Rainer / Saathoff, Harald / Möhler, Ottmar / Kirkby, Jasper / Worsnop, Douglas R / Kulmala, Markku / Stratmann, Frank / Hansel, Armin / Curtius, Joachim / Welti, André / Riva, Matthieu / Donahue, Neil M / Baltensperger, Urs / El Haddad, Imad

Environmental science & technology

2023 Volume 57, Issue 6, Page(s) 2297–2309

Abstract: The mechanistic pathway by which high relative humidity (RH) affects gas-particle partitioning remains poorly understood, although many studies report increased secondary organic aerosol (SOA) yields at high RH. Here, we use real-time, molecular ... ...

Abstract	The mechanistic pathway by which high relative humidity (RH) affects gas-particle partitioning remains poorly understood, although many studies report increased secondary organic aerosol (SOA) yields at high RH. Here, we use real-time, molecular measurements of both the gas and particle phase to provide a mechanistic understanding of the effect of RH on the partitioning of biogenic oxidized organic molecules (from α-pinene and isoprene) at low temperatures (243 and 263 K) at the CLOUD chamber at CERN. We observe increases in SOA mass of 45 and 85% with increasing RH from 10-20 to 60-80% at 243 and 263 K, respectively, and attribute it to the increased partitioning of semi-volatile compounds. At 263 K, we measure an increase of a factor 2-4 in the concentration of C
MeSH term(s)	Monoterpenes/chemistry ; Air Pollutants ; Humidity ; Aerosols
Chemical Substances	Monoterpenes ; Air Pollutants ; Aerosols
Language	English
Publishing date	2023-01-30
Publishing country	United States
Document type	Journal Article ; Research Support, Non-U.S. Gov't ; Research Support, U.S. Gov't, Non-P.H.S.
ISSN	1520-5851
ISSN (online)	1520-5851
DOI	10.1021/acs.est.2c04587
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Book ; Online: Measurement of iodine species and sulfuric acid using bromide chemical ionization mass spectrometers

eISSN: 1867-8548

2020

Abstract	Iodine species are important in the marine atmosphere for oxidation and new-particle formation. Understanding iodine chemistry and iodine new-particle formation requires high time resolution, high sensitivity, and simultaneous measurements of many iodine species. Here, we describe the application of bromide chemical ionization mass spectrometers (Br-CIMS) to this task. During iodine new-particle formation experiments in the Cosmics Leaving OUtdoor Droplets (CLOUD) chamber, we have measured gas-phase iodine species and sulfuric acid using two Br-CIMS, one coupled to a Multi-scheme chemical IONization inlet (Br-MION-CIMS) and the other to a Filter Inlet for Gasses and AEROsols inlet (Br-FIGAERO-CIMS). From offline calibrations and inter-comparisons with other instruments attached to the CLOUD chamber, we have quantified the sensitivities of the Br-MION-CIMS to HOI, I 2 , and H 2 SO 4 and obtain detection limits of 5.8 × 10 6 , 6.3 × 10 5 , and 2.0 × 10 5 molec cm −3 , respectively, for a 2-min integration time. From binding energy calculations, we estimate the detection limit for HIO 3 to be 1.2 × 10 5 molec cm −3 , based on an assumption of maximum sensitivity. Detection limits in the Br-FIGAERO-CIMS are around one order of magnitude higher than those in the Br-MION-CIMS; for example, the detection limits for HOI and HIO 3 are 3.3 × 10 7 and 5.1 × 10 6 molec cm −3 , respectively. Our comparisons of the performance of the MION inlet and the FIGAERO inlet show that bromide chemical ionization mass spectrometers using either atmospheric pressure or reduced pressure interfaces are well-matched to measuring iodine species and sulfuric acid in marine environments.
Subject code	333
Language	English
Publishing date	2020-12-18
Publishing country	de
Document type	Book ; Online
Database	BASE - Bielefeld Academic Search Engine (life sciences selection)

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Article ; Online: Iodine oxoacids enhance nucleation of sulfuric acid particles in the atmosphere.

He, Xu-Cheng / Simon, Mario / Iyer, Siddharth / Xie, Hong-Bin / Rörup, Birte / Shen, Jiali / Finkenzeller, Henning / Stolzenburg, Dominik / Zhang, Rongjie / Baccarini, Andrea / Tham, Yee Jun / Wang, Mingyi / Amanatidis, Stavros / Piedehierro, Ana A / Amorim, Antonio / Baalbaki, Rima / Brasseur, Zoé / Caudillo, Lucía / Chu, Biwu /

Dada, Lubna / Duplissy, Jonathan / El Haddad, Imad / Flagan, Richard C / Granzin, Manuel / Hansel, Armin / Heinritzi, Martin / Hofbauer, Victoria / Jokinen, Tuija / Kemppainen, Deniz / Kong, Weimeng / Krechmer, Jordan / Kürten, Andreas / Lamkaddam, Houssni / Lopez, Brandon / Ma, Fangfang / Mahfouz, Naser G A / Makhmutov, Vladimir / Manninen, Hanna E / Marie, Guillaume / Marten, Ruby / Massabò, Dario / Mauldin, Roy L / Mentler, Bernhard / Onnela, Antti / Petäjä, Tuukka / Pfeifer, Joschka / Philippov, Maxim / Ranjithkumar, Ananth / Rissanen, Matti P / Schobesberger, Siegfried / Scholz, Wiebke / Schulze, Benjamin / Surdu, Mihnea / Thakur, Roseline C / Tomé, António / Wagner, Andrea C / Wang, Dongyu / Wang, Yonghong / Weber, Stefan K / Welti, André / Winkler, Paul M / Zauner-Wieczorek, Marcel / Baltensperger, Urs / Curtius, Joachim / Kurtén, Theo / Worsnop, Douglas R / Volkamer, Rainer / Lehtipalo, Katrianne / Kirkby, Jasper / Donahue, Neil M / Sipilä, Mikko / Kulmala, Markku

Science (New York, N.Y.)

2023 Volume 382, Issue 6676, Page(s) 1308–1314

Abstract: The main nucleating vapor in the atmosphere is thought to be sulfuric acid ( ... ...

Abstract	The main nucleating vapor in the atmosphere is thought to be sulfuric acid (H
Language	English
Publishing date	2023-12-14
Publishing country	United States
Document type	Journal Article
ZDB-ID	128410-1
ISSN	1095-9203 ; 0036-8075
ISSN (online)	1095-9203
ISSN	0036-8075
DOI	10.1126/science.adh2526
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Article ; Online: Survival of newly formed particles in haze conditions.

Marten, Ruby / Xiao, Mao / Rörup, Birte / Wang, Mingyi / Kong, Weimeng / He, Xu-Cheng / Stolzenburg, Dominik / Pfeifer, Joschka / Marie, Guillaume / Wang, Dongyu S / Scholz, Wiebke / Baccarini, Andrea / Lee, Chuan Ping / Amorim, Antonio / Baalbaki, Rima / Bell, David M / Bertozzi, Barbara / Caudillo, Lucía / Chu, Biwu /

Dada, Lubna / Duplissy, Jonathan / Finkenzeller, Henning / Carracedo, Loïc Gonzalez / Granzin, Manuel / Hansel, Armin / Heinritzi, Martin / Hofbauer, Victoria / Kemppainen, Deniz / Kürten, Andreas / Lampimäki, Markus / Lehtipalo, Katrianne / Makhmutov, Vladimir / Manninen, Hanna E / Mentler, Bernhard / Petäjä, Tuukka / Philippov, Maxim / Shen, Jiali / Simon, Mario / Stozhkov, Yuri / Tomé, António / Wagner, Andrea C / Wang, Yonghong / Weber, Stefan K / Wu, Yusheng / Zauner-Wieczorek, Marcel / Curtius, Joachim / Kulmala, Markku / Möhler, Ottmar / Volkamer, Rainer / Winkler, Paul M / Worsnop, Douglas R / Dommen, Josef / Flagan, Richard C / Kirkby, Jasper / Donahue, Neil M / Lamkaddam, Houssni / Baltensperger, Urs / El Haddad, Imad

Environmental science: atmospheres

2022 Volume 2, Issue 3, Page(s) 491–499

Abstract: Intense new particle formation events are regularly observed under highly polluted conditions, despite the high loss rates of nucleated clusters. Higher than expected cluster survival probability implies either ineffective scavenging by pre-existing ... ...

Abstract	Intense new particle formation events are regularly observed under highly polluted conditions, despite the high loss rates of nucleated clusters. Higher than expected cluster survival probability implies either ineffective scavenging by pre-existing particles or missing growth mechanisms. Here we present experiments performed in the CLOUD chamber at CERN showing particle formation from a mixture of anthropogenic vapours, under condensation sinks typical of haze conditions, up to 0.1 s
Language	English
Publishing date	2022-04-08
Publishing country	England
Document type	Journal Article
ISSN	2634-3606
ISSN (online)	2634-3606
DOI	10.1039/d2ea00007e
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