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  1. Article ; Online: Coordination-Induced Multivalent Self-Assembling Catalysts for Spectral Sensing Zn

    Li, Shuai-Bing / Shen, Jiang-Shan

    Inorganic chemistry

    2023  Volume 62, Issue 24, Page(s) 9454–9462

    Abstract: The introduction of signal amplification to molecular spectral sensing systems is an intriguing topic in supramolecular analytical chemistry. In this study, click chemistry was used to generate a triazole moiety to bridge with a long hydrophobic alkyl ... ...

    Abstract The introduction of signal amplification to molecular spectral sensing systems is an intriguing topic in supramolecular analytical chemistry. In this study, click chemistry was used to generate a triazole moiety to bridge with a long hydrophobic alkyl chain (C
    Language English
    Publishing date 2023-06-03
    Publishing country United States
    Document type Journal Article
    ZDB-ID 1484438-2
    ISSN 1520-510X ; 0020-1669
    ISSN (online) 1520-510X
    ISSN 0020-1669
    DOI 10.1021/acs.inorgchem.3c00545
    Database MEDical Literature Analysis and Retrieval System OnLINE

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  2. Article ; Online: Modulating Dual Fluorescence Emissions in Imine-Based Probes to Distinguish D

    Ji, Rui-Xue / Shen, Jiang-Shan

    The journal of physical chemistry. B

    2023  Volume 127, Issue 5, Page(s) 1229–1236

    Abstract: How to distinguish ... ...

    Abstract How to distinguish D
    Language English
    Publishing date 2023-01-25
    Publishing country United States
    Document type Journal Article
    ISSN 1520-5207
    ISSN (online) 1520-5207
    DOI 10.1021/acs.jpcb.2c08070
    Database MEDical Literature Analysis and Retrieval System OnLINE

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  3. Article ; Online: A Non-Hydrolysis Reaction-Based Imine for Fluorescence Response toward Al

    Jiang, Xu / Ji, Rui-Xue / Shen, Jiang-Shan

    ChemPlusChem

    2023  Volume 88, Issue 3, Page(s) e202300037

    Abstract: Designing an imine-based fluorescent probe capable of greatly suppressing the tendency of intrinsic hydrolysis reaction is an attractive topic in the field of chemo-/biosensing. In this work, hydrophobic 1,1'-binaphthyl-2,2'-diamine containing two amine ... ...

    Abstract Designing an imine-based fluorescent probe capable of greatly suppressing the tendency of intrinsic hydrolysis reaction is an attractive topic in the field of chemo-/biosensing. In this work, hydrophobic 1,1'-binaphthyl-2,2'-diamine containing two amine groups was introduced to synthesize probe R-1 bearing two imine bonds linked by two salicylaldehyde (SAs). The hydrophobicity of binaphthyl moiety and the unique clamp-like structure formed from double imine bonds and from ortho-OH on SA part make probe R-1 is able to function as an ideal receptor to coordinate with Al
    Language English
    Publishing date 2023-02-16
    Publishing country Germany
    Document type Journal Article
    ISSN 2192-6506
    ISSN (online) 2192-6506
    DOI 10.1002/cplu.202300037
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  4. Article: Enantioselective Dynamic Exchange Reactions of Imines

    Ji, Rui-Xue / Liu, Ning / Shen, Jiang-Shan

    Journal of organic chemistry. 2021 Sept. 06, v. 86, no. 18

    2021  

    Abstract: Although dynamic reactions of imines have been extensively studied, the dynamic behaviors manipulated by chirality remain nearly unexplored. In this work, enantioselective amine exchange reactions were demonstrated as a first example via the reaction of ... ...

    Abstract Although dynamic reactions of imines have been extensively studied, the dynamic behaviors manipulated by chirality remain nearly unexplored. In this work, enantioselective amine exchange reactions were demonstrated as a first example via the reaction of enantiomeric chiral amines such as natural amino acids with a series of innovative axially chiral 1,1′-binaphthyl-2,2′-diamine (BNDA)-based imines that were prepared from the condensation reactions between BNDA and salicylaldehyde (SA) or its derivatives. This enantioselective dynamic behavior can be directly indicated by the degree of the fluorescence response of the R-configuration of imines to the d-enantiomer of chiral amine, because the released BNDA can serve as the fluorescence signal output when the amine exchange reaction occurs, which is far higher than the response to its l-enantiomer under identical experimental conditions. For the S-configuration of chiral imines, the fluorescence response is the opposite. The enantioselective exchange reaction can be tuned by altering the electron-withdrawing or electron-donating capability of the substituent at position 4 or 5 of the SA part of chiral imines. Not only o-OH groups in SA-based imines but also protic solvents used as reaction media were found to be important to the dynamic behavior at high rates.
    Keywords enantioselectivity ; fluorescence ; hydroxybenzaldehyde ; imines ; optical isomerism ; organic chemistry
    Language English
    Dates of publication 2021-0906
    Size p. 12932-12944.
    Publishing place American Chemical Society
    Document type Article
    ZDB-ID 123490-0
    ISSN 1520-6904 ; 0022-3263
    ISSN (online) 1520-6904
    ISSN 0022-3263
    DOI 10.1021/acs.joc.1c01620
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    In stock of ZB MED Bonn / Germany

    Z 4' 49/42: Show issues
    Z 7.1: Show issues

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  5. Article: A Multi-Catalytic Sensing for Hydrogen Peroxide, Glucose, and Organophosphorus Pesticides Based on Carbon Dots.

    Li, Ping / Sun, Xiang-Ying / Shen, Jiang-Shan

    Frontiers in chemistry

    2021  Volume 9, Page(s) 713104

    Abstract: In this work, a facile one-pot hydrothermal route was employed to synthesize a series of fluorescent carbon dots (CDs) by using 20 natural amino acids, respectively, as the starting materials. It was found that the CDs synthesized using phenylalanine ... ...

    Abstract In this work, a facile one-pot hydrothermal route was employed to synthesize a series of fluorescent carbon dots (CDs) by using 20 natural amino acids, respectively, as the starting materials. It was found that the CDs synthesized using phenylalanine could possess the intrinsic peroxidase-like activity that could effectively catalyze a traditional peroxidase substrate like 3, 3', 5, 5'- tetramethylbenzidine (TMB) in the presence of H
    Language English
    Publishing date 2021-07-12
    Publishing country Switzerland
    Document type Journal Article
    ZDB-ID 2711776-5
    ISSN 2296-2646
    ISSN 2296-2646
    DOI 10.3389/fchem.2021.713104
    Database MEDical Literature Analysis and Retrieval System OnLINE

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  6. Article ; Online: Enantioselective Dynamic Exchange Reactions of Imines.

    Ji, Rui-Xue / Liu, Ning / Shen, Jiang-Shan

    The Journal of organic chemistry

    2021  Volume 86, Issue 18, Page(s) 12932–12944

    Abstract: Although dynamic reactions of imines have been extensively studied, the dynamic behaviors manipulated by chirality remain nearly unexplored. In this work, enantioselective amine exchange reactions were demonstrated as a first example via the reaction of ... ...

    Abstract Although dynamic reactions of imines have been extensively studied, the dynamic behaviors manipulated by chirality remain nearly unexplored. In this work, enantioselective amine exchange reactions were demonstrated as a first example via the reaction of enantiomeric chiral amines such as natural amino acids with a series of innovative axially chiral 1,1'-binaphthyl-2,2'-diamine (BNDA)-based imines that were prepared from the condensation reactions between BNDA and salicylaldehyde (SA) or its derivatives. This enantioselective dynamic behavior can be directly indicated by the degree of the fluorescence response of the
    MeSH term(s) Amines ; Catalysis ; Diamines ; Imines ; Stereoisomerism
    Chemical Substances Amines ; Diamines ; Imines
    Language English
    Publishing date 2021-09-06
    Publishing country United States
    Document type Journal Article ; Research Support, Non-U.S. Gov't
    ZDB-ID 123490-0
    ISSN 1520-6904 ; 0022-3263
    ISSN (online) 1520-6904
    ISSN 0022-3263
    DOI 10.1021/acs.joc.1c01620
    Database MEDical Literature Analysis and Retrieval System OnLINE

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    In stock of ZB MED Cologne/Königswinter

    Zs.A 4473: Show issues Location:
    Je nach Verfügbarkeit (siehe Angabe bei Bestand)
    bis Jg. 1994: Bestellungen von Artikeln über das Online-Bestellformular
    Jg. 1995 - 2021: Lesesall (2.OG)
    ab Jg. 2022: Lesesaal (EG)

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  7. Article ; Online: Minimalistic Artificial Catalysts with Esterase-Like Activity from Multivalent Nanofibers Formed by the Self-Assembly of Dipeptides.

    Liu, Ning / Li, Shuai-Bing / Zheng, Yan-Zhen / Xu, Su-Ying / Shen, Jiang-Shan

    ACS omega

    2022  Volume 8, Issue 2, Page(s) 2491–2500

    Abstract: Imitating and incorporating the multiple key structural features observed in natural enzymes into a minimalistic molecule to develop an artificial catalyst with outstanding catalytic efficiency is an attractive topic for chemists. Herein, we designed and ...

    Abstract Imitating and incorporating the multiple key structural features observed in natural enzymes into a minimalistic molecule to develop an artificial catalyst with outstanding catalytic efficiency is an attractive topic for chemists. Herein, we designed and synthesized one class of minimalistic dipeptide molecules containing a terminal -SH group and a terminal His-Phe dipeptide head linked by a hydrophobic alkyl chain with different lengths, marked as HS-C
    Language English
    Publishing date 2022-12-30
    Publishing country United States
    Document type Journal Article
    ISSN 2470-1343
    ISSN (online) 2470-1343
    DOI 10.1021/acsomega.2c06972
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  8. Article ; Online: Reaction-based fluorescence probes for "turn on" sensing fluoride ions.

    He, Wen-Ying / Liu, Ning / Jiang, Xu / Zheng, Yan-Zhen / Lin, Zhi-Wei / Shen, Jiang-Shan

    Organic & biomolecular chemistry

    2022  Volume 20, Issue 6, Page(s) 1191–1195

    Abstract: Introducing a weak covalent bond into an originally highly fluorescent molecule to create a non-fluorescent probe is able to provide a new way to detect some nucleophilic targets with enhanced sensitivity. Herein, this is the first time that a ... ...

    Abstract Introducing a weak covalent bond into an originally highly fluorescent molecule to create a non-fluorescent probe is able to provide a new way to detect some nucleophilic targets with enhanced sensitivity. Herein, this is the first time that a tetraphenylethene (TPE)-based probe (TPEONO
    Language English
    Publishing date 2022-02-09
    Publishing country England
    Document type Journal Article ; Research Support, Non-U.S. Gov't
    ZDB-ID 2097583-1
    ISSN 1477-0539 ; 1477-0520
    ISSN (online) 1477-0539
    ISSN 1477-0520
    DOI 10.1039/d1ob02324a
    Database MEDical Literature Analysis and Retrieval System OnLINE

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  9. Article ; Online: Polyfluoroalkyl Chain-Based Assemblies for Biomimetic Catalysis.

    Liu, Ning / Gao, Ping / Lu, Hai-Yan / Fang, Lei / Nicolas, Julien / Ha-Duong, Tâp / Shen, Jiang-Shan

    Chemistry (Weinheim an der Bergstrasse, Germany)

    2023  Volume 30, Issue 1, Page(s) e202302669

    Abstract: Amphiphobic fluoroalkyl chains are exploited for creating robust and diverse self-assembled biomimetic catalysts. Long terminal perfluoroalkyl chains ( ... ...

    Abstract Amphiphobic fluoroalkyl chains are exploited for creating robust and diverse self-assembled biomimetic catalysts. Long terminal perfluoroalkyl chains (C
    Language English
    Publishing date 2023-11-13
    Publishing country Germany
    Document type Journal Article
    ZDB-ID 1478547-X
    ISSN 1521-3765 ; 0947-6539
    ISSN (online) 1521-3765
    ISSN 0947-6539
    DOI 10.1002/chem.202302669
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  10. Article: Facile access to versatile aza-macrolides through iridium-catalysed cascade allyl-amination/macrolactonization

    Fu, Wei / Wang, Lianhui / Yang, Zi / Shen, Jiang-Shan / Tang, Fei / Zhang, Jiayi / Cui, Xiuling

    Chemical communications. 2020 Jan. 21, v. 56, no. 6

    2020  

    Abstract: Direct access to benzo-fused aza-macrolides was successfully achieved through iridium-catalysed intermolecular decarboxylative coupling of vinylethylene carbonates with isatoic anhydrides under relatively mild reaction conditions. Notably, this reaction ... ...

    Abstract Direct access to benzo-fused aza-macrolides was successfully achieved through iridium-catalysed intermolecular decarboxylative coupling of vinylethylene carbonates with isatoic anhydrides under relatively mild reaction conditions. Notably, this reaction proceeded through sequential allyl-amination/macrolactonization upon extrusion of CO₂. Moreover, favourable fluorescence properties could be observed in the title macrocyclic products.
    Keywords anhydrides ; carbon dioxide ; carbonates ; catalytic activity ; chemical reactions ; extrusion ; fluorescence ; iridium
    Language English
    Dates of publication 2020-0121
    Size p. 960-963.
    Publishing place The Royal Society of Chemistry
    Document type Article
    ZDB-ID 1472881-3
    ISSN 1364-548X ; 1359-7345 ; 0009-241X
    ISSN (online) 1364-548X
    ISSN 1359-7345 ; 0009-241X
    DOI 10.1039/c9cc07372h
    Database NAL-Catalogue (AGRICOLA)

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