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  1. Article: Supramolecular isomerism and structural flexibility in coordination networks sustained by cadmium rod building blocks.

    Andaloussi, Yassin H / Bezrukov, Andrey A / Sensharma, Debobroto / Zaworotko, Michael J

    CrystEngComm

    2023  Volume 25, Issue 29, Page(s) 4175–4181

    Abstract: Bifunctional N-donor carboxylate linkers generally ... ...

    Abstract Bifunctional N-donor carboxylate linkers generally afford
    Language English
    Publishing date 2023-07-04
    Publishing country England
    Document type Journal Article
    ISSN 1466-8033
    ISSN 1466-8033
    DOI 10.1039/d3ce00557g
    Database MEDical Literature Analysis and Retrieval System OnLINE

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  2. Article ; Online: The Effect of Pendent Groups upon Flexibility in Coordination Networks with Square Lattice Topology.

    Li, Xia / Sensharma, Debobroto / Koupepidou, Kyriaki / Kong, Xiang-Jing / Zaworotko, Michael J

    ACS materials letters

    2023  Volume 5, Issue 9, Page(s) 2567–2575

    Abstract: Gas or vapor-induced phase transformations in flexible coordination networks (CNs) offer the potential to exceed the performance of their rigid counterparts for separation and storage applications. However, whereas ligand modification has been used to ... ...

    Abstract Gas or vapor-induced phase transformations in flexible coordination networks (CNs) offer the potential to exceed the performance of their rigid counterparts for separation and storage applications. However, whereas ligand modification has been used to alter the properties of such stimulus-responsive materials, they remain understudied compared with their rigid counterparts. Here, we report that a family of Zn
    Language English
    Publishing date 2023-08-22
    Publishing country United States
    Document type Journal Article
    ISSN 2639-4979
    ISSN (online) 2639-4979
    DOI 10.1021/acsmaterialslett.3c00565
    Database MEDical Literature Analysis and Retrieval System OnLINE

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  3. Article ; Online: Water vapour induced structural flexibility in a square lattice coordination network.

    Koupepidou, Kyriaki / Bezrukov, Andrey A / Castell, Dominic C / Sensharma, Debobroto / Mukherjee, Soumya / Zaworotko, Michael J

    Chemical communications (Cambridge, England)

    2023  Volume 59, Issue 93, Page(s) 13867–13870

    Abstract: Herein, we introduce a new square lattice topology coordination network, sql-(1,3-bib)(ndc)-Ni, with three types of connection and detail its gas and vapour induced phase transformations. Exposure to humidity resulted in an S-shaped isotherm profile, ... ...

    Abstract Herein, we introduce a new square lattice topology coordination network, sql-(1,3-bib)(ndc)-Ni, with three types of connection and detail its gas and vapour induced phase transformations. Exposure to humidity resulted in an S-shaped isotherm profile, suggesting potential utility of such materials as desiccants.
    Language English
    Publishing date 2023-11-21
    Publishing country England
    Document type Journal Article
    ZDB-ID 1472881-3
    ISSN 1364-548X ; 1359-7345 ; 0009-241X
    ISSN (online) 1364-548X
    ISSN 1359-7345 ; 0009-241X
    DOI 10.1039/d3cc04109c
    Database MEDical Literature Analysis and Retrieval System OnLINE

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  4. Article: Dinuclear Copper Sulfate-Based Square Lattice Topology Network with High Alkyne Selectivity.

    Andaloussi, Yassin H / Sensharma, Debobroto / Bezrukov, Andrey A / Castell, Dominic C / He, Tao / Darwish, Shaza / Zaworotko, Michael J

    Crystal growth & design

    2024  Volume 24, Issue 6, Page(s) 2573–2579

    Abstract: Porous coordination networks (PCNs) sustained by inorganic anions that serve as linker ligands can offer high selectivity toward specific gases or vapors in gas mixtures. Such inorganic anions are best exemplified by electron-rich fluorinated anions, e.g. ...

    Abstract Porous coordination networks (PCNs) sustained by inorganic anions that serve as linker ligands can offer high selectivity toward specific gases or vapors in gas mixtures. Such inorganic anions are best exemplified by electron-rich fluorinated anions, e.g., SiF
    Language English
    Publishing date 2024-02-27
    Publishing country United States
    Document type Journal Article
    ISSN 1528-7483
    ISSN 1528-7483
    DOI 10.1021/acs.cgd.4c00094
    Database MEDical Literature Analysis and Retrieval System OnLINE

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  5. Article: Pillar Modularity in

    Sensharma, Debobroto / Wilson, Benjamin H / Kumar, Naveen / O'Hearn, Daniel J / Zaworotko, Michael J

    Crystal growth & design

    2022  Volume 22, Issue 9, Page(s) 5472–5480

    Abstract: Hybrid ultramicroporous materials (HUMs) are porous coordination networks composed of combinations of organic and inorganic linker ligands with a pore diameter of <7 Å. Despite their benchmark gas sorption selectivity for several industrially relevant ... ...

    Abstract Hybrid ultramicroporous materials (HUMs) are porous coordination networks composed of combinations of organic and inorganic linker ligands with a pore diameter of <7 Å. Despite their benchmark gas sorption selectivity for several industrially relevant gas separations and their inherent modularity, the structural and compositional diversity of HUMs remains underexplored. In this contribution, we report a family of six HUMs (
    Language English
    Publishing date 2022-08-19
    Publishing country United States
    Document type Journal Article
    ISSN 1528-7483
    ISSN 1528-7483
    DOI 10.1021/acs.cgd.2c00561
    Database MEDical Literature Analysis and Retrieval System OnLINE

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  6. Article ; Online: Crystal Engineering of a New Hexafluorogermanate Pillared Hybrid Ultramicroporous Material Delivers Enhanced Acetylene Selectivity.

    Harvey-Reid, Nathan C / Sensharma, Debobroto / Mukherjee, Soumya / Patil, Komal M / Kumar, Naveen / Nikkhah, Sousa Javan / Vandichel, Matthias / Zaworotko, Michael J / Kruger, Paul E

    ACS applied materials & interfaces

    2024  Volume 16, Issue 4, Page(s) 4803–4810

    Abstract: Hybrid ultramicroporous materials (HUMs), metal-organic platforms that incorporate inorganic pillars, are a promising class of porous solids. A key area of interest for such materials is gas separation, where HUMs have already established benchmark ... ...

    Abstract Hybrid ultramicroporous materials (HUMs), metal-organic platforms that incorporate inorganic pillars, are a promising class of porous solids. A key area of interest for such materials is gas separation, where HUMs have already established benchmark performances. Thanks to their ready compositional modularity, we report the design and synthesis of a new HUM,
    Language English
    Publishing date 2024-01-23
    Publishing country United States
    Document type Journal Article
    ISSN 1944-8252
    ISSN (online) 1944-8252
    DOI 10.1021/acsami.3c16634
    Database MEDical Literature Analysis and Retrieval System OnLINE

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  7. Article ; Online: Effect of Polymorphism on the Sorption Properties of a Flexible Square-Lattice Topology Coordination Network.

    Subanbekova, Aizhamal / Bezrukov, Andrey A / Bon, Volodymyr / Nikolayenko, Varvara I / Koupepidou, Kyriaki / Sensharma, Debobroto / Javan Nikkhah, Sousa / Wang, Shi-Qiang / Kaskel, Stefan / Vandichel, Matthias / Zaworotko, Michael J

    ACS applied materials & interfaces

    2024  

    Abstract: The stimulus-responsive behavior of coordination networks (CNs), which switch between closed (nonporous) and open (porous) phases, is of interest because of its potential utility in gas storage and separation. Herein, we report two polymorphs of a new ... ...

    Abstract The stimulus-responsive behavior of coordination networks (CNs), which switch between closed (nonporous) and open (porous) phases, is of interest because of its potential utility in gas storage and separation. Herein, we report two polymorphs of a new square-lattice (
    Language English
    Publishing date 2024-04-26
    Publishing country United States
    Document type Journal Article
    ISSN 1944-8252
    ISSN (online) 1944-8252
    DOI 10.1021/acsami.4c03777
    Database MEDical Literature Analysis and Retrieval System OnLINE

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  8. Article ; Online: Crystal engineering of porous coordination networks to enable separation of C2 hydrocarbons.

    Mukherjee, Soumya / Sensharma, Debobroto / Chen, Kai-Jie / Zaworotko, Michael J

    Chemical communications (Cambridge, England)

    2020  Volume 56, Issue 72, Page(s) 10419–10441

    Abstract: Crystal engineering, the field of chemistry that studies the design, properties, and applications of crystals, is exemplified by the emergence over the past thirty years of porous coordination networks (PCNs), including metal-organic frameworks (MOFs) ... ...

    Abstract Crystal engineering, the field of chemistry that studies the design, properties, and applications of crystals, is exemplified by the emergence over the past thirty years of porous coordination networks (PCNs), including metal-organic frameworks (MOFs) and hybrid coordination networks (HCNs). PCNs have now come of age thanks to their amenability to design from first principles and how this in turn can result in new materials with task-specific features. Herein, we focus upon how control over the pore chemistry and pore size of PCNs has been leveraged to create a new generation of physisorbents for efficient purification of light hydrocarbons (LHs). The impetus for this research comes from the need to address LH purification processes based upon cryogenic separation, distillation, chemisorption or solvent extraction, each of which is energy intensive. Adsorptive separation by physisorbents (in general) and PCNs (in particular) can offer two advantages over these existing approaches: improved energy efficiency; lower plant size/cost. Unfortunately, most existing physisorbents suffer from low uptake and/or poor sorbate selectivity and are therefore unsuitable for trace separations of LHs including the high volume C2 LHs (C
    Language English
    Publishing date 2020-08-06
    Publishing country England
    Document type Journal Article
    ZDB-ID 1472881-3
    ISSN 1364-548X ; 1359-7345 ; 0009-241X
    ISSN (online) 1364-548X
    ISSN 1359-7345 ; 0009-241X
    DOI 10.1039/d0cc04645k
    Database MEDical Literature Analysis and Retrieval System OnLINE

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  9. Article: Crystal engineering of porous coordination networks to enable separation of C2 hydrocarbons

    Mukherjee, Soumya / Sensharma, Debobroto / Chen, Kai-Jie / Zaworotko, Michael J

    Chemical communications. 2020 Sept. 10, v. 56, no. 72

    2020  

    Abstract: Crystal engineering, the field of chemistry that studies the design, properties, and applications of crystals, is exemplified by the emergence over the past thirty years of porous coordination networks (PCNs), including metal–organic frameworks (MOFs) ... ...

    Abstract Crystal engineering, the field of chemistry that studies the design, properties, and applications of crystals, is exemplified by the emergence over the past thirty years of porous coordination networks (PCNs), including metal–organic frameworks (MOFs) and hybrid coordination networks (HCNs). PCNs have now come of age thanks to their amenability to design from first principles and how this in turn can result in new materials with task-specific features. Herein, we focus upon how control over the pore chemistry and pore size of PCNs has been leveraged to create a new generation of physisorbents for efficient purification of light hydrocarbons (LHs). The impetus for this research comes from the need to address LH purification processes based upon cryogenic separation, distillation, chemisorption or solvent extraction, each of which is energy intensive. Adsorptive separation by physisorbents (in general) and PCNs (in particular) can offer two advantages over these existing approaches: improved energy efficiency; lower plant size/cost. Unfortunately, most existing physisorbents suffer from low uptake and/or poor sorbate selectivity and are therefore unsuitable for trace separations of LHs including the high volume C2 LHs (C₂Hₓ, x = 2, 4, 6). This situation is rapidly changing thanks to PCN sorbents that have set new performance benchmarks for several C2 separations. Herein, we review and analyse PCN sorbents with respect to the supramolecular chemistry of sorbent–sorbate binding and detail the crystal engineering approaches that have enabled the exquisite control over pore size and pore chemistry that affords highly selective binding sites. Whereas the structure–function relationships that have emerged offer important design principles, several development roadblocks remain to be overcome.
    Keywords distillation ; energy efficiency ; porosity ; solvents ; sorbents
    Language English
    Dates of publication 2020-0910
    Size p. 10419-10441.
    Publishing place The Royal Society of Chemistry
    Document type Article
    Note NAL-AP-2-clean
    ZDB-ID 1472881-3
    ISSN 1364-548X ; 1359-7345 ; 0009-241X
    ISSN (online) 1364-548X
    ISSN 1359-7345 ; 0009-241X
    DOI 10.1039/d0cc04645k
    Database NAL-Catalogue (AGRICOLA)

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  10. Article ; Online: CO

    Ullah, Saif / Tan, Kui / Sensharma, Debobroto / Kumar, Naveen / Mukherjee, Soumya / Bezrukov, Andrey A / Li, Jing / Zaworotko, Michael J / Thonhauser, Timo

    Angewandte Chemie (International ed. in English)

    2022  Volume 61, Issue 35, Page(s) e202206613

    Abstract: Although pyrazine-linked hybrid ultramicroporous materials (HUMs, pore size <7 Å) are benchmark physisorbents for trace carbon dioxide ( ... ...

    Abstract Although pyrazine-linked hybrid ultramicroporous materials (HUMs, pore size <7 Å) are benchmark physisorbents for trace carbon dioxide (CO
    Language English
    Publishing date 2022-07-08
    Publishing country Germany
    Document type Journal Article
    ZDB-ID 2011836-3
    ISSN 1521-3773 ; 1433-7851
    ISSN (online) 1521-3773
    ISSN 1433-7851
    DOI 10.1002/anie.202206613
    Database MEDical Literature Analysis and Retrieval System OnLINE

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