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Article ; Online: Synthesis, Stepwise Bromination, and Functionalization of Picene Diimide.

Wang, Xin / Chen, Li / Li, Nuoya / Wu, Di / Xia, Jianlong

Chemistry (Weinheim an der Bergstrasse, Germany)

2023 Volume 29, Issue 28, Page(s) e202300480

Abstract: Materials Synthesis and Processing Polycyclic aromatic hydrocarbon (PAH) diimides are indispensable candidates for n-type organic semiconductors in organic optoelectronic devices. Developing new PAH diimide building blocks are of remarkable significance ... ...

Abstract	Materials Synthesis and Processing Polycyclic aromatic hydrocarbon (PAH) diimides are indispensable candidates for n-type organic semiconductors in organic optoelectronic devices. Developing new PAH diimide building blocks are of remarkable significance for material diversity and further advance in organic semiconductors. In this contribution, 4,5,8,9-picene diimide (PiDI) was designed and synthesized. Controllable stepwise bromination of PiDI were accomplished to afford 13-monobromo-, 13,14-dibromo-, 2,13,14-tribromo- and 2,11,13,14-tetrabromo-PiDI. Moreover, cyanation of 2,11,13,14-tetrabromo-PiDI gave the corresponding tetracyanated PiDI, which can be utilized as n-type semiconductor with OFET electron mobility up 0.073 cm
Language	English
Publishing date	2023-03-29
Publishing country	Germany
Document type	Journal Article
ZDB-ID	1478547-X
ISSN	1521-3765 ; 0947-6539
ISSN (online)	1521-3765
ISSN	0947-6539
DOI	10.1002/chem.202300480
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Article ; Online: Synthesis and characterization of azulene-based BO-doped heteroaromatics

Zhao, Jingjing / Huang, Huaxi / Li, Nuoya / Wang, Dongxue / Wu, Di / Xia, Jianlong

Tetrahedron. 2023 Sept., v. 144 p.133581-

2023

Abstract: Simultaneously incorporating heteroatoms and nonbenzenoid aromatic hydrocarbons, such as azulene, into polycyclic aromatic hydrocarbons, offers a robust strategy for designing molecules with aesthetic appeal and unique properties. This study presents the ...

Abstract	Simultaneously incorporating heteroatoms and nonbenzenoid aromatic hydrocarbons, such as azulene, into polycyclic aromatic hydrocarbons, offers a robust strategy for designing molecules with aesthetic appeal and unique properties. This study presents the successful synthesis and characterization of a series of azulene-based BO-doped heteroaromatics. Investigation into their optical and electrochemical properties, through UV–vis absorption, cyclic voltammetry, and DFT calculations, reveal their sensitivity to fluoride ions, making them promising candidates for chemosensor applications. Notably, unlike the parent azulene, which is sensitive to acid, these new compounds show negligible changes in absorption and NMR spectra when exposed to excess trifluoroacetic acid. This observation suggests that the introduction of BO unit effectively restrains the protonation of azulene moiety.
Keywords	absorption ; aesthetics ; azulene ; electrochemistry ; fluorides ; moieties ; protonation ; ultraviolet-visible spectroscopy ; voltammetry ; Polycyclic aromatic hydrocarbons (PAHs) ; BO-Doping ; F− sensor
Language	English
Dates of publication	2023-09
Publishing place	Elsevier Ltd
Document type	Article ; Online
ZDB-ID	204285-x
ISSN	1464-5416 ; 0040-4020 ; 0563-2064
ISSN (online)	1464-5416
ISSN	0040-4020 ; 0563-2064
DOI	10.1016/j.tet.2023.133581
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Zs.B 1076: Show issues

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Article ; Online: Enhanced Antipediatric Sarcoma Effect of Everolimus with Secukinumab by Targeting IL17A.

Huang, Dan / Wu, Zhipeng / Wu, Zhengyi / Li, Nuoya / Hao, Liang / Li, Kuangfan / Zeng, Junquan / Qiu, Bingbing / Zhang, Shouhua / Yan, Jinlong

Molecular cancer therapeutics

2024 Volume 23, Issue 5, Page(s) 721–732

Abstract: In this study, we explored the therapeutic potential of everolimus, an mTOR inhibitor, in a patient-derived xenograft (PDX) of rhabdomyosarcoma, the most prevalent malignant pediatric sarcoma. In addition, rhabdoid tumor cell line A-204 and Ewings ... ...

Abstract	In this study, we explored the therapeutic potential of everolimus, an mTOR inhibitor, in a patient-derived xenograft (PDX) of rhabdomyosarcoma, the most prevalent malignant pediatric sarcoma. In addition, rhabdoid tumor cell line A-204 and Ewings sarcoma cell line A-673 were cultured to assess the in vitro effect of everolimus. Furthermore, the cell-derived xenograft (CDX) of A-673 was established and treated with everolimus in vivo. IHC and Western blotting were performed to detect the expressions of pertinent proteins. Results showed that everolimus intervention had limited inhibitory effect on PDX tumor growth compared with cyclophosphamide. Nevertheless, everolimus treatment significantly influenced the phosphorylation levels of S6 kinase beta 1 (S6K1) and eIF4E-binding protein 1 (p-4E-BP1), resulting in the inhibition of angiogenesis in vitro and in vivo. Interestingly, everolimus led to an upregulation in the level of IL17A in sarcoma cells. Notably, when secukinumab, a mAb of IL17A, was combined with everolimus, it synergistically enhanced the inhibitory effect of everolimus on sarcoma cell proliferation in vitro and on the growth of PDX or CDX xenograft tumors in vivo. Importantly, this combination therapy did not affect the mTOR signaling. These results indicate that everolimus exerts an antipediatric sarcoma effect by inhibiting mTOR signal. However, everolimus induces sarcoma cells to produce IL17A, which promotes tumor cell survival and counteracts its antipediatric sarcoma effect. The combination of secukinumab effectively eliminates the effects of IL17A, thereby improving the therapeutic efficacy of everolimus in the context of pediatric sarcomas.
MeSH term(s)	Everolimus/pharmacology ; Humans ; Animals ; Mice ; Antibodies, Monoclonal, Humanized/pharmacology ; Antibodies, Monoclonal, Humanized/therapeutic use ; Xenograft Model Antitumor Assays ; Interleukin-17/metabolism ; Interleukin-17/antagonists & inhibitors ; Cell Proliferation/drug effects ; Cell Line, Tumor ; Rhabdomyosarcoma/drug therapy ; Rhabdomyosarcoma/pathology ; Sarcoma/drug therapy ; Sarcoma/pathology ; Antineoplastic Combined Chemotherapy Protocols/pharmacology ; Antineoplastic Combined Chemotherapy Protocols/therapeutic use ; Drug Synergism
Chemical Substances	Everolimus (9HW64Q8G6G) ; Antibodies, Monoclonal, Humanized ; Interleukin-17 ; secukinumab (DLG4EML025) ; IL17A protein, human
Language	English
Publishing date	2024-01-31
Publishing country	United States
Document type	Journal Article ; Research Support, Non-U.S. Gov't
ZDB-ID	2063563-1
ISSN	1538-8514 ; 1535-7163
ISSN (online)	1538-8514
ISSN	1535-7163
DOI	10.1158/1535-7163.MCT-23-0342
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Zs.A 5750: Show issues

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Article ; Online: hsa-miR-34a-5p Ameliorates Hepatic Ischemia/Reperfusion Injury Via Targeting HNF4α.

Zheng, Xiaoqiang / Wang, Gang / Yuan, Jiang / Li, Nuoya / Yan, Biaolei / Yan, Jinlong / Sheng, Yanling

The Turkish journal of gastroenterology : the official journal of Turkish Society of Gastroenterology

2022 Volume 33, Issue 7, Page(s) 596–605

Abstract: Background: To investigate the relationship between the expression level of hsa-miR-34a-5p and liver injury and to further explore its regulatory signaling pathways Methods: Liver tissue and blood were collected from 60 patients undergoing hepatectomy. ... ...

Abstract	Background: To investigate the relationship between the expression level of hsa-miR-34a-5p and liver injury and to further explore its regulatory signaling pathways Methods: Liver tissue and blood were collected from 60 patients undergoing hepatectomy. We constructed a rat HIRI model and treated it with an intraperitoneal injection of agomir-miR-34a-5p or agomir-normal control (NC) for 7 days after the surgery. The pathological changes of agomir-miR-34a-5p or agomir-normal control (NC) groups were compared. 7702 and AML12 cells were transfected with mimics NC or miR-34a-5p mimics and then treated with H2O2 for 6 hours. Cell apoptosis was detected by flow cytometry, Western blot, and terminal deoxynucleotidyl transferase-mediated dUTP nick-end labeling, respectively. Furthermore, the target genes of miR- 34a-5p were identified by luciferase reporter gene assay and were verified in vitro. Results: The relatively high miR-34a-5p expression group revealed a lower level of alanine aminotransferase and aspartate aminotrans- ferase compared with the relatively low miR-34a-5p expression group. HIRI+agomir-miR-34a-5p rats exhibited significantly higher miR-34a-5p expression, lower serum alanine aminotransferase, aspartate aminotransferase, alleviated hepatic necrosis, reduced hepa- tocyte apoptosis, and decreased expression of apoptosis-related proteins, when compared with HIRI+agomir-NC rats (P < .05). After hydrogen peroxide treatment, alpha mouse liver-12 cell (AML-12) and normal liver cell line LO2 (LO2) cells transfected with miR-34a-5p mimics had significantly lower apoptosis rate compared with miR-34a-5p mimics NC group (P < .05). Hepatocyte nuclear factor 4α was identified as a miR-34a-5p target gene. Hepatocyte nuclear factor 4α expression was significantly downregulated in AML12 and HL-7702 (7702) cells transfected with miR-34a-5p (P < .05). Moreover, AML12 and 7702 cells transfected with miR-34a-5p signifi- cantly showed higher c-Jun N-terminal kinase (JNK), P38, cleavage cas-3, and BCL2 associated X (Bax) protein levels compared with AML12 and 7702 cells transfected with agomir-NC. Conclusion: miR-34a-5p possibly protected the liver from I/R injury through downregulating Hepatocyte nuclear factor 4α to inhibit the JNK/P38 signaling pathway.
MeSH term(s)	Animals ; Apoptosis/genetics ; Hepatocyte Nuclear Factor 4 ; Hepatocyte Nuclear Factors/metabolism ; Hydrogen Peroxide/metabolism ; Ischemia/metabolism ; Ischemia/pathology ; Liver/pathology ; Mice ; MicroRNAs/genetics ; MicroRNAs/metabolism ; Rats ; Rats, Sprague-Dawley ; Reperfusion Injury/genetics ; Reperfusion Injury/prevention & control
Chemical Substances	Hepatocyte Nuclear Factor 4 ; Hepatocyte Nuclear Factors ; Hnf4a protein, mouse ; Hnf4a protein, rat ; MIRN34a microRNA, mouse ; MIRN34a microRNA, rat ; MicroRNAs ; Hydrogen Peroxide (BBX060AN9V)
Language	English
Publishing date	2022-07-25
Publishing country	Turkey
Document type	Journal Article
ZDB-ID	1340275-4
ISSN	2148-5607 ; 1300-4948
ISSN (online)	2148-5607
ISSN	1300-4948
DOI	10.5152/tjg.2022.21169
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Zs.A 4524: Show issues

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Article ; Online: USP1 Promotes GC Metastasis via Stabilizing ID2.

Li, Nuoya / Wu, Lei / Zuo, Xingye / Luo, Huilong / Sheng, Yanling / Yan, Jinlong

Disease markers

2021 Volume 2021, Page(s) 3771990

Abstract: Gastric cancer (GC) is one of the most common malignant tumors all over the world. And recurrence and metastasis are still the main causes of low survival rate for advanced GC. USP1 has been shown overexpressed in multiple cancers, which indicate its ... ...

Abstract	Gastric cancer (GC) is one of the most common malignant tumors all over the world. And recurrence and metastasis are still the main causes of low survival rate for advanced GC. USP1 has been shown overexpressed in multiple cancers, which indicate its important biomarker in tumorigenesis and development. Our study is aimed at defining the exact role of USP1 on GC metastasis and the underlying mechanism. USP1 was firstly found overexpressed in GC tissues and relatively high-expression levels conferred poor survival rates. Then, real-time cellular analysis (RTCA) showed that USP1 knockdown inhibited GC metastasis both in vitro and in vivo. Mechanically, we demonstrated that USP1 promoted GC metastasis via upregulating ID2 expression and further confirmed that USP1 stabilized ID2 expression through deubiquitinating ID2 in GC. In conclusion, our study showed that USP1 promoted GC metastasis via stabilizing ID2 expression, which provides a potential biomarker and therapy target for GC.
MeSH term(s)	Cell Line, Tumor ; Gene Expression Regulation, Neoplastic ; Gene Knockdown Techniques ; Humans ; Inhibitor of Differentiation Protein 2/metabolism ; Neoplasm Metastasis/physiopathology ; Stomach Neoplasms/pathology ; Survival Analysis ; Ubiquitin-Specific Proteases/genetics ; Ubiquitin-Specific Proteases/metabolism ; Ubiquitin-Specific Proteases/physiology ; Ubiquitination ; Up-Regulation/physiology
Chemical Substances	ID2 protein, human ; Inhibitor of Differentiation Protein 2 ; USP1 protein, human (EC 3.4.19.12) ; Ubiquitin-Specific Proteases (EC 3.4.19.12)
Language	English
Publishing date	2021-11-27
Publishing country	United States
Document type	Journal Article
ZDB-ID	604951-5
ISSN	1875-8630 ; 0278-0240
ISSN (online)	1875-8630
ISSN	0278-0240
DOI	10.1155/2021/3771990
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Zs.A 1856: Show issues			Location: Je nach Verfügbarkeit (siehe Angabe bei Bestand) bis Jg. 1994: Bestellungen von Artikeln über das Online-Bestellformular Jg. 1995 - 2021: Lesesall (1.OG) ab Jg. 2022: Lesesaal (EG)
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Article: Direct Z-Scheme 0D/2D Heterojunction of CsPbBr₃ Quantum Dots/Bi₂WO₆ Nanosheets for Efficient Photocatalytic CO₂ Reduction

Wang, Jichong / Wang, Jin / Li, Nuoya / Du, Xinyi / Ma, Jun / He, Chaohua / Li, Zhengquan

ACS applied materials & interfaces. 2020 June 22, v. 12, no. 28

2020

Abstract: Photocatalytic CO₂ reduction is an appealing approach to convert solar energy into high value-added chemicals. All-inorganic CsPbBr₃ quantum dots (QDs) have emerged as a promising photocatalyst for reducing CO₂. However, pristine CsPbBr₃ has a low ... ...

Abstract	Photocatalytic CO₂ reduction is an appealing approach to convert solar energy into high value-added chemicals. All-inorganic CsPbBr₃ quantum dots (QDs) have emerged as a promising photocatalyst for reducing CO₂. However, pristine CsPbBr₃ has a low catalytic performance, mainly due to severe charge recombination. Herein, a 0D/2D heterojunction of CsPbBr₃ QDs/Bi₂WO₆ nanosheet (CPB/BWO) photocatalysts is fabricated for photocatalytic CO₂ reduction. The CPB/BWO photocatalyst achieves excellent photocatalytic performance: the total yield of CH₄/CO is 503 μmol g–¹, nearly 9.5 times higher than the pristine CsPbBr₃. The CPB/BWO heterojunction also exhibits much-improved stability during photocatalytic reactions. On the basis of various characterization techniques, our investigations verified a direct Z-scheme charge migration mechanism between CsPbBr₃ QDs and Bi₂WO₆ nanosheets. The improved photocatalytic performance is originated from the high spatial separation of photoexcited charge carriers in CPB/BWO, which can also preserve strong individual redox abilities of two components. This work reports an efficient direct Z-scheme heterojunction photocatalytic system based on metal halide perovskites. The novel strategy we proposed may bring up new opportunities for the development of metal halide perovskite photocatalysts with greatly enhanced activities.
Keywords	carbon dioxide ; carbon monoxide ; methane ; nanosheets ; photocatalysis ; photocatalysts ; quantum dots ; solar energy ; value added
Language	English
Dates of publication	2020-0622
Size	p. 31477-31485.
Publishing place	American Chemical Society
Document type	Article
ISSN	1944-8252
DOI	10.1021/acsami.0c08152
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Article ; Online: ZnSe Nanorods-CsSnCl

Li, Nuoya / Chen, Xujian / Wang, Jin / Liang, Xinmeng / Ma, Lintao / Jing, Xiaolang / Chen, De-Li / Li, Zhengquan

ACS nano

2022 Volume 16, Issue 2, Page(s) 3332–3340

Abstract: Utilizing sunlight to convert ... ...

Abstract	Utilizing sunlight to convert CO
Language	English
Publishing date	2022-02-04
Publishing country	United States
Document type	Journal Article
ISSN	1936-086X
ISSN (online)	1936-086X
DOI	10.1021/acsnano.1c11442
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Article ; Online: Development and Validation of a Differential Diagnosis Model for Acute Appendicitis and Henoch-Schonlein Purpura in Children.

Zhan, Yishan / Wu, Min / Li, Kehao / Chen, Qiang / Li, Nuoya / Zheng, Weiming / Zhu, Yourong / Peng, Xiaojie / Zhang, Shouhua / Tao, Qiang

Pediatric allergy, immunology, and pulmonology

2022 Volume 35, Issue 2, Page(s) 86–94

Abstract: Objective: ...

Abstract	Objective:
MeSH term(s)	Appendicitis/diagnosis ; C-Reactive Protein/analysis ; C-Reactive Protein/metabolism ; Child ; Diagnosis, Differential ; Humans ; IgA Vasculitis/diagnosis ; Retrospective Studies
Chemical Substances	C-Reactive Protein (9007-41-4)
Language	English
Publishing date	2022-06-20
Publishing country	United States
Document type	Journal Article ; Research Support, Non-U.S. Gov't
ZDB-ID	2566338-0
ISSN	2151-3228 ; 2151-321X
ISSN (online)	2151-3228
ISSN	2151-321X
DOI	10.1089/ped.2021.0218
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Zs.B 3041: Show issues

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Article ; Online: Direct Z-Scheme 0D/2D Heterojunction of CsPbBr

Wang, Jichong / Wang, Jin / Li, Nuoya / Du, Xinyi / Ma, Jun / He, Chaohua / Li, Zhengquan

ACS applied materials & interfaces

2020 Volume 12, Issue 28, Page(s) 31477–31485

Abstract: Photocatalytic ... ...

Abstract	Photocatalytic CO
Language	English
Publishing date	2020-07-04
Publishing country	United States
Document type	Journal Article
ISSN	1944-8252
ISSN (online)	1944-8252
DOI	10.1021/acsami.0c08152
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Article ; Online: Air pollution weaken your muscle? Evidence from a cross-sectional study on sarcopenia in central China.

Zhang, Faxue / Li, Tianzhou / Chen, Bingbing / Li, Nuoya / Zhang, Xupeng / Zhu, Shijie / Zhao, Gaichan / Zhang, Xiaowei / Ma, TingTing / Zhou, Fang / Liu, Hao / Zhu, Wei

Ecotoxicology and environmental safety

2023 Volume 258, Page(s) 114962

Abstract: Background: As the world experiences a demographic shift towards aging populations, there will be a significant surge in the number of sarcopenia patients, along with an unprecedented expansion in the associated economic burden. The multitudinous risk ... ...

Abstract	Background: As the world experiences a demographic shift towards aging populations, there will be a significant surge in the number of sarcopenia patients, along with an unprecedented expansion in the associated economic burden. The multitudinous risk factors for sarcopenia have been reported, but evidence for air pollution remains rare. Methods: This cross-sectional study employed multi-stage random sampling to select 1592 participants over 40 years of age from Hubei Province. Daily mean concentrations of air pollutants were collected ChinaHighAirPollutants dataset. Unconditional logistic regression models were utilized to investigate the associations between air pollution and sarcopenia. Results: For each 1 μg/m Conclusions: Our results produced evidence for a relationship between air pollution exposure and the increased prevalence of sarcopenia in China. Public health and relevant departments should make efforts to prevent sarcopenia, particularly in China experiencing rapid demographic aging.
MeSH term(s)	Female ; Humans ; Adult ; Middle Aged ; Cross-Sectional Studies ; Sarcopenia/etiology ; Sarcopenia/chemically induced ; Air Pollution/adverse effects ; Air Pollution/analysis ; Air Pollutants/adverse effects ; Air Pollutants/analysis ; China/epidemiology ; Particulate Matter/adverse effects ; Particulate Matter/analysis ; Muscles/chemistry ; Environmental Exposure/adverse effects ; Environmental Exposure/analysis ; Nitrogen Dioxide/analysis
Chemical Substances	Air Pollutants ; Particulate Matter ; Nitrogen Dioxide (S7G510RUBH)
Language	English
Publishing date	2023-04-28
Publishing country	Netherlands
Document type	Journal Article
ZDB-ID	436536-7
ISSN	1090-2414 ; 0147-6513
ISSN (online)	1090-2414
ISSN	0147-6513
DOI	10.1016/j.ecoenv.2023.114962
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