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Article: Hierarchical Nanoheterostructure of HFIP-Grafted α-Fe

Wang, Xuechun / Liu, Jingyuan / Li, Rumin / Yu, Jing / Liu, Qi / Zhu, Jiahui / Liu, Peili

2024 Volume 14, Issue 3

Abstract: New and efficient sensors of nerve agents are urgently demanded to prevent them from causing mass casualties in war or terrorist attacks. So, in this work, a novel hierarchical nanoheterostructure was synthesized via the direct growth of α- ... ...

Abstract	New and efficient sensors of nerve agents are urgently demanded to prevent them from causing mass casualties in war or terrorist attacks. So, in this work, a novel hierarchical nanoheterostructure was synthesized via the direct growth of α-Fe
Language	English
Publishing date	2024-02-02
Publishing country	Switzerland
Document type	Journal Article
ZDB-ID	2662255-5
ISSN	2079-4991
ISSN	2079-4991
DOI	10.3390/nano14030305
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Article ; Online: Co Single Atoms Anchored in N and P Co-doped Porous Carbon Fibers for Efficient Water Splitting.

Li, Jie / Zhu, Jiahui / Jia, Ziqi / Li, Rumin / Yu, Jing

Chemistry, an Asian journal

2023 Volume 18, Issue 15, Page(s) e202300393

Abstract: Single atom catalysts (SACs) show potential application for highly efficient water splitting. Herein, we designed Co single atoms (SAs) dispersed on N and P co-doped porous carbon nanofibers as electrocatalysts for hydrogen evolution reaction (HER) and ... ...

Abstract	Single atom catalysts (SACs) show potential application for highly efficient water splitting. Herein, we designed Co single atoms (SAs) dispersed on N and P co-doped porous carbon nanofibers as electrocatalysts for hydrogen evolution reaction (HER) and oxygen evolution reaction (OER). The configuration of Co SAs is proved to coordinate with 4 N/O atoms. The long-range interactions between doped P atoms and Co-N
Language	English
Publishing date	2023-07-07
Publishing country	Germany
Document type	Journal Article
ZDB-ID	2233006-9
ISSN	1861-471X ; 1861-4728
ISSN (online)	1861-471X
ISSN	1861-4728
DOI	10.1002/asia.202300393
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Article ; Online: Three-Step Depletion Strategy of Glutathione: Tunable Metal-Organic-Framework-Engineered Nanozymes for Driving Oxidative/Nitrative Stress to Maximize Ferroptosis Therapy.

Li, Wenting / Liu, Shikai / Ding, He / Zhao, Ruoxi / Zang, Pengyu / Li, Siyi / Fang, Linyang / Li, Rumin / Zhang, Manjie / Yang, Piaoping

Nano letters

2024 Volume 24, Issue 6, Page(s) 2071–2080

Abstract: Ferroptosis is a novel type of nonapoptotic programmed cell death involving the accumulation of lipid peroxidation (LPO) to a lethal threshold. Herein, we propose tunable zeolitic imidazolate framework (ZIFs)-engineered biodegradable nanozymes for ... ...

Abstract	Ferroptosis is a novel type of nonapoptotic programmed cell death involving the accumulation of lipid peroxidation (LPO) to a lethal threshold. Herein, we propose tunable zeolitic imidazolate framework (ZIFs)-engineered biodegradable nanozymes for ferroptosis mediated by both reactive oxygen species (ROS) and nitrogen species (RNS). l-Arginine is utilized as an exogenous nitric oxide donor and loaded into hollow ZIFs@MnO
MeSH term(s)	Reactive Oxygen Species ; Metal-Organic Frameworks ; Ferroptosis ; Manganese Compounds/pharmacology ; Oxides ; Oxidative Stress ; Glutathione
Chemical Substances	Reactive Oxygen Species ; Metal-Organic Frameworks ; Manganese Compounds ; Oxides ; Glutathione (GAN16C9B8O)
Language	English
Publishing date	2024-02-02
Publishing country	United States
Document type	Journal Article
ISSN	1530-6992
ISSN (online)	1530-6992
DOI	10.1021/acs.nanolett.3c04813
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Article ; Online: Dual-inhibition of lactate metabolism and Prussian blue-mediated radical generation for enhanced chemodynamic therapy and antimetastatic effect.

Li, Wenting / Liu, Shikai / Zhang, Yangyang / Zhou, Jialing / Li, Rumin / Gai, Shili / Zhong, Lei / Yang, Piaoping

Nanoscale

2023 Volume 15, Issue 20, Page(s) 9214–9228

Abstract: Numerous research studies have proved that lactate is pivotal in tumor proliferation, metastasis, and recurrence, so disrupting the lactate metabolism in the tumor microenvironment (TME) has become one of the effective methods of tumor treatment. Herein, ...

Abstract	Numerous research studies have proved that lactate is pivotal in tumor proliferation, metastasis, and recurrence, so disrupting the lactate metabolism in the tumor microenvironment (TME) has become one of the effective methods of tumor treatment. Herein, we have developed a versatile nanoparticle (HCLP NP) based on hollow Prussian blue (HPB) as the functional carrier for loading α-cyano-4-hydroxycinnamate (CHC), and lactate oxidase (LOD), followed by coating with polyethylene glycol to enhance chemodynamic therapy (CDT) and the antimetastatic effect of cancer. The obtained HCLP NPs would be degraded under endogenous mild acidity within the TME to simultaneously release CHC and LOD. CHC inhibits the expression of monocarboxylate transporter 1 in tumors, thereby interrupting the uptake of lactate from the outside and alleviating tumor hypoxia by reducing lactate aerobic respiration. Meanwhile, the released LOD can catalyze the decomposition of lactate into hydrogen peroxide, further enhancing the efficacy of CDT by generating plenty of toxic reactive oxygen species through the Fenton reaction. The strong absorbance at about 800 nm endows HCLP NPs with excellent photoacoustic imaging properties. Both
MeSH term(s)	Humans ; Biological Transport ; Ferrocyanides/pharmacology ; Cell Respiration ; Lactic Acid ; Hydrogen Peroxide ; Tumor Microenvironment ; Neoplasms ; Cell Line, Tumor ; Nanoparticles
Chemical Substances	ferric ferrocyanide (TLE294X33A) ; Ferrocyanides ; Lactic Acid (33X04XA5AT) ; Hydrogen Peroxide (BBX060AN9V)
Language	English
Publishing date	2023-05-25
Publishing country	England
Document type	Journal Article
ZDB-ID	2515664-0
ISSN	2040-3372 ; 2040-3364
ISSN (online)	2040-3372
ISSN	2040-3364
DOI	10.1039/d3nr01052j
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Article ; Online: Surface hydrolysis-anchored eugenol self-polishing marine antifouling coating.

Sha, Jianang / Liu, Xin / Chen, Rongrong / Yu, Jing / Liu, Qi / Liu, Jingyuan / Zhu, Jiahui / Liu, Peili / Li, Rumin / Wang, Jun

Journal of colloid and interface science

2023 Volume 637, Page(s) 67–75

Abstract: Traditional self-polishing antifouling coatings kill surface organisms by releasing toxic substances, which are damaging to the ecosystem. As a natural antimicrobial substance, eugenol is environmentally friendly and has been proven by different research ...

Abstract	Traditional self-polishing antifouling coatings kill surface organisms by releasing toxic substances, which are damaging to the ecosystem. As a natural antimicrobial substance, eugenol is environmentally friendly and has been proven by different research teams to be effective in enhancing the anti-fouling effect of coatings in the real sea. While in these previous research works, the eugenol was released directly into the seawater thus cannot further serve as surface antifouling effect, leading to a limited antifouling effect of the coating. In this work, the quaternary ammonium component was introduced into the butyl ester-based resin - poly (eugenol methacrylate - acryloyloxyethyltrimethyl ammonium chloride - hexafluorobutyl methacrylate - methyl methacrylate - butyl methacrylate - ethylene glycol methyl ether acrylate) (EMQFP) coating for the first time by simple one-step free radical polymerization method. On the one hand, the eugenol produced by hydrolysis is anchored to the quaternary ammonium on the coating surface for a period of time due to the cationic-π interaction, instead of being released into seawater immediately after hydrolysis, thus increasing the utilization rate of eugenol; on the other hand, the negatively charged carboxylate groups generated after hydrolysis in the coating are mutually attracted to quaternary ammonium through electrostatic effect, so the resin chain segment conformation on the coating surface adjusted to produce zwitterionic-like structure, and the hydration of zwitterionic inhibits primary fouling adhesion.
Language	English
Publishing date	2023-01-14
Publishing country	United States
Document type	Journal Article
ZDB-ID	241597-5
ISSN	1095-7103 ; 0021-9797
ISSN (online)	1095-7103
ISSN	0021-9797
DOI	10.1016/j.jcis.2023.01.058
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Article ; Online: Fe-MMT/WO

Liu, Ning / Yu, Jing / Zhang, Hongsen / Zhu, Jiahui / Liu, Qi / Chen, Rongrong / Li, Ying / Li, Rumin / Wang, Jun

Chemosphere

2023 Volume 344, Page(s) 140321

Abstract: The preparation of Fe-MMT/ ... ...

Abstract	The preparation of Fe-MMT/WO
MeSH term(s)	Uranium ; Iron ; Catalysis ; Light ; Electron Transport
Chemical Substances	Uranium (4OC371KSTK) ; Iron (E1UOL152H7)
Language	English
Publishing date	2023-10-01
Publishing country	England
Document type	Journal Article
ZDB-ID	120089-6
ISSN	1879-1298 ; 0045-6535 ; 0366-7111
ISSN (online)	1879-1298
ISSN	0045-6535 ; 0366-7111
DOI	10.1016/j.chemosphere.2023.140321
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Article: Mussel-inspired polydopamine microspheres self-adhered on natural hemp fibers for marine uranium harvesting and photothermal-enhanced antifouling properties

Gu, Huiquan / Liu, Qi / Zhu, Jiahui / Sun, Gaohui / Liu, Jingyuan / Yu, Jing / Li, Rumin / Li, Ying / Wang, Jun

Journal of colloid and interface science. 2022 Apr. 10,

2022

Abstract: The rapid development of nuclear energy and the accelerated consumption of uranium (U(VI)) ores have forced researchers to turn to marine U(VI) harvesting. However, the performance of marine U(VI) harvesting materials was challenged by the combination of ...

Abstract	The rapid development of nuclear energy and the accelerated consumption of uranium (U(VI)) ores have forced researchers to turn to marine U(VI) harvesting. However, the performance of marine U(VI) harvesting materials was challenged by the combination of ultralow concentrations of U(VI), high concentrations of various interfering ions and biofouling from abundant marine living organisms. Natural abundant hemp fibers (HFs) were adhered by mussel-inspired polydopamine microspheres (HFMPDA) during self-polymerization. Both HFs and PDA are derived from natural products with low-cost and eco-friendly properties to guarantee compatibility with biological marine environments. HFMPDA exhibits an outstanding distribution coefficient of 10.51 ± 0.51 L·g⁻¹ for U(VI) and great fouling resistance. The coordination forms between the U(VI) ion and HFMPDA were investigated by density functional theory (DFT), and the antifouling property was simulated by molecular dynamics (MD) calculations. The adsorption capacity of HFMPDA is 128.43 ± 3.26 μg·g⁻¹, which is 1.75 and 6.05 times higher than that of HFPDA (only covered by PDA) and V(V), respectively, after immersion for 34 days in the Yellow Sea, China. These polydopamine microspheres adhered to HF will be a photothermal marine U(VI) harvesting material with enhanced selectivity and fouling resistance.
Keywords	adsorption ; antifouling activities ; biofouling ; density functional theory ; hemp ; microparticles ; molecular dynamics ; nuclear power ; uranium ; China ; Yellow Sea
Language	English
Dates of publication	2022-0410
Publishing place	Elsevier Inc.
Document type	Article
Note	Pre-press version
ZDB-ID	241597-5
ISSN	1095-7103 ; 0021-9797
ISSN (online)	1095-7103
ISSN	0021-9797
DOI	10.1016/j.jcis.2022.04.065
Database	NAL-Catalogue (AGRICOLA)

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Article: A high-flux antibacterial poly(amidoxime)-polyacrylonitrile blend membrane for highly efficient uranium extraction from seawater

Yu, Jiaqi / Zhang, Hongsen / Liu, Qi / Zhu, Jiahui / Yu, Jing / Sun, Gaohui / Li, Rumin / Wang, Jun

Journal of hazardous materials. 2022 Oct. 15, v. 440

2022

Abstract: Uranium is an important fuel for nuclear power, with 4.5 billion tons of it stored in the oceans, 1,000 times more than on land. Polymer membrane materials are widely used in the marine resources fields, due to their convenient collection, good ... ...

Abstract	Uranium is an important fuel for nuclear power, with 4.5 billion tons of it stored in the oceans, 1,000 times more than on land. Polymer membrane materials are widely used in the marine resources fields, due to their convenient collection, good separation and can work continuously. Herein, a poly(amidoxime)-polyacrylonitrile blend membrane (PCP) with high flux, excellent antibacterial properties and uranium adsorption performance has been prepared by using the phase inversion method, and the prepared membrane was used for highly efficient uranium extraction from seawater. In static adsorption experiments, the PCP membrane reached adsorption equilibrium after 48 h, and the adsorption capacity was 303.89 mg/g (C₀ =50 mg/L). In dynamic adsorption experiments, it was found that the lower flow rate and higher number of membrane layers were favorable for dynamic adsorption. In addition, the water flux of the PCP membrane was 7.4 times higher than that of the PAN membrane. The adsorption mechanism can be attributed to the chelation between amino and hydroxyl groups in CS, amidoxime group in poly(amidoxime) and uranyl ions. The simple preparation process coupled with the excellent adsorption performance indicated that the PCP membrane would be a promising material for the uranium extraction from seawater.
Keywords	adsorption ; chelation ; nuclear power ; polymers ; seawater ; uranium ; uranyl ions
Language	English
Dates of publication	2022-1015
Publishing place	Elsevier B.V.
Document type	Article
ZDB-ID	1491302-1
ISSN	1873-3336 ; 0304-3894
ISSN (online)	1873-3336
ISSN	0304-3894
DOI	10.1016/j.jhazmat.2022.129735
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Article ; Online: MOF-derived electrochemical catalyst Cu-N/C for the enhancement of amperometric oxygen detection.

Yin, Wenyan / Zhang, Milin / Liu, Jingyuan / Alali, Khaled Tawfik / Yu, Jing / Zhu, Jiahui / Liu, Peili / Li, Rumin / Wang, Jun

Nanoscale

2022 Volume 14, Issue 5, Page(s) 1796–1806

Abstract: Electrochemical sensors using ionic liquids as electrolytes for oxygen detection are now getting more and more attention. Recently, an ionic liquid combined with an electrochemically active catalyst system has become popular for boosting the sensing ... ...

Abstract	Electrochemical sensors using ionic liquids as electrolytes for oxygen detection are now getting more and more attention. Recently, an ionic liquid combined with an electrochemically active catalyst system has become popular for boosting the sensing performance of oxygen sensors. In this work, the imidazolyl-based ionic liquid 1-butyl-2,3-dimethylimidazole bis((trifluoromethyl)sulfonyl)imide [Bmmim][TFSI] is first prepared by a facile two-step method. Subsequently, a transition metal and N-codoped porous carbon oxygen reduction electrochemical catalyst Cu-N/C is synthesized by calcining the Cu-doped ZIF-8 precursor and then blending it in different ratios with the ionic liquid [Bmmim][TFSI] as composite electrolytes for oxygen detection. The composite electrolyte Cu-N/C/[Bmmim][TFSI] exhibits increased responses in cyclic voltammetry (CV) and chronoamperometry (CA) relative to that of the pure ionic liquid. Furthermore, the CV and CA data show that 6% Cu-N/C/[Bmmim][TFSI] has the optimum oxygen sensing response with an enhanced reduction peak current, a sensitivity of 0.1678 μA/[% O
Language	English
Publishing date	2022-02-03
Publishing country	England
Document type	Journal Article
ZDB-ID	2515664-0
ISSN	2040-3372 ; 2040-3364
ISSN (online)	2040-3372
ISSN	2040-3364
DOI	10.1039/d1nr06758c
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Article ; Online: Theory-Guided Design of a Method to Obtain Competitive Balance between U(VI) Adsorption and Swaying Zwitterion-Induced Fouling Resistance on Natural Hemp Fibers.

Gu, Huiquan / Yu, Jing / Zhang, Hongsen / Sun, Gaohui / Li, Rumin / Liu, Peili / Li, Ying / Wang, Jun

International journal of molecular sciences

2022 Volume 23, Issue 12

Abstract: The competitive balance between uranium (VI) (U(VI)) adsorption and fouling resistance is of great significance in guaranteeing the full potential of U(VI) adsorbents in seawater, and it is faced with insufficient research. To fill the gap in this field, ...

Abstract	The competitive balance between uranium (VI) (U(VI)) adsorption and fouling resistance is of great significance in guaranteeing the full potential of U(VI) adsorbents in seawater, and it is faced with insufficient research. To fill the gap in this field, a molecular dynamics (MD) simulation was employed to explore the influence and to guide the design of mass-produced natural hemp fibers (HFs). Sulfobetaine (SB)- and carboxybetaine (CB)-type zwitterions containing soft side chains were constructed beside amidoxime (AO) groups on HFs (HFAS and HFAC) to form a hydration layer based on the terminal hydrophilic groups. The soft side chains were swayed by waves to form a hydration-layer area with fouling resistance and to simultaneously expel water molecules surrounding the AO groups. HFAS exhibited greater antifouling properties than that of HFAO and HFAC. The U(VI) adsorption capacity of HFAS was almost 10 times higher than that of HFAO, and the max mass rate of U:V was 4.3 after 35 days of immersion in marine water. This paper offers a theory-guided design of a method to the competitive balance between zwitterion-induced fouling resistance and seawater U(VI) adsorption on natural materials.
MeSH term(s)	Adsorption ; Cannabis ; Hydrophobic and Hydrophilic Interactions ; Uranium/chemistry ; Water/chemistry
Chemical Substances	Water (059QF0KO0R) ; Uranium (4OC371KSTK)
Language	English
Publishing date	2022-06-10
Publishing country	Switzerland
Document type	Journal Article
ZDB-ID	2019364-6
ISSN	1422-0067 ; 1422-0067 ; 1661-6596
ISSN (online)	1422-0067
ISSN	1422-0067 ; 1661-6596
DOI	10.3390/ijms23126517
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