Article ; Online: Ionic Covalent Organic Frameworks-Derived Cobalt Single Atoms and Nanoparticles for Efficient Oxygen Electrocatalysis.
Small methods
2022 Volume 7, Issue 2, Page(s) e2201371
Abstract: Metal single atoms show outstanding electrocatalytic activity owing to the abundant atomic reactive sites and superior stability. However, the preparation of single atoms suffers from inexorable metal aggregation which is harmful to electrocatalytic ... ...
Abstract | Metal single atoms show outstanding electrocatalytic activity owing to the abundant atomic reactive sites and superior stability. However, the preparation of single atoms suffers from inexorable metal aggregation which is harmful to electrocatalytic activity. Here, ionic covalent organic frameworks (iCOFs) are employed as the sacrificial precursor to mitigate the metal aggregation and subsequent formation of bulky particles. Molecular dynamics simulation shows that iCOFs can trap and confine more Co ions as compared to neutral COFs, resulting in the formation of a catalyst composed of Co single atoms and uniformly distributed Co nanoparticles (Co |
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Language | English |
Publishing date | 2022-12-30 |
Publishing country | Germany |
Document type | Journal Article |
ISSN | 2366-9608 |
ISSN (online) | 2366-9608 |
DOI | 10.1002/smtd.202201371 |
Database | MEDical Literature Analysis and Retrieval System OnLINE |
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