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  1. Article ; Online: Advancing electrocatalytic nitrogen fixation: insights from molecular systems.

    Peters, Jonas C

    Faraday discussions

    2023  Volume 243, Page(s) 450–472

    Abstract: Nitrogen fixation has a rich history within the inorganic chemistry community. In recent years attention has (re)focused on developing electrocatalytic systems capable of mediating the nitrogen reduction reaction ( ... ...

    Abstract Nitrogen fixation has a rich history within the inorganic chemistry community. In recent years attention has (re)focused on developing electrocatalytic systems capable of mediating the nitrogen reduction reaction (N
    Language English
    Publishing date 2023-07-19
    Publishing country England
    Document type Journal Article
    ISSN 1364-5498
    ISSN (online) 1364-5498
    DOI 10.1039/d3fd00017f
    Database MEDical Literature Analysis and Retrieval System OnLINE

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  2. Article ; Online: Catalytic Reduction of Cyanide to Ammonia and Methane at a Mononuclear Fe Site.

    Johansen, Christian M / Peters, Jonas C

    Journal of the American Chemical Society

    2024  Volume 146, Issue 8, Page(s) 5343–5354

    Abstract: Nitrogenase enzymes catalyze nitrogen reduction ( ... ...

    Abstract Nitrogenase enzymes catalyze nitrogen reduction (N
    Language English
    Publishing date 2024-02-15
    Publishing country United States
    Document type Journal Article
    ZDB-ID 3155-0
    ISSN 1520-5126 ; 0002-7863
    ISSN (online) 1520-5126
    ISSN 0002-7863
    DOI 10.1021/jacs.3c12395
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  3. Article ; Online: Highly Selective Fe-Catalyzed Nitrogen Fixation to Hydrazine Enabled by Sm(II) Reagents with Tailored Redox Potential and p

    Boyd, Emily A / Peters, Jonas C

    Journal of the American Chemical Society

    2023  Volume 145, Issue 27, Page(s) 14784–14792

    Abstract: Controlling product selectivity in multiproton, multielectron reductions of unsaturated small molecules is of fundamental interest in catalysis. For the ... ...

    Abstract Controlling product selectivity in multiproton, multielectron reductions of unsaturated small molecules is of fundamental interest in catalysis. For the N
    Language English
    Publishing date 2023-06-27
    Publishing country United States
    Document type Journal Article
    ZDB-ID 3155-0
    ISSN 1520-5126 ; 0002-7863
    ISSN (online) 1520-5126
    ISSN 0002-7863
    DOI 10.1021/jacs.3c03352
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  4. Article ; Online: Sm(II)-Mediated Proton-Coupled Electron Transfer: Quantifying Very Weak N-H and O-H Homolytic Bond Strengths and Factors Controlling Them.

    Boyd, Emily A / Peters, Jonas C

    Journal of the American Chemical Society

    2022  Volume 144, Issue 46, Page(s) 21337–21346

    Abstract: Coordination of alcohols to the single-electron reductant samarium diiodide ( ... ...

    Abstract Coordination of alcohols to the single-electron reductant samarium diiodide (SmI
    MeSH term(s) Protons ; Electrons ; Oxidation-Reduction ; Electron Transport
    Chemical Substances Protons ; samarium diiodide (L15T8U41LC)
    Language English
    Publishing date 2022-11-08
    Publishing country United States
    Document type Journal Article ; Research Support, U.S. Gov't, Non-P.H.S. ; Research Support, Non-U.S. Gov't ; Research Support, N.I.H., Extramural
    ZDB-ID 3155-0
    ISSN 1520-5126 ; 0002-7863
    ISSN (online) 1520-5126
    ISSN 0002-7863
    DOI 10.1021/jacs.2c09580
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  5. Article ; Online: Light Alters the NH

    Garrido-Barros, Pablo / Chalkley, Matthew J / Peters, Jonas C

    Angewandte Chemie (International ed. in English)

    2023  Volume 62, Issue 9, Page(s) e202216693

    Abstract: Whereas synthetically catalyzed nitrogen reduction ( ... ...

    Abstract Whereas synthetically catalyzed nitrogen reduction (N
    Language English
    Publishing date 2023-01-24
    Publishing country Germany
    Document type Journal Article
    ZDB-ID 2011836-3
    ISSN 1521-3773 ; 1433-7851
    ISSN (online) 1521-3773
    ISSN 1433-7851
    DOI 10.1002/anie.202216693
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  6. Article ; Online: Enhanced Ammonia Oxidation Catalysis by a Low-Spin Iron Complex Featuring

    Zott, Michael D / Peters, Jonas C

    Journal of the American Chemical Society

    2021  Volume 143, Issue 20, Page(s) 7612–7616

    Abstract: The goal of using ammonia as a solar fuel motivates the development of selective ammonia oxidation (AO) catalysts for fuel cell applications. Herein, we describe Fe-mediated AO electrocatalysis with [( ... ...

    Abstract The goal of using ammonia as a solar fuel motivates the development of selective ammonia oxidation (AO) catalysts for fuel cell applications. Herein, we describe Fe-mediated AO electrocatalysis with [(bpyPy
    MeSH term(s) Ammonia/chemistry ; Catalysis ; Ferrous Compounds/chemistry ; Molecular Conformation ; Oxidation-Reduction ; Stereoisomerism
    Chemical Substances Ferrous Compounds ; Ammonia (7664-41-7)
    Language English
    Publishing date 2021-05-17
    Publishing country United States
    Document type Journal Article ; Research Support, N.I.H., Extramural ; Research Support, Non-U.S. Gov't ; Research Support, U.S. Gov't, Non-P.H.S.
    ZDB-ID 3155-0
    ISSN 1520-5126 ; 0002-7863
    ISSN (online) 1520-5126
    ISSN 0002-7863
    DOI 10.1021/jacs.1c02232
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  7. Article ; Online: Tripodal P

    Fajardo, Javier / Peters, Jonas C

    Inorganic chemistry

    2021  Volume 60, Issue 2, Page(s) 1220–1227

    Abstract: Terminal dinitrogen complexes of iron ligated by tripodal, tetradentate ... ...

    Abstract Terminal dinitrogen complexes of iron ligated by tripodal, tetradentate P
    Language English
    Publishing date 2021-01-07
    Publishing country United States
    Document type Journal Article
    ZDB-ID 1484438-2
    ISSN 1520-510X ; 0020-1669
    ISSN (online) 1520-510X
    ISSN 0020-1669
    DOI 10.1021/acs.inorgchem.0c03354
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  8. Article: Synthesis and Functionalization Reactivity of Fe-Thiocarbonyl and Thiocarbyne Complexes.

    Deegan, Meaghan M / Peters, Jonas C

    Polyhedron

    2021  Volume 209

    Abstract: The remarkable catalytic transformation of CO to liquid hydrocarbons by Fe and Co catalysts in the industrial Fischer-Tropsch process motivates interest in developing well-defined systems to model aspects of this chemistry. One of the most interesting ... ...

    Abstract The remarkable catalytic transformation of CO to liquid hydrocarbons by Fe and Co catalysts in the industrial Fischer-Tropsch process motivates interest in developing well-defined systems to model aspects of this chemistry. One of the most interesting potential intermediates in this chemistry is a terminally-bound, first row metal carbide, yet a molecular model of this species remains elusive. With this in mind, we targeted the synthesis of highly-activated Fe-thiocarbonyl complexes, as prospective precursors to S-functionalization, C-S bond cleavage, and carbide generation. Herein, we describe the synthesis of three Fe-CS complexes that can be alkylated to generate a series of terminal Fe-carbynes that could be characterized across three oxidation states. Strategies to access C-S bond scission from these species are discussed, including limitations that, thus far, have precluded the generation of a terminal Fe-carbide for this system.
    Language English
    Publishing date 2021-09-04
    Publishing country England
    Document type Journal Article
    ZDB-ID 2000326-2
    ISSN 0277-5387
    ISSN 0277-5387
    DOI 10.1016/j.poly.2021.115461
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  9. Article ; Online: Intermolecular Proton-Coupled Electron Transfer Reactivity from a Persistent Charge-Transfer State for Reductive Photoelectrocatalysis.

    Garrido-Barros, Pablo / Romero, Catherine G / Winkler, Jay R / Peters, Jonas C

    Journal of the American Chemical Society

    2024  

    Abstract: Interest in applying proton-coupled electron transfer (PCET) reagents in reductive electro- and photocatalysis requires strategies that mitigate the competing hydrogen evolution reaction. Photoexcitation of a PCET donor to a charge-separated state (CSS) ... ...

    Abstract Interest in applying proton-coupled electron transfer (PCET) reagents in reductive electro- and photocatalysis requires strategies that mitigate the competing hydrogen evolution reaction. Photoexcitation of a PCET donor to a charge-separated state (CSS) can produce a powerful H-atom donor capable of being electrochemically recycled at a comparatively anodic potential corresponding to its ground state. However, the challenge is designing a mediator with a sufficiently long-lived excited state for bimolecular reactivity. Here, we describe a powerful ferrocene-derived photoelectrochemical PCET mediator exhibiting an unusually long-lived CSS (τ ∼ 0.9 μs). In addition to detailed photophysical studies, proof-of-concept stoichiometric and catalytic proton-coupled reductive transformations are presented, which illustrate the promise of this approach.
    Language English
    Publishing date 2024-04-26
    Publishing country United States
    Document type Journal Article
    ZDB-ID 3155-0
    ISSN 1520-5126 ; 0002-7863
    ISSN (online) 1520-5126
    ISSN 0002-7863
    DOI 10.1021/jacs.4c02610
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  10. Article ; Online: Catalytic transfer hydrogenation of N

    Johansen, Christian M / Boyd, Emily A / Peters, Jonas C

    Science advances

    2022  Volume 8, Issue 43, Page(s) eade3510

    Abstract: Inspired by momentum in applications of reductive photoredox catalysis to organic synthesis, photodriven transfer hydrogenations toward deep (>2 ... ...

    Abstract Inspired by momentum in applications of reductive photoredox catalysis to organic synthesis, photodriven transfer hydrogenations toward deep (>2 e
    Language English
    Publishing date 2022-10-26
    Publishing country United States
    Document type Journal Article
    ZDB-ID 2810933-8
    ISSN 2375-2548 ; 2375-2548
    ISSN (online) 2375-2548
    ISSN 2375-2548
    DOI 10.1126/sciadv.ade3510
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