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  1. Article: Strategies to Improve the Energy Storage Properties of Perovskite Lead-Free Relaxor Ferroelectrics: A Review.

    Veerapandiyan, Vignaswaran / Benes, Federica / Gindel, Theresa / Deluca, Marco

    Materials (Basel, Switzerland)

    2020  Volume 13, Issue 24

    Abstract: Electrical energy storage systems (EESSs) with high energy density and power density are essential for the effective miniaturization of future electronic devices. Among different EESSs available in the market, dielectric capacitors relying on swift ... ...

    Abstract Electrical energy storage systems (EESSs) with high energy density and power density are essential for the effective miniaturization of future electronic devices. Among different EESSs available in the market, dielectric capacitors relying on swift electronic and ionic polarization-based mechanisms to store and deliver energy already demonstrate high power densities. However, different intrinsic and extrinsic contributions to energy dissipations prevent ceramic-based dielectric capacitors from reaching high recoverable energy density levels. Interestingly, relaxor ferroelectric-based dielectric capacitors, because of their low remnant polarization, show relatively high energy density and thus display great potential for applications requiring high energy density properties. In this study, some of the main strategies to improve the energy density properties of perovskite lead-free relaxor systems are reviewed, including (i) chemical modification at different crystallographic sites, (ii) chemical additives that do not target lattice sites, and (iii) novel processing approaches dedicated to bulk ceramics, thick and thin films, respectively. Recent advancements are summarized concerning the search for relaxor materials with superior energy density properties and the appropriate choice of both composition and processing routes to match various applications' needs. Finally, future trends in computationally-aided materials design are presented.
    Language English
    Publishing date 2020-12-16
    Publishing country Switzerland
    Document type Journal Article ; Review
    ZDB-ID 2487261-1
    ISSN 1996-1944
    ISSN 1996-1944
    DOI 10.3390/ma13245742
    Database MEDical Literature Analysis and Retrieval System OnLINE

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  2. Book ; Online: Strategies to Improve the Energy Storage Properties of Perovskite Lead-Free Relaxor Ferroelectrics

    Veerapandiyan, Vignaswaran / Benes, Federica / Gindel, Theresa / Deluca, Marco

    A Review

    2021  

    Abstract: Electrical energy storage systems (EESSs) with high energy density and power density are essential for the effective miniaturization of future electronic devices. Among different EESSs available in the market, dielectric capacitors relying on swift ... ...

    Abstract Electrical energy storage systems (EESSs) with high energy density and power density are essential for the effective miniaturization of future electronic devices. Among different EESSs available in the market, dielectric capacitors relying on swift electronic and ionic polarization-based mechanisms to store and deliver energy already demonstrate high power densities. However, different intrinsic and extrinsic contributions to energy dissipations prevent ceramic-based dielectric capacitors from reaching high recoverable energy density levels. Interestingly, relaxor ferroelectric-based dielectric capacitors, because of their low remnant polarization, show relatively high energy density and thus display great potential for applications requiring high energy density properties. Here, some of the main strategies to improve the energy density properties of perovskite lead-free relaxor systems are reviewed. This includes (i) chemical modification at different crystallographic sites, (ii) chemical additives that do not target lattice sites and (iii) novel processing approaches dedicated to bulk ceramics, thick and thin films, respectively. Recent advancements are summarized concerning the search for relaxor materials with superior energy density properties and the appropriate choice of both composition and processing route to match various needs in the application. Finally, future trends in computationally-aided materials design are presented.

    Comment: 47 pages, 11 figures, 2 tables
    Keywords Condensed Matter - Materials Science
    Subject code 541
    Publishing date 2021-04-08
    Publishing country us
    Document type Book ; Online
    Database BASE - Bielefeld Academic Search Engine (life sciences selection)

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  3. Book ; Online: Hexavalent (Me-W/Mo)-modified (Ba,Ca)TiO$_3$-Bi(Mg,Me)O$_3$ perovskites for high-temperature dielectrics

    Schulz, Thomas / Veerapandiyan, Vignaswaran K. / Gindel, Theresa / Deluca, Marco / Töpfer, Jörg

    2021  

    Abstract: We report on the synthesis of complex lead-free perovskite-type (1-x)(Ba$_{0.8}$Ca$_{0.2}$)TiO$_3$-xBi(Mg$_{0.75}$W$_{0.25}$)O$_3$ (BCT-xBMW) and (1-x)(Ba$_{0.8}$Ca$_{0.2}$)TiO$_3$-xBi(Mg$_{0.75}$Mo$_{0.25}$)O$_3$ (BCT-xBMM) solid solutions via ... ...

    Abstract We report on the synthesis of complex lead-free perovskite-type (1-x)(Ba$_{0.8}$Ca$_{0.2}$)TiO$_3$-xBi(Mg$_{0.75}$W$_{0.25}$)O$_3$ (BCT-xBMW) and (1-x)(Ba$_{0.8}$Ca$_{0.2}$)TiO$_3$-xBi(Mg$_{0.75}$Mo$_{0.25}$)O$_3$ (BCT-xBMM) solid solutions via conventional solid-state reaction route. The sintering temperature was adjusted as a function of composition x to obtain dense samples (relative densities over 95%) at the same time minimizing bismuth evaporation. X-ray diffraction analysis shows formation of single-phase perovskites for $0 \le x \le 0.10$ in the BCT-xBMW series and increasing concentrations of impurity phases for $x \ge 0.15$ and for $x \ge 0.05$ in BCT-xBMM. A transition from a tetragonal to pseudo-cubic perovskite structure is observed in BCT-xBMW and BCT-xBMM at $x = 0.05$. The dielectric response has been characterized between -60 $^\circ$C and 300 $^\circ$C for BCT-xBMW, and between 30 $^\circ$C and 300 $^\circ$C for BCT-xBMM using impedance spectroscopy, showing a transition from ferroelectric to relaxor-like behavior at $x \ge 0.05$. Additional polarization and Raman spectroscopy measurements reveal the occurrence of highly disordered systems. Analysis of the Raman spectra indicates structural phase changes and lattice modifications caused by chemical substitution. For the composition 0.8Ba$_{0.8}$Ca$_{0.2}$TiO$_3$-0.2Bi(Mg$_{0.75}$W$_{0.25}$)O$_3$ a temperature-stable permittivity of about 600 ($\pm 15$% between 60 $^\circ$C and 300 $^\circ$C) and small losses of $\tan\delta < 0.02$ for $T \le 230$ $^\circ$C at 1 kHz are observed, making it a suitable dielectric material for high temperature capacitors.
    Keywords Condensed Matter - Materials Science
    Subject code 669
    Publishing date 2021-10-29
    Publishing country us
    Document type Book ; Online
    Database BASE - Bielefeld Academic Search Engine (life sciences selection)

    Full text online

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    Inter-library loan at ZB MED

    Your chosen title can be delivered directly to ZB MED Cologne location if you are registered as a user at ZB MED Cologne.

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