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Article ; Online: Correction to Redox Catalysis Promoted Activation of Sulfur Redox Chemistry for Energy-Dense Flexible Solid-State Zn-S Battery.

Zhang, Hong / Shang, Zhoutai / Luo, Gen / Jiao, Shuhong / Cao, Ruiguo / Chen, Qianwang / Lu, Ke

ACS nano

2022 Volume 16, Issue 4, Page(s) 6937–6938

Language	English
Publishing date	2022-03-24
Publishing country	United States
Document type	Published Erratum
ISSN	1936-086X
ISSN (online)	1936-086X
DOI	10.1021/acsnano.2c02258
Database	MEDical Literature Analysis and Retrieval System OnLINE

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Article ; Online: Unveiling the Critical Role of Ion Coordination Configuration of Ether Electrolytes for High Voltage Lithium Metal Batteries.

Chen, Shunqiang / Fan, JiaJia / Cui, Zhuangzhuang / Tan, Lijiang / Ruan, Digen / Zhao, Xin / Jiang, Jinyu / Jiao, Shuhong / Ren, Xiaodi

Angewandte Chemie (International ed. in English)

2023 Volume 62, Issue 23, Page(s) e202219310

Abstract: Albeit ethers are favorable electrolyte solvents for lithium (Li) metal anode, their inferior oxidation stability (<4.0 V vs. Li/ ... ...

Abstract	Albeit ethers are favorable electrolyte solvents for lithium (Li) metal anode, their inferior oxidation stability (<4.0 V vs. Li/Li
Language	English
Publishing date	2023-04-28
Publishing country	Germany
Document type	Journal Article
ZDB-ID	2011836-3
ISSN	1521-3773 ; 1433-7851
ISSN (online)	1521-3773
ISSN	1433-7851
DOI	10.1002/anie.202219310
Database	MEDical Literature Analysis and Retrieval System OnLINE

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Article ; Online: Monolithic Nickel Catalyst Featured with High-Density Crystalline Steps for Stable Hydrogen Evolution at Large Current Density.

Lei, Zhanwu / Liu, Peng / Yang, Xin / Zou, Peichao / Nairan, Adeela / Jiao, Shuhong / Cao, Ruiguo / Wang, Wenlong / Kang, Feiyu / Yang, Cheng

Small (Weinheim an der Bergstrasse, Germany)

2023 Volume 19, Issue 33, Page(s) e2301247

Abstract: Producing hydrogen via electrochemical water splitting with minimum environmental harm can help resolve the energy crisis in a sustainable way. Here, this work fabricates the pure nickel nanopyramid arrays (NNAs) with dense high-index crystalline steps ... ...

Abstract	Producing hydrogen via electrochemical water splitting with minimum environmental harm can help resolve the energy crisis in a sustainable way. Here, this work fabricates the pure nickel nanopyramid arrays (NNAs) with dense high-index crystalline steps as the cata electrode via a screw dislocation-dominated growth kinetic for long-term durable and large current density hydrogen evolution reaction. Such a monolithic NNAs electrode offers an ultralow overpotential of 469 mV at a current density of 5000 mA cm
Language	English
Publishing date	2023-04-22
Publishing country	Germany
Document type	Journal Article
ZDB-ID	2168935-0
ISSN	1613-6829 ; 1613-6810
ISSN (online)	1613-6829
ISSN	1613-6810
DOI	10.1002/smll.202301247
Database	MEDical Literature Analysis and Retrieval System OnLINE

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Article ; Online: Molecular anchoring of free solvents for high-voltage and high-safety lithium metal batteries.

Cui, Zhuangzhuang / Jia, Zhuangzhuang / Ruan, Digen / Nian, Qingshun / Fan, Jiajia / Chen, Shunqiang / He, Zixu / Wang, Dazhuang / Jiang, Jinyu / Ma, Jun / Ou, Xing / Jiao, Shuhong / Wang, Qingsong / Ren, Xiaodi

Nature communications

2024 Volume 15, Issue 1, Page(s) 2033

Abstract: Constraining the electrochemical reactivity of free solvent molecules is pivotal for developing high-voltage lithium metal batteries, especially for ether solvents with high Li metal compatibility but low oxidation stability ( <4.0 V vs ... ...

Abstract	Constraining the electrochemical reactivity of free solvent molecules is pivotal for developing high-voltage lithium metal batteries, especially for ether solvents with high Li metal compatibility but low oxidation stability ( <4.0 V vs Li
Language	English
Publishing date	2024-03-06
Publishing country	England
Document type	Journal Article
ZDB-ID	2553671-0
ISSN	2041-1723 ; 2041-1723
ISSN (online)	2041-1723
ISSN	2041-1723
DOI	10.1038/s41467-024-46186-y
Database	MEDical Literature Analysis and Retrieval System OnLINE

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Article ; Online: Using the Natural Scenes’ Edges for Assessing Image Quality Blindly and Efficiently

Saifeldeen Abdalmajeed / Jiao Shuhong

Mathematical Problems in Engineering, Vol

2015 Volume 2015

Keywords	Mathematics ; QA1-939 ; Science ; Q ; Engineering (General). Civil engineering (General) ; TA1-2040 ; Technology ; T
Language	English
Publishing date	2015-01-01T00:00:00Z
Publisher	Hindawi Publishing Corporation
Document type	Article ; Online
Database	BASE - Bielefeld Academic Search Engine (life sciences selection)

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Article: Regulating Li₂S Deposition by Ostwald Ripening in Lithium–Sulfur Batteries

Wang, Shuai / Huang, Fanyang / Li, Xinpeng / Li, Wanxia / Chen, Yawei / Tang, Xin / Jiao, Shuhong / Cao, Ruiguo

ACS applied materials & interfaces. 2022 Jan. 14, v. 14, no. 3

2022

Abstract: The lithium–sulfur (Li–S) batteries have attracted tremendous attention from both academia and industry for their high energy density and environmental benignity. However, the cell performance suffers from the passivation of the conductive matrix caused ... ...

Abstract	The lithium–sulfur (Li–S) batteries have attracted tremendous attention from both academia and industry for their high energy density and environmental benignity. However, the cell performance suffers from the passivation of the conductive matrix caused by uncontrolled lithium sulfide (Li₂S) deposition. Therefore, regulation of Li₂S deposition is essential to advanced Li–S batteries. In this work, the role of temperature in regulating Li₂S deposition is comprehensively investigated. At room temperature (25 °C), Li₂S exhibits a two-dimensional (2D) growth mode. The dense and insulating Li₂S film covers the conductive surface rapidly, inhibiting the charge transfer for subsequent polysulfide reduction. Consequently, the severe passivation of the conductive surface degrades the cell performance. In contrast, three-dimensional (3D) Li₂S is formed at a high temperature (60 °C) because of a faster Ostwald ripening rate at an elevated temperature. The passivation of the conductive matrix is mitigated effectively, and the cell performance is enhanced significantly, thanks to the formation of 3D Li₂S. Ostwald ripening is also valid for Li–S cells under rigorous conditions. The cell working at 60 °C achieves a high specific capacity of 1228 mA h g–¹ under the conditions of high S loading and a lean electrolyte (S loading = 3.6 mg cm–², electrolyte/sulfur ratio = 3 μL mg–¹), which is substantially higher than that at 25 °C. This work enriches the intrinsic understanding of Li₂S deposition in Li–S batteries and provides facile strategies for improving the cell performance under practical conditions.
Keywords	ambient temperature ; electrolytes ; energy density ; industry ; lithium sulfide ; sulfur
Language	English
Dates of publication	2022-0114
Size	p. 4204-4210.
Publishing place	American Chemical Society
Document type	Article
ISSN	1944-8252
DOI	10.1021/acsami.1c22025
Database	NAL-Catalogue (AGRICOLA)

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Article ; Online: Ensemble Effect of Ruthenium Single-Atom and Nanoparticle Catalysts for Efficient Hydrogen Evolution in Neutral Media

Liu, Yang / Wu, Jianghua / Zhang, Yuchen / Jin, Xu / Li, Jianming / Xi, Xiaoke / Deng, Yu / Jiao, Shuhong / Lei, Zhanwu / Lee, L. H. Y. / Cao, Ruiguo

ACS Applied Materials & Interfaces. 2023 Mar. 11, v. 15, no. 11 p.14240-14249

2023

Abstract: Hydrogen evolution reaction (HER) plays a key role in electrochemical water splitting, which is a sustainable way for hydrogen production. The kinetics of HER is sluggish in neutral media that requires noble metal catalysts to alleviate energy ... ...

Abstract	Hydrogen evolution reaction (HER) plays a key role in electrochemical water splitting, which is a sustainable way for hydrogen production. The kinetics of HER is sluggish in neutral media that requires noble metal catalysts to alleviate energy consumption during the HER process. Here, we present a catalyst comprising a ruthenium single atom (Ru₁) and nanoparticle (Ruₙ) loaded on the nitrogen-doped carbon substrate (Ru₁-Ruₙ/CN), which exhibits excellent activity and superior durability for neutral HER. Benefiting from the synergistic effect between single atoms and nanoparticles in the Ru₁-Ruₙ/CN, the catalyst exhibits a very low overpotential down to 32 mV at a current density of 10 mA cm-² while maintaining excellent stability up to 700 h at a current density of 20 mA cm-² during the long-term test. Computational calculations reveal that, in the Ru₁-Ruₙ/CN catalyst, the existence of Ru nanoparticles affects the interactions between Ru single-atom sites and reactants and thus improves the catalytic activity of HER. This work highlights the ensemble effect of electrocatalysts for HER and could shed light on the rational design of efficient catalysts for other multistep electrochemical reactions.
Keywords	carbon ; catalysts ; catalytic activity ; durability ; electrochemistry ; energy ; hydrogen production ; nanoparticles ; ruthenium ; synergism ; single atom ; nanoparticle ; synergistic effects ; hydrogen evolution reaction ; neutral water splitting
Language	English
Dates of publication	2023-0311
Size	p. 14240-14249.
Publishing place	American Chemical Society
Document type	Article ; Online
ISSN	1944-8252
DOI	10.1021/acsami.2c20863
Database	NAL-Catalogue (AGRICOLA)

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Article ; Online: Redox Catalysis Promoted Activation of Sulfur Redox Chemistry for Energy-Dense Flexible Solid-State Zn-S Battery.

Zhang, Hong / Shang, Zhoutai / Luo, Gen / Jiao, Shuhong / Cao, Ruiguo / Chen, Qianwang / Lu, Ke

ACS nano

2021 Volume 16, Issue 5, Page(s) 7344–7351

Abstract: In aqueous Zn-ion batteries, the intercalation chemistry often foil attempts at the realization of high energy density. Unlocking the full potential of zinc-sulfur redox chemistry requires the manipulation of the feedbacks between kinetic response and ... ...

Abstract	In aqueous Zn-ion batteries, the intercalation chemistry often foil attempts at the realization of high energy density. Unlocking the full potential of zinc-sulfur redox chemistry requires the manipulation of the feedbacks between kinetic response and the cathode's composition. The cell degradation mechanism also should be tracked simultaneously. Herein, we design a high-energy Zn-S system where the high-capacity cathode was fabricated by
Language	English
Publishing date	2021-12-10
Publishing country	United States
Document type	Journal Article
ISSN	1936-086X
ISSN (online)	1936-086X
DOI	10.1021/acsnano.1c08645
Database	MEDical Literature Analysis and Retrieval System OnLINE

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Article ; Online: Regulating Li

Wang, Shuai / Huang, Fanyang / Li, Xinpeng / Li, Wanxia / Chen, Yawei / Tang, Xin / Jiao, Shuhong / Cao, Ruiguo

ACS applied materials & interfaces

2022 Volume 14, Issue 3, Page(s) 4204–4210

Abstract: The lithium-sulfur (Li-S) batteries have attracted tremendous attention from both academia and industry for their high energy density and environmental benignity. However, the cell performance suffers from the passivation of the conductive matrix caused ... ...

Abstract	The lithium-sulfur (Li-S) batteries have attracted tremendous attention from both academia and industry for their high energy density and environmental benignity. However, the cell performance suffers from the passivation of the conductive matrix caused by uncontrolled lithium sulfide (Li
Language	English
Publishing date	2022-01-14
Publishing country	United States
Document type	Journal Article
ISSN	1944-8252
ISSN (online)	1944-8252
DOI	10.1021/acsami.1c22025
Database	MEDical Literature Analysis and Retrieval System OnLINE

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Article ; Online: Constructing Three-Dimensional Topological Zn Deposition for Long-Life Aqueous Zn-Ion Batteries.

Yan, Mengdie / Huang, Fanyang / Zhao, Xuesong / Zhang, Fenglin / Dong, Ning / Jiao, Shuhong / Cao, Ruiguo / Pan, Huilin

ACS applied materials & interfaces

2022 Volume 14, Issue 45, Page(s) 51010–51017

Abstract: Uniform and compact Zn deposition-dissolution is essential to achieve high Coulombic efficiency and long lifespan for Zn anodes. More attention has been commonly focused on the suppression of macroscopic Zn dendrites in the previous reports. The rational ...

Abstract	Uniform and compact Zn deposition-dissolution is essential to achieve high Coulombic efficiency and long lifespan for Zn anodes. More attention has been commonly focused on the suppression of macroscopic Zn dendrites in the previous reports. The rational control of the microstructure of Zn deposition to prevent the intrinsic volume expansion and pulverization of Zn metal so as to stabilize Zn anodes is less discussed. Herein, we construct a three-dimensional topological Zn deposition at the nanoscale through an in situ electrochemical process in the optimal hybrid aqueous electrolyte. The topological electrode structure can efficiently accommodate microscopic strain and volume variation and thus largely preserve the macroscopic integrity and electrical contact of Zn anodes, leading to enhanced reversibility and stability. With the unique topological structure of Zn deposition, the Coulombic efficiency of Zn anodes could reach >99.9% with excellent cycling over 1182 h at 2 mA cm
Language	English
Publishing date	2022-11-07
Publishing country	United States
Document type	Journal Article
ISSN	1944-8252
ISSN (online)	1944-8252
DOI	10.1021/acsami.2c16070
Database	MEDical Literature Analysis and Retrieval System OnLINE

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