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  1. Article ; Online: Engineering Surface Passivation and Hole Transport Layer on Hematite Photoanodes Enabling Robust Photoelectrocatalytic Water Oxidation.

    Xie, Huimin / Song, Yurou / Jiao, Yuye / Gao, Lihua / Shi, Shaobo / Wang, Chen / Hou, Jungang

    ACS nano

    2024  

    Abstract: Regulation of charge transport at the molecular level is essential to elucidating the kinetics of junction photoelectrodes across the heterointerface for photoelectrochemical (PEC) water oxidation. Herein, an integrated photoanode as the prototype was ... ...

    Abstract Regulation of charge transport at the molecular level is essential to elucidating the kinetics of junction photoelectrodes across the heterointerface for photoelectrochemical (PEC) water oxidation. Herein, an integrated photoanode as the prototype was constructed by use of a 5,10,15,20-tetrakis(4-carboxyphenyl) porphyrin-cobalt molecule (CoTCPP) and ZnO on hematite (α-Fe
    Language English
    Publishing date 2024-02-11
    Publishing country United States
    Document type Journal Article
    ISSN 1936-086X
    ISSN (online) 1936-086X
    DOI 10.1021/acsnano.3c11638
    Database MEDical Literature Analysis and Retrieval System OnLINE

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  2. Article ; Online: BiVO

    Shi, Shaobo / Song, Yurou / Jiao, Yuye / Jin, Dingfeng / Li, Zhuwei / Xie, Huimin / Gao, Lihua / Sun, Licheng / Hou, Jungang

    Nano letters

    2024  

    Abstract: Photoelectrochemical (PEC) cells provide a promising solution for the synthesis of hydrogen peroxide ( ... ...

    Abstract Photoelectrochemical (PEC) cells provide a promising solution for the synthesis of hydrogen peroxide (H
    Language English
    Publishing date 2024-04-29
    Publishing country United States
    Document type Journal Article
    ISSN 1530-6992
    ISSN (online) 1530-6992
    DOI 10.1021/acs.nanolett.4c00901
    Database MEDical Literature Analysis and Retrieval System OnLINE

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  3. Article ; Online: Metal-Organic Framework Glass Catalysts from Melting Glass-Forming Cobalt-Based Zeolitic Imidazolate Framework for Boosting Photoelectrochemical Water Oxidation.

    Song, Yurou / Ren, Yanhan / Cheng, Huijie / Jiao, Yuye / Shi, Shaobo / Gao, Lihua / Xie, Huimin / Gao, Junfeng / Sun, Licheng / Hou, Jungang

    Angewandte Chemie (International ed. in English)

    2023  Volume 62, Issue 32, Page(s) e202306420

    Abstract: Sluggish oxygen evolution kinetics and serious charge recombination restrict the development of photoelectrochemical (PEC) water splitting. The advancement of novel metal-organic frameworks (MOFs) catalysts bears practical significance for improving PEC ... ...

    Abstract Sluggish oxygen evolution kinetics and serious charge recombination restrict the development of photoelectrochemical (PEC) water splitting. The advancement of novel metal-organic frameworks (MOFs) catalysts bears practical significance for improving PEC water splitting performance. Herein, a MOF glass catalyst through melting glass-forming cobalt-based zeolitic imidazolate framework (Co-a
    Language English
    Publishing date 2023-06-28
    Publishing country Germany
    Document type Journal Article
    ZDB-ID 2011836-3
    ISSN 1521-3773 ; 1433-7851
    ISSN (online) 1521-3773
    ISSN 1433-7851
    DOI 10.1002/anie.202306420
    Database MEDical Literature Analysis and Retrieval System OnLINE

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  4. Article: Engineering Single-Atom Active Sites on Covalent Organic Frameworks for Boosting CO₂ Photoreduction

    Ran, Lei / Li, Zhuwei / Ran, Bei / Cao, Jiaqi / Zhao, Yue / Shao, Teng / Song, Yurou / Leung, Michael K. H. / Sun, Licheng / Hou, Jungang

    Journal of the American Chemical Society. 2022 Sept. 06, v. 144, no. 37

    2022  

    Abstract: Solar carbon dioxide (CO₂) conversion is an emerging solution to meet the challenges of sustainable energy systems and environmental/climate concerns. However, the construction of isolated active sites not only influences catalytic activity but also ... ...

    Abstract Solar carbon dioxide (CO₂) conversion is an emerging solution to meet the challenges of sustainable energy systems and environmental/climate concerns. However, the construction of isolated active sites not only influences catalytic activity but also limits the understanding of the structure–catalyst relationship of CO₂ reduction. Herein, we develop a universal synthetic protocol to fabricate different single-atom metal sites (e.g., Fe, Co, Ni, Zn, Cu, Mn, and Ru) anchored on the triazine-based covalent organic framework (SAS/Tr-COF) backbone with the bridging structure of metal–nitrogen–chlorine for high-performance catalytic CO₂ reduction. Remarkably, the as-synthesized Fe SAS/Tr-COF as a representative catalyst achieved an impressive CO generation rate as high as 980.3 μmol g–¹ h–¹ and a selectivity of 96.4%, over approximately 26 times higher than that of the pristine Tr-COF under visible light irradiation. From X-ray absorption fine structure analysis and density functional theory calculations, the superior photocatalytic performance is attributed to the synergic effect of atomically dispersed metal sites and Tr-COF host, decreasing the reaction energy barriers for the formation of *COOH intermediates and promoting CO₂ adsorption and activation as well as CO desorption. This work not only affords rational design of state-of-the-art catalysts at the molecular level but also provides in-depth insights for efficient CO₂ conversion.
    Keywords X-ray absorption spectroscopy ; adsorption ; carbon dioxide ; catalysts ; climate ; density functional theory ; desorption ; energy ; irradiation ; light ; photocatalysis ; photoreduction ; renewable energy sources ; synergism
    Language English
    Dates of publication 2022-0906
    Size p. 17097-17109.
    Publishing place American Chemical Society
    Document type Article
    ZDB-ID 3155-0
    ISSN 1520-5126 ; 0002-7863
    ISSN (online) 1520-5126
    ISSN 0002-7863
    DOI 10.1021/jacs.2c06920
    Database NAL-Catalogue (AGRICOLA)

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    In stock of ZB MED Bonn / Germany

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  5. Article ; Online: Engineering Single-Atom Active Sites on Covalent Organic Frameworks for Boosting CO

    Ran, Lei / Li, Zhuwei / Ran, Bei / Cao, Jiaqi / Zhao, Yue / Shao, Teng / Song, Yurou / Leung, Michael K H / Sun, Licheng / Hou, Jungang

    Journal of the American Chemical Society

    2022  Volume 144, Issue 37, Page(s) 17097–17109

    Abstract: Solar carbon dioxide ( ... ...

    Abstract Solar carbon dioxide (CO
    Language English
    Publishing date 2022-09-06
    Publishing country United States
    Document type Journal Article
    ZDB-ID 3155-0
    ISSN 1520-5126 ; 0002-7863
    ISSN (online) 1520-5126
    ISSN 0002-7863
    DOI 10.1021/jacs.2c06920
    Database MEDical Literature Analysis and Retrieval System OnLINE

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    Kategorien

    In stock of ZB MED Bonn / Germany

    Z 4' 55/32: Show issues
    Z 7.3: Show issues

    Order via subito

    This service is chargeable due to the Delivery terms set by subito. Orders including an article and supplementary material will be classified as separate orders. In these cases, fees will be demanded for each order.

    Inter-library loan at ZB MED

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  6. Article ; Online: Engineering MoO

    Song, Yurou / Zhang, Xiaomeng / Zhang, Yanxue / Zhai, Panlong / Li, Zhuwei / Jin, Dingfeng / Cao, Jiaqi / Wang, Chen / Zhang, Bo / Gao, Junfeng / Sun, Licheng / Hou, Jungang

    Angewandte Chemie (International ed. in English)

    2022  Volume 61, Issue 16, Page(s) e202200946

    Abstract: The development of semiconductor photoanodes is of great practical interest for the realization of photoelectrochemical (PEC) water splitting. Herein, MXene quantum dots (MQD) were grafted on a ... ...

    Abstract The development of semiconductor photoanodes is of great practical interest for the realization of photoelectrochemical (PEC) water splitting. Herein, MXene quantum dots (MQD) were grafted on a BiVO
    Language English
    Publishing date 2022-02-21
    Publishing country Germany
    Document type Journal Article
    ZDB-ID 2011836-3
    ISSN 1521-3773 ; 1433-7851
    ISSN (online) 1521-3773
    ISSN 1433-7851
    DOI 10.1002/anie.202200946
    Database MEDical Literature Analysis and Retrieval System OnLINE

    Full text online

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