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Article ; Online: Dynamical linear modeling estimates of long-term ozone trends from homogenized Dobson Umkehr profiles at Arosa/Davos, Switzerland

E. Maillard Barras / A. Haefele / R. Stübi / A. Jouberton / H. Schill / I. Petropavlovskikh / K. Miyagawa / M. Stanek / L. Froidevaux

Atmospheric Chemistry and Physics, Vol 22, Pp 14283-

2022 Volume 14302

Abstract: Six collocated spectrophotometers based in Arosa/Davos, Switzerland, have been measuring ozone profiles continuously since 1956 for the oldest Dobson instrument and since 2005 for the Brewer instruments. The datasets of these two ground-based triads ( ... ...

Abstract	Six collocated spectrophotometers based in Arosa/Davos, Switzerland, have been measuring ozone profiles continuously since 1956 for the oldest Dobson instrument and since 2005 for the Brewer instruments. The datasets of these two ground-based triads (three Dobsons and three Brewers) allow for continuous intercomparisons and derivation of long-term trend estimates. Mainly, two periods in the post-2000 Dobson D051 dataset show anomalies when compared to the Brewer triad time series: in 2011–2013, an offset has been attributed to technical interventions during the renewal of the spectrophotometer acquisition system, and in 2018, an offset with respect to the Brewer triad has been detected following an instrumental change on the spectrophotometer wedge. In this study, the worldwide longest Umkehr dataset (1956–2020) is carefully homogenized using collocated and simultaneous Dobson and Brewer measurements. A recently published report ( Garane et al. , 2022 ) described results of an independent homogenization of the same dataset performed by comparison to the Modern-Era Retrospective analysis for Research and Applications version 2 (MERRA-2) Global Modeling Initiative (M2GMI) model simulations. In this paper, the two versions of homogenized Dobson D051 records are intercompared to analyze residual differences found during the correction periods. The Aura Microwave Limb Sounder (MLS) station overpass record (2005–2020) is used as an independent reference for the comparisons. The two homogenized data records show common correction periods, except for the 2017–2018 period, and the corrections are similar in magnitude. In addition, the post-2000 ozone profile trends are estimated from the two homogenized Dobson D051 time series by dynamical linear modeling (DLM), and results are compared with the DLM trends derived from the collocated Brewer Umkehr time series. By first investigating the long-term Dobson ozone record for trends using the well-established multilinear regression (MLR) method, we find that the trends ...
Keywords	Physics ; QC1-999 ; Chemistry ; QD1-999
Subject code	333
Language	English
Publishing date	2022-11-01T00:00:00Z
Publisher	Copernicus Publications
Document type	Article ; Online
Database	BASE - Bielefeld Academic Search Engine (life sciences selection)

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Article ; Online: Stratospheric ozone measurements at Arosa (Switzerland)

J. Staehelin / P. Viatte / R. Stübi / F. Tummon / T. Peter

Atmospheric Chemistry and Physics, Vol 18, Pp 6567-

history and scientific relevance

2018 Volume 6584

Abstract: Climatic Observatory (LKO) in Arosa (Switzerland), marking the beginning of the world's longest series of total (or column) ozone measurements. They were driven by the recognition that atmospheric ozone is important for human health, as well as by ... ...

Abstract	Climatic Observatory (LKO) in Arosa (Switzerland), marking the beginning of the world's longest series of total (or column) ozone measurements. They were driven by the recognition that atmospheric ozone is important for human health, as well as by scientific curiosity about what was, at the time, an ill characterised atmospheric trace gas. From around the mid-1950s to the beginning of the 1970s studies of high atmosphere circulation patterns that could improve weather forecasting was justification for studying stratospheric ozone. In the mid-1970s, a paradigm shift occurred when it became clear that the damaging effects of anthropogenic ozone-depleting substances (ODSs), such as long-lived chlorofluorocarbons, needed to be documented. This justified continuing the ground-based measurements of stratospheric ozone. Levels of ODSs peaked around the mid-1990s as a result of a global environmental policy to protect the ozone layer, implemented through the 1987 Montreal Protocol and its subsequent amendments and adjustments. Consequently, chemical destruction of stratospheric ozone started to slow around the mid-1990s. To some extent, this raises the question as to whether continued ozone observation is indeed necessary. In the last decade there has been a tendency to reduce the costs associated with making ozone measurements globally including at Arosa. However, the large natural variability in ozone on diurnal, seasonal, and interannual scales complicates the capacity for demonstrating the success of the Montreal Protocol. Chemistry-climate models also predict a <q>super-recovery</q> of the ozone layer at mid-latitudes in the second half of this century, i.e. an increase of ozone concentrations beyond pre-1970 levels, as a consequence of ongoing climate change. These factors, and identifying potentially unexpected stratospheric responses to climate change, support the continued need to document stratospheric ozone changes. This is particularly valuable at the Arosa site, due to the unique length of the ...
Keywords	Physics ; QC1-999 ; Chemistry ; QD1-999
Subject code	290
Language	English
Publishing date	2018-05-01T00:00:00Z
Publisher	Copernicus Publications
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Article ; Online: A method to derive the Site Atmospheric State Best Estimate (SASBE) of ozone profiles from radiosonde and passive microwave data

E. Maillard Barras / A. Haefele / R. Stübi / D. Ruffieux

Atmospheric Measurement Techniques Discussions, Vol 8, Iss 3, Pp 3399-

2015 Volume 3422

Abstract: We present a method to derive the site atmospheric state best estimate (SASBE) of the ozone profile combining brightness temperature spectra around the 142 GHz absorption line of ozone measured by the microwave radiometer SOMORA and ozone profiles ... ...

Abstract	We present a method to derive the site atmospheric state best estimate (SASBE) of the ozone profile combining brightness temperature spectra around the 142 GHz absorption line of ozone measured by the microwave radiometer SOMORA and ozone profiles measured by the radiosonde (RS). The SASBE ozone profile is obtained using the radiosonde ozone profile as a priori information in an optimal estimation retrieval of the SOMORA radiometer. The resulting ozone profile ranges from ground up to 65 km altitude and makes optimal use of the available information at each altitude. The high vertical resolution of the radiosonde profile can be conserved and the uncertainty of the SASBE is well defined at each altitude. A SASBE ozone profile dataset has been generated for Payerne, Switzerland, with a temporal resolution of 3 profiles a week for the time period ranging from 2011 to 2013. The relative difference of the SASBE ozone profiles to the AURA/MLS ozone profiles lies between −3 to 6% over the vertical range of 20–65 km. Above 20 km, the agreement between the SASBE and AURA/MLS ozone profiles is better than the agreement between the operational SOMORA ozone data set and AURA/MLS. Below 20 km the SASBE ozone data are identical to the radiosonde measurements. The same method has been applied to ECWMF-ERA interim ozone profiles and SOMORA data to generate a SASBE dataset with a time resolution of 4 profiles per day. These SASBE ozone profiles agree between −4 and +8% with AURA/MLS. The improved agreement of the SASBE datasets with AURA/MLS above 20 km demonstrates the benefit of better a priori information in the retrieval of ozone from brightness temperature data.
Keywords	Meteorology. Climatology ; QC851-999 ; Physics ; QC1-999 ; Science ; Q ; Engineering (General). Civil engineering (General) ; TA1-2040 ; Earthwork. Foundations ; TA715-787
Subject code	290
Language	English
Publishing date	2015-03-01T00:00:00Z
Publisher	Copernicus Publications
Document type	Article ; Online
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Article ; Online: Evaluation of the use of five laboratory-determined ozone absorption cross sections in Brewer and Dobson retrieval algorithms

A. Redondas / R. Evans / R. Stuebi / U. Köhler / M. Weber

Atmospheric Chemistry and Physics, Vol 14, Iss 3, Pp 1635-

2014 Volume 1648

Abstract: The primary ground-based instruments used to report total column ozone (TOC) are Brewer and Dobson spectrophotometers in separate networks. These instruments make measurements of the UV irradiances, and through a well-defined process, a TOC value is ... ...

Abstract	The primary ground-based instruments used to report total column ozone (TOC) are Brewer and Dobson spectrophotometers in separate networks. These instruments make measurements of the UV irradiances, and through a well-defined process, a TOC value is produced. Inherent to the algorithm is the use of a laboratory-determined cross-section data set. We used five ozone cross-section data sets: three data sets that are based on measurements of Bass and Paur; one derived from Daumont, Brion and Malicet (DBM); and a new set determined by Institute of Experimental Physics (IUP), University of Bremen. The three Bass and Paur (1985) sets are as follows: quadratic temperature coefficients from the IGACO (a glossary is provided in Appendix A) web page (IGQ4), the Brewer network operational calibration set (BOp), and the set used by Bernhard et al. (2005) in the reanalysis of the Dobson absorption coefficient values (B05). The ozone absorption coefficients for Brewer and Dobson instruments are then calculated using the normal Brewer operative method, which is essentially the same as that used for Dobson instruments. Considering the standard TOC algorithm for the Brewer instruments and comparing to the Brewer standard operational calibration data set, using the slit functions for the individual instruments, we find the IUP data set changes the calculated TOC by −0.5%, the DBM data set changes the calculated TOC by −3.2%, and the IGQ4 data set at −45 °C changes the calculated TOC by +1.3%. Considering the standard algorithm for the Dobson instruments, and comparing to results using the official 1992 ozone absorption coefficients values and the single set of slit functions defined for all Dobson instruments, the calculated TOC changes by +1%, with little variation depending on which data set is used. We applied the changes to the European Dobson and Brewer reference instruments during the Izaña 2012 Absolute Calibration Campaign. With the application of a common Langley calibration and the IUP cross section, the differences ...
Keywords	Physics ; QC1-999 ; Chemistry ; QD1-999
Subject code	290
Language	English
Publishing date	2014-02-01T00:00:00Z
Publisher	Copernicus Publications
Document type	Article ; Online
Database	BASE - Bielefeld Academic Search Engine (life sciences selection)

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Article ; Online: Evaluation of the use of five laboratory determined ozone absorption cross sections in brewer and dobson retrieval algorithms

A. Redondas / R. Evans / R. Stuebi / U. Köhler / M. Weber

Atmospheric Chemistry and Physics Discussions, Vol 13, Iss 9, Pp 22979-

2013 Volume 23021

Abstract: The primary ground-based instruments used to report total column ozone (TOC) are Brewer and Dobson Spectrophotometers, in separate networks. These instruments make measurements of the UV irradiances, and through a well-defined process a TOC value is ... ...

Abstract	The primary ground-based instruments used to report total column ozone (TOC) are Brewer and Dobson Spectrophotometers, in separate networks. These instruments make measurements of the UV irradiances, and through a well-defined process a TOC value is produced. Inherent in the algorithm is the use of a laboratory determined cross-section data set. We used five ozone cross section data sets: three Bass and Paur, Daumont, Malicet and Brion (DMB) and a new Institute of Environmental Physics (IUP), University of Bremen, set. The three Bass and Paur (1985) sets are: quadratic temperature coefficients from IGACO web page (IGQ4), the Brewer network operational calibration set (BOp), and the set used by Bernhard et al. (2005), in the reanalysis of the Dobson absorption coefficient values (B05). The ozone absorption coefficients for Brewer and Dobson are then calculated using the normal Brewer operative method which is essentially the same as used on Dobson. Considering the standard TOC algorithm for the Brewer instruments and comparing to the Brewer standard operational calibration data set, using the slit functions for the individual instruments: we find the UIP data set changes the calculated TOC by −0.5%, the DBM data set changes the calculate TOC by −3.2%, and the IGQ4 data set at −45 °C changes the calculated TOC by +1.3%. Considering the standard algorithm for the Dobson instruments, and comparing to results using the official 1992 ozone absorption coefficients values and the single set of slit functions defined for all Dobson instruments, the calculated TOC changes by +1%, with little variation depending on which data set is used We applied the changes to the European Dobson and Brewer reference instruments during the Izaña 2012 Absolute Calibration Campaign. The application of a common Langley calibration and the IUP cross section the differences between Brewer and Dobson vanish whereas using Bass and Paur and DBM produce differences of 1.5% and 2% respectively. A study of temperature dependence of these cross section (XS) data sets is presented using the Arosa, Switzerland total ozone record of 2003–2006, obtained from two Brewer instrument types and a Dobson instrument, combined with the stratospheric ozone and temperature profiles from the Payerne soundings in the same period. The seasonal dependence of the differences between the results from the various instruments is greatly reduced with the application of temperature dependent absorption coefficients, with the greatest reduction obtained using the IUP data set.
Keywords	Environmental sciences ; GE1-350 ; Geography. Anthropology. Recreation ; G ; DOAJ:Environmental Sciences ; DOAJ:Earth and Environmental Sciences ; Geophysics. Cosmic physics ; QC801-809
Subject code	333
Language	English
Publishing date	2013-09-01T00:00:00Z
Publisher	Copernicus Publications
Document type	Article ; Online
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Article ; Online: Trajectory matching of ozonesondes and MOZAIC measurements in the UTLS – Part 2

J. Staufer / J. Staehelin / R. Stübi / T. Peter / F. Tummon / V. Thouret

Atmospheric Measurement Techniques, Vol 7, Iss 1, Pp 241-

Application to the global ozonesonde network

2014 Volume 266

Abstract: Both balloon-borne electrochemical ozonesondes and MOZAIC (measurements of ozone, water vapour, carbon monoxide and nitrogen oxides by in-service Airbus aircraft) provide very valuable data sets for ozone studies in the upper troposphere/lower ... ...

Abstract	Both balloon-borne electrochemical ozonesondes and MOZAIC (measurements of ozone, water vapour, carbon monoxide and nitrogen oxides by in-service Airbus aircraft) provide very valuable data sets for ozone studies in the upper troposphere/lower stratosphere (UTLS). Although MOZAIC's highly accurate UV-photometers are regularly inspected and recalibrated annually, recent analyses cast some doubt on the long-term stability of their ozone analysers. To investigate this further, we perform a 16 yr comparison (1994–2009) of UTLS ozone measurements from balloon-borne ozonesondes and MOZAIC. The analysis uses fully three-dimensional trajectories computed from ERA-Interim (European Centre for Medium-Range Weather Forecasts Re-analysis) wind fields to find matches between the two measurement platforms. Although different sensor types (Brewer-Mast and Electrochemical Concentration Cell ozonesondes) were used, most of the 28 launch sites considered show considerable differences of up to 25% compared to MOZAIC in the mid-1990s, followed by a systematic tendency to smaller differences of around 5–10% in subsequent years. The reason for the difference before 1998 remains unclear, but observations from both sondes and MOZAIC require further examination to be reliable enough for use in robust long-term trend analyses starting before 1998. According to our analysis, ozonesonde measurements at tropopause altitudes appear to be rather insensitive to changing the type of the Electrochemical Concentration Cell ozonesonde, provided the cathode sensing solution strength remains unchanged. Scoresbysund (Greenland) showed systematically 5% higher readings after changing from Science Pump Corporation sondes to ENSCI Corporation sondes, while a 1.0% KI cathode electrolyte was retained.
Keywords	Meteorology. Climatology ; QC851-999 ; Physics ; QC1-999 ; Science ; Q ; DOAJ:Meteorology and Climatology ; DOAJ:Earth and Environmental Sciences
Publishing date	2014-01-01T00:00:00Z
Publisher	Copernicus GmbH
Document type	Article ; Online
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Article ; Online: Ground-based ozone profiles over central Europe

L. Bernet / T. von Clarmann / S. Godin-Beekmann / G. Ancellet / E. Maillard Barras / R. Stübi / W. Steinbrecht / N. Kämpfer / K. Hocke

Atmospheric Chemistry and Physics, Vol 19, Pp 4289-

incorporating anomalous observations into the analysis of stratospheric ozone trends

2019 Volume 4309

Abstract: Observing stratospheric ozone is essential to assess whether the Montreal Protocol has succeeded in saving the ozone layer by banning ozone depleting substances. Recent studies have reported positive trends, indicating that ozone is recovering in the ... ...

Abstract	Observing stratospheric ozone is essential to assess whether the Montreal Protocol has succeeded in saving the ozone layer by banning ozone depleting substances. Recent studies have reported positive trends, indicating that ozone is recovering in the upper stratosphere at mid-latitudes, but the trend magnitudes differ, and uncertainties are still high. Trends and their uncertainties are influenced by factors such as instrumental drifts, sampling patterns, discontinuities, biases, or short-term anomalies that may all mask a potential ozone recovery. The present study investigates how anomalies, temporal measurement sampling rates, and trend period lengths influence resulting trends. We present an approach for handling suspicious anomalies in trend estimations. For this, we analysed multiple ground-based stratospheric ozone records in central Europe to identify anomalous periods in data from the GROund-based Millimetre-wave Ozone Spectrometer (GROMOS) located in Bern, Switzerland. The detected anomalies were then used to estimate ozone trends from the GROMOS time series by considering the anomalous observations in the regression. We compare our improved GROMOS trend estimate with results derived from the other ground-based ozone records (lidars, ozonesondes, and microwave radiometers), that are all part of the Network for the Detection of Atmospheric Composition Change (NDACC). The data indicate positive trends of 1 % decade −1 to 3 % decade −1 at an altitude of about 39 km (3 hPa ), providing a confirmation of ozone recovery in the upper stratosphere in agreement with satellite observations. At lower altitudes, the ground station data show inconsistent trend results, which emphasize the importance of ongoing research on ozone trends in the lower stratosphere. Our presented method of a combined analysis of ground station data provides a useful approach to recognize and to reduce uncertainties in stratospheric ozone trends by considering anomalies in the trend estimation. We conclude that stratospheric trend ...
Keywords	Physics ; QC1-999 ; Chemistry ; QD1-999
Subject code	333
Language	English
Publishing date	2019-04-01T00:00:00Z
Publisher	Copernicus Publications
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Article ; Online: Trajectory matching of ozonesondes and MOZAIC measurements in the UTLS – Part 2

J. Staufer / J. Staehelin / R. Stübi / T. Peter / F. Tummon / V. Thouret

Atmospheric Measurement Techniques Discussions, Vol 6, Iss 4, Pp 7099-

Application to the global ozonesonde network

2013 Volume 7148

Abstract: Ozone, an important greenhouse gas, has the largest climate forcing in the tropopause region, meaning that knowledge of long-term ozone changes in the upper troposphere/lower stratosphere (UTLS) is particularly important. Here, we perform a 16 yr ... ...

Abstract	Ozone, an important greenhouse gas, has the largest climate forcing in the tropopause region, meaning that knowledge of long-term ozone changes in the upper troposphere/lower stratosphere (UTLS) is particularly important. Here, we perform a 16 yr comparison (1994–2009) of UTLS ozone measurements from balloon-borne ozonesondes and MOZAIC (measurements of ozone, water vapor, carbon monoxide and nitrogen oxides by in-service Airbus aircraft). The analysis uses trajectories computed from ERA-Interim wind fields to find matches between the two measurement platforms. Ozonesonde data quality is most critical in the UTLS, where natural variability is high, particularly close to the tropopause. On average, at the 28 launch sites considered, ozone mixing ratios measured by the sondes exceed MOZAIC data by 5–15%, with differences being smaller in the LS than in the UT at many launch sites. For most sites, sondes and MOZAIC data are in close agreement after 1998. Before 1998 ozone mixing ratios measured by the Brewer–Mast (BM) sondes and Electrochemical Concentration Cell (ECC) sondes are systematically (up to 20%) higher than the MOZAIC UV photometers. The reason for this large difference remains unclear. Results also show that after 1998 large background current signals may affect ozonesonde performance, limiting the determination of reliable ozone trends in the UTLS. Sonde measurements appear to be insensitive to changing the type of ECC ozonesonde, provided the cathode sensing solution strength remains unchanged. Only Scoresbysund (Greenland) showed systematically higher readings after changing from Science Pump Corporation sondes to ENSCI Corporation sondes, while keeping a 1.0% KI cathode electrolyte. This suggests that ECC sondes, provided their background current and sensing solutions are properly monitored, are robust and reliable tools for ozone trend studies in the UTLS.
Keywords	Meteorology. Climatology ; QC851-999 ; Physics ; QC1-999 ; Science ; Q ; DOAJ:Meteorology and Climatology ; DOAJ:Earth and Environmental Sciences
Subject code	290
Language	English
Publishing date	2013-08-01T00:00:00Z
Publisher	Copernicus GmbH
Document type	Article ; Online
Database	BASE - Bielefeld Academic Search Engine (life sciences selection)

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Article ; Online: Trajectory matching of ozonesondes and MOZAIC measurements in the UTLS – Part 1

J. Staufer / J. Staehelin / R. Stübi / T. Peter / F. Tummon / V. Thouret

Atmospheric Measurement Techniques Discussions, Vol 6, Iss 4, Pp 7063-

Method description and application at Payerne, Switzerland

2013 Volume 7098

Abstract: With the aim of improving ozonesonde observations in the upper troposphere/lower stratosphere (UTLS), we use three-dimensional forward and backward trajectories, driven by ERA-Interim wind fields to match and compare ozonesonde measurements at Payerne ( ... ...

Abstract	With the aim of improving ozonesonde observations in the upper troposphere/lower stratosphere (UTLS), we use three-dimensional forward and backward trajectories, driven by ERA-Interim wind fields to match and compare ozonesonde measurements at Payerne (Switzerland) with observations from the MOZAIC aircraft program from 1994–2009. The uncertainties associated with the sonde–MOZAIC match technique were assessed using "self-matches", i.e. matches of instruments of the same type, such as MOZAIC–MOZAIC. Despite strong vertical ozone gradients of ozone at the tropopause, which render the match approach difficult, the method provides excellent results, showing mean differences between different MOZAIC aircraft of ±2% (typically with a few hours between the up- and downstream match points). Matches between MOZAIC aircraft and Payerne ozonesondes show an agreement of ±5% for sondes equipped with electrochemical concentration cells (ECC) and between <5% (not scaled to total ozone) and <10% (scaled) for the Brewer–Mast (BM) sondes after 1998. Prior to 1998, BM sondes show an offset of around 20% (scaled). No break can be identified through the change from the BM to ECC sonde types in September 2002. A comparison of BM sondes with ozone measurements from the NOXAR B747 project for the period 1995–1996 show a smaller offset of around 15% (scaled), which may indicate a small drift in the MOZAIC calibration.
Keywords	Meteorology. Climatology ; QC851-999 ; Physics ; QC1-999 ; Science ; Q ; DOAJ:Meteorology and Climatology ; DOAJ:Earth and Environmental Sciences ; Engineering (General). Civil engineering (General) ; TA1-2040 ; Earthwork. Foundations ; TA715-787
Subject code	551
Language	English
Publishing date	2013-08-01T00:00:00Z
Publisher	Copernicus Publications
Document type	Article ; Online
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Article ; Online: Updated trends of the stratospheric ozone vertical distribution in the 60° S–60° N latitude range based on the LOTUS regression model

S. Godin-Beekmann / N. Azouz / V. F. Sofieva / D. Hubert / I. Petropavlovskikh / P. Effertz / G. Ancellet / D. A. Degenstein / D. Zawada / L. Froidevaux / S. Frith / J. Wild / S. Davis / W. Steinbrecht / T. Leblanc / R. Querel / K. Tourpali / R. Damadeo / E. Maillard Barras /

R. Stübi / C. Vigouroux / C. Arosio / G. Nedoluha / I. Boyd / R. Van Malderen / E. Mahieu / D. Smale / R. Sussmann

Atmospheric Chemistry and Physics, Vol 22, Pp 11657-

2022 Volume 11673

Abstract: This study presents an updated evaluation of stratospheric ozone profile trends in the 60 ∘ S–60 ∘ N latitude range over the 2000–2020 period using an updated version of the Long-term Ozone Trends and Uncertainties in the Stratosphere (LOTUS) regression ... ...

Abstract	This study presents an updated evaluation of stratospheric ozone profile trends in the 60 ∘ S–60 ∘ N latitude range over the 2000–2020 period using an updated version of the Long-term Ozone Trends and Uncertainties in the Stratosphere (LOTUS) regression model that was used to evaluate such trends up to 2016 for the last WMO Ozone Assessment (2018). In addition to the derivation of detailed trends as a function of latitude and vertical coordinates, the regressions are performed with the datasets averaged over broad latitude bands, i.e. 60–35 ∘ S, 20 ∘ S–20 ∘ N and 35–60 ∘ N. The same methodology as in the last assessment is applied to combine trends in these broad latitude bands in order to compare the results with the previous studies. Longitudinally resolved merged satellite records are also considered in order to provide a better comparison with trends retrieved from ground-based records, e.g. lidar, ozonesondes, Umkehr, microwave and Fourier transform infrared (FTIR) spectrometers at selected stations where long-term time series are available. The study includes a comparison with trends derived from the REF-C2 simulations of the Chemistry Climate Model Initiative (CCMI-1). This work confirms past results showing an ozone increase in the upper stratosphere, which is now significant in the three broad latitude bands. The increase is largest in the Northern and Southern Hemisphere midlatitudes, with ∼2.2 ± 0.7 % per decade at ∼2.1 hPa and ∼2.1 ± 0.6 % per decade at ∼3.2 hPa respectively compared to ∼1.6 ± 0.6 % per decade at ∼2.6 hPa in the tropics. New trend signals have emerged from the records, such as a significant decrease in ozone in the tropics around 35 hPa and a non-significant increase in ozone in the southern midlatitudes at about 20 hPa. Non-significant negative ozone trends are derived in the lowermost stratosphere, with the most pronounced trends in the tropics. While a very good agreement is obtained between trends from merged satellite records and the CCMI-1 REF-C2 simulation in the upper ...
Keywords	Physics ; QC1-999 ; Chemistry ; QD1-999
Subject code	333
Language	English
Publishing date	2022-09-01T00:00:00Z
Publisher	Copernicus Publications
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