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  1. Article: [Characteristics of Water-soluble Inorganic Ions in Atmospheric Aerosols in Shenyang].

    Miao, Hong-Yan / Wen, Tian-Xue / Wang, Lu / Xu, Hui

    Huan jing ke xue= Huanjing kexue

    2018  Volume 37, Issue 6, Page(s) 2017–2024

    Abstract: To investigate the levels and seasonal variation of water soluble inorganic components in ambient aerosol in Shenyang, 25 samples were collected with Andersen cascade sampler from Jun. 2012 to May. 2013 and nine water-soluble ions in samples were ... ...

    Abstract To investigate the levels and seasonal variation of water soluble inorganic components in ambient aerosol in Shenyang, 25 samples were collected with Andersen cascade sampler from Jun. 2012 to May. 2013 and nine water-soluble ions in samples were analyzed by IC. The different characteristics of aerosols between clean and pollution days in winter were discussed based on these samples. The results showed that the annual concentrations of total water soluble inorganic ions were 22.30 μg·m<sup>-3</sup> and 14.29 μg·m<sup>-3</sup> in fine and coarse particles, and SO
    MeSH term(s) Aerosols/analysis ; Air Pollutants/analysis ; China ; Environmental Monitoring ; Ions/analysis ; Particle Size ; Particulate Matter/analysis ; Solubility ; Water
    Chemical Substances Aerosols ; Air Pollutants ; Ions ; Particulate Matter ; Water (059QF0KO0R)
    Language Chinese
    Publishing date 2018-07-02
    Publishing country China
    Document type Journal Article
    ISSN 0250-3301
    ISSN 0250-3301
    DOI 10.13227/j.hjkx.2016.06.003
    Database MEDical Literature Analysis and Retrieval System OnLINE

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  2. Article: [Characterization and Size Distribution of Carbonaceous Aerosols at Mountain Dinghu].

    Li, An-Na / Wen, Tian-Xue / Hua, Wei / Yang, Yuan / Meng, Ze / Hu, Bo / Xin, Jin-Yuan

    Huan jing ke xue= Huanjing kexue

    2020  Volume 41, Issue 9, Page(s) 3908–3917

    Abstract: To understand the characterization and sources of carbonaceous aerosols at Mountain Dinghu, organic carbon (OC) and elemental carbon (EC) in size-resolved aerosol samples were measured at a regional background site in South China using a DRI Model 2001A ... ...

    Abstract To understand the characterization and sources of carbonaceous aerosols at Mountain Dinghu, organic carbon (OC) and elemental carbon (EC) in size-resolved aerosol samples were measured at a regional background site in South China using a DRI Model 2001A analyzer. The average mass concentrations of organic carbon (OC) are (5.6±2.0) μg ·m
    MeSH term(s) Aerosols/analysis ; Air Pollutants/analysis ; Carbon/analysis ; China ; Environmental Monitoring ; Particle Size ; Particulate Matter/analysis ; Seasons
    Chemical Substances Aerosols ; Air Pollutants ; Particulate Matter ; Carbon (7440-44-0)
    Language Chinese
    Publishing date 2020-10-29
    Publishing country China
    Document type Journal Article
    ISSN 0250-3301
    ISSN 0250-3301
    DOI 10.13227/j.hjkx.201911237
    Database MEDical Literature Analysis and Retrieval System OnLINE

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  3. Article: [Concentrations and Size Distributions of Water-soluble Inorganic Ions in Aerosol Particles in Taiyuan, Shanxi].

    Wang, Lu / Wen, Tian-Xue / Miao, Hong-Yan / Gao, Wen-Kang / Wang, Yue-Si

    Huan jing ke xue= Huanjing kexue

    2018  Volume 37, Issue 9, Page(s) 3249–3257

    Abstract: Size-resolved filter samples were collected in Taiyuan every other week from June 2012 to May 2014. The mass concentrations of water-soluble ions ( ... ...

    Abstract Size-resolved filter samples were collected in Taiyuan every other week from June 2012 to May 2014. The mass concentrations of water-soluble ions (Na
    Language Chinese
    Publishing date 2018-06-30
    Publishing country China
    Document type English Abstract ; Journal Article
    ISSN 0250-3301
    ISSN 0250-3301
    DOI 10.13227/j.hjkx.2016.09.002
    Database MEDical Literature Analysis and Retrieval System OnLINE

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  4. Article: [Characteristics of the Size Distribution of Water Soluble Inorganic Ions in Sanya, Hainan].

    Wang, Lu / Liu, Zi-Rui / Wen, Tian-Xue / Miao, Hong-Yan / Wang, Yue-Si

    Huan jing ke xue= Huanjing kexue

    2018  Volume 38, Issue 4, Page(s) 1298–1306

    Abstract: Size-resolved filter samples were collected in Sanya every other week from June 2012 to May 2014. The mass concentrations of water-soluble inorganic ions, including anions ( ... ...

    Abstract Size-resolved filter samples were collected in Sanya every other week from June 2012 to May 2014. The mass concentrations of water-soluble inorganic ions, including anions (Cl
    Language Chinese
    Publishing date 2018-08-02
    Publishing country China
    Document type English Abstract ; Journal Article
    ISSN 0250-3301
    ISSN 0250-3301
    DOI 10.13227/j.hjkx.201608081
    Database MEDical Literature Analysis and Retrieval System OnLINE

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  5. Article ; Online: Observational Insights into Isoprene Secondary Organic Aerosol Formation through the Epoxide Pathway at Three Urban Sites from Northern to Southern China.

    Zhang, Yu-Qing / Ding, Xiang / He, Quan-Fu / Wen, Tian-Xue / Wang, Jun-Qi / Yang, Kong / Jiang, Hao / Cheng, Qian / Liu, Ping / Wang, Zi-Rui / He, Yun-Feng / Hu, Wei-Wei / Wang, Qiao-Yun / Xin, Jin-Yuan / Wang, Yue-Si / Wang, Xin-Ming

    Environmental science & technology

    2022  Volume 56, Issue 8, Page(s) 4795–4805

    Abstract: Isoprene is the most abundant precursor of global secondary organic aerosol (SOA). The epoxide pathway plays a critical role in isoprene SOA (iSOA) formation, in which isoprene epoxydiols (IEPOX) and/or hydroxymethyl-methyl-α-lactone (HMML) can react ... ...

    Abstract Isoprene is the most abundant precursor of global secondary organic aerosol (SOA). The epoxide pathway plays a critical role in isoprene SOA (iSOA) formation, in which isoprene epoxydiols (IEPOX) and/or hydroxymethyl-methyl-α-lactone (HMML) can react with nucleophilic sulfate and water producing isoprene-derived organosulfates (iOSs) and oxygen-containing tracers (iOTs), respectively. This process is complicated and highly influenced by anthropogenic emissions, especially in the polluted urban atmospheres. In this study, we took a 1-year measurement of the paired iOSs and iOTs formed through the IEPOX and HMML pathways at the three urban sites from northern to southern China. The annual average concentrations of iSOA products at the three sites ranged from 14.6 to 36.5 ng m
    MeSH term(s) Aerosols/analysis ; Air Pollutants ; Butadienes ; Epoxy Compounds ; Hemiterpenes ; Pentanes ; Sulfates ; Water
    Chemical Substances Aerosols ; Air Pollutants ; Butadienes ; Epoxy Compounds ; Hemiterpenes ; Pentanes ; Sulfates ; Water (059QF0KO0R) ; isoprene (0A62964IBU)
    Language English
    Publishing date 2022-03-02
    Publishing country United States
    Document type Journal Article ; Research Support, Non-U.S. Gov't
    ISSN 1520-5851
    ISSN (online) 1520-5851
    DOI 10.1021/acs.est.1c06974
    Database MEDical Literature Analysis and Retrieval System OnLINE

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  6. Article: Spatial and seasonal variations of sugars (alcohol) in China: Emerging results from the CARE-China network

    Li, XingRu / Wen, TianXue / Xin, JinYuan / Liu, Zirui / Liu, Shuiqiao / Li, Dong / Zhang, Ruiying / Wang, Yingfeng / Wang, YueSi

    Atmospheric environment. 2019 July 15, v. 209

    2019  

    Abstract: The “Campaign on Atmospheric Aerosol Research” network of China (CARE-China) is a long-term project for the study of the spatio-temporal distributions of physical aerosol characteristics as well as the chemical components and optical properties of ... ...

    Abstract The “Campaign on Atmospheric Aerosol Research” network of China (CARE-China) is a long-term project for the study of the spatio-temporal distributions of physical aerosol characteristics as well as the chemical components and optical properties of aerosols over China. This study presents the size-segregated sugars from the CARE-China network. Sugars associated with size-segregated particulate matter at 8 regions (North China (NC), East China (EC), Northeast China (NE), and Central China (CC), South China (SC), Northwest China (NE), Southwest China (SW) and the Tibetan Plateau (TP)) including 14 sites over China from January 2013 to December 2014 were analyzed via gas chromatography mass spectrometry. Mass concentrations of measured sugars varied considerably with location and season, ranging from 0.20 to 5588 ng m−3, with the majority from levoglucosan (170 ± 207 ngm−3, accounting for 48% of total sugars), followed by sucrose (44.6 ± 39.6 ngm−3, accounting for 11.3% of sugar), and sorbitol (35.5 ± 42.2 ng m−3, accounting for 10.0% of sugars). The highest levels of sugars were observed in urban sites in Central and Southwest China, whereas the lowest concentrations occurred in background and Tibetan Plateau sites. A distinct seasonal variability of sugars was observed, with higher in the winter or autumn and lower during the summer at urban sites. Inconsistent seasonal trends were observed at the background sites located in the higher latitudes, which were characteristic with the highest concentration occurred in spring. Levoglucosan, galactosan and mannosan were found to be dominant in fine size range <1.1 μm, accounting approximately 59% of all size-segregated sugars. Sucrose was enriched in the size range of 3.3–9.0 μm for almost all sampling sites. Concentrations of trehalose and sorbitol in the three size particles were similar. The OC from biomass burning was estimated to be in the range of 0.93–58.7 μg C m−3, with the highest level OCBB% were observed in urban sites in summer and winter. The contributions of biomass burning to OC in the rest of sites were higher in autumn and winter than in spring and summer. Higher OCBB% was observed in spring at the background sites located in Northwest and Northeast China.
    Keywords aerosols ; atmospheric chemistry ; autumn ; biomass ; burning ; gas chromatography-mass spectrometry ; latitude ; optical properties ; particulates ; seasonal variation ; sorbitol ; spatial distribution ; spring ; sucrose ; summer ; trehalose ; urban areas ; winter ; China
    Language English
    Dates of publication 2019-0715
    Size p. 136-143.
    Publishing place Elsevier Ltd
    Document type Article
    ZDB-ID 216368-8
    ISSN 0004-6981 ; 1352-2310
    ISSN 0004-6981 ; 1352-2310
    DOI 10.1016/j.atmosenv.2019.04.029
    Database NAL-Catalogue (AGRICOLA)

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  7. Article: [Seasonal variation of water-soluble ions in PM2.5 at Changbai Mountain].

    Zhao, Ya-Nan / Wang, Yue-Si / Wen, Tian-Xue / Dai, Guan-Hua

    Huan jing ke xue= Huanjing kexue

    2014  Volume 35, Issue 1, Page(s) 9–14

    Abstract: To study seasonal variation of water-soluble ions in PM2.5 at Changbai Mountain. PM2.5 was collected with a high-volume sampler from Jun. 2005 to Dec. 2008, and the concentrations of water-soluble ions were analyzed using ion chromatography. The results ... ...

    Abstract To study seasonal variation of water-soluble ions in PM2.5 at Changbai Mountain. PM2.5 was collected with a high-volume sampler from Jun. 2005 to Dec. 2008, and the concentrations of water-soluble ions were analyzed using ion chromatography. The results showed that the three major ions of SO4(2-), NH4+ and NO3 showed obvious seasonal variation. The mass concentration of SO4(2-) was the highest in summer and lowest in autumn. The mass concentration of NO3- was the highest in winter and lowest in summer. The seasonal variation of NH4+ was influenced by SO4(2-) and NO3-. The total concentrations of water-soluble ions in PM2.5 from different directions were evidently different, following the order of NE < NW < SW, with the average concentrations of 5.43, 7.63 and 10.26 microg x m(-3), respectively. Ca2+ was strongly correlated with CO3(2-), and the correlation(R) was higher in spring (0.74) than that in summer (0.30).
    MeSH term(s) Aerosols/analysis ; Air Pollutants/analysis ; China ; Environmental Monitoring ; Ions/analysis ; Particle Size ; Particulate Matter/analysis ; Seasons ; Water
    Chemical Substances Aerosols ; Air Pollutants ; Ions ; Particulate Matter ; Water (059QF0KO0R)
    Language Chinese
    Publishing date 2014-01
    Publishing country China
    Document type English Abstract ; Journal Article
    ISSN 0250-3301
    ISSN 0250-3301
    Database MEDical Literature Analysis and Retrieval System OnLINE

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  8. Article: [Mass Concentrations and Size Distributions of Water-soluble Inorganic Ions in Atmospheric Aerosols in Beibei District, Chongqing].

    Li, Yan-Pei / Hao, Qing-Ju / Wen, Tian-Xue / Ji, Dong-Sheng / Liu, Zi-Rui / Wang, Yue-Si / Jiang, Chang-Sheng

    Huan jing ke xue= Huanjing kexue

    2018  Volume 39, Issue 9, Page(s) 4002–4013

    Abstract: In order to study the concentration and distribution characteristics of water-soluble inorganic ions in aerosol particles of the Beibei district of Chongqing, aerosol samples were collected with an Andersen cascade impactor between March 2014 and ... ...

    Abstract In order to study the concentration and distribution characteristics of water-soluble inorganic ions in aerosol particles of the Beibei district of Chongqing, aerosol samples were collected with an Andersen cascade impactor between March 2014 and February 2015. Water-soluble inorganic ions, including Na
    Language Chinese
    Publishing date 2018-09-06
    Publishing country China
    Document type English Abstract ; Journal Article
    ISSN 0250-3301
    ISSN 0250-3301
    DOI 10.13227/j.hjkx.201712077
    Database MEDical Literature Analysis and Retrieval System OnLINE

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  9. Article: [Pollution Characteristics of Organic Carbon and Elemental Carbon in Atmospheric Aerosols in Beibei District, Chongqing].

    Peng, Xiao-le / Hao, Qing-Ju / Wen, Tian-Xue / Ji, Dong-Sheng / Liu, Zi-Rui / Wang, Yue-Si / Chen, Jian-Bo / Jiang, Chang-Sheng

    Huan jing ke xue= Huanjing kexue

    2018  Volume 39, Issue 8, Page(s) 3502–3510

    Abstract: To study the pollution characteristics of atmospheric carbon aerosols, aerosol samples were collected via a cascade impactor (Andersen) from March 2014 to February 2015 in Beibei District, Chongqing. Organic carbon (OC) and element carbon (EC) were ... ...

    Abstract To study the pollution characteristics of atmospheric carbon aerosols, aerosol samples were collected via a cascade impactor (Andersen) from March 2014 to February 2015 in Beibei District, Chongqing. Organic carbon (OC) and element carbon (EC) were detected using a DRI 2001A carbon analyzer. The results showed that the annual average concentrations of OC and EC in PM
    Language Chinese
    Publishing date 2018-08-02
    Publishing country China
    Document type English Abstract ; Journal Article
    ISSN 0250-3301
    ISSN 0250-3301
    DOI 10.13227/j.hjkx.201711205
    Database MEDical Literature Analysis and Retrieval System OnLINE

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  10. Article: Observational Insights into Isoprene Secondary Organic Aerosol Formation through the Epoxide Pathway at Three Urban Sites from Northern to Southern China

    Zhang, Yu-Qing / Ding, Xiang / He, Quan-Fu / Wen, Tian-Xue / Wang, Jun-Qi / Yang, Kong / Jiang, Hao / Cheng, Qian / Liu, Ping / Wang, Zi-Rui / He, Yun-Feng / Hu, Wei-Wei / Wang, Qiao-Yun / Xin, Jin-Yuan / Wang, Yue-Si / Wang, Xin-Ming

    Environmental science & technology. 2022 Mar. 02, v. 56, no. 8

    2022  

    Abstract: Isoprene is the most abundant precursor of global secondary organic aerosol (SOA). The epoxide pathway plays a critical role in isoprene SOA (iSOA) formation, in which isoprene epoxydiols (IEPOX) and/or hydroxymethyl-methyl-α-lactone (HMML) can react ... ...

    Abstract Isoprene is the most abundant precursor of global secondary organic aerosol (SOA). The epoxide pathway plays a critical role in isoprene SOA (iSOA) formation, in which isoprene epoxydiols (IEPOX) and/or hydroxymethyl-methyl-α-lactone (HMML) can react with nucleophilic sulfate and water producing isoprene-derived organosulfates (iOSs) and oxygen-containing tracers (iOTs), respectively. This process is complicated and highly influenced by anthropogenic emissions, especially in the polluted urban atmospheres. In this study, we took a 1-year measurement of the paired iOSs and iOTs formed through the IEPOX and HMML pathways at the three urban sites from northern to southern China. The annual average concentrations of iSOA products at the three sites ranged from 14.6 to 36.5 ng m–³. We found that the nucleophilic–addition reaction of isoprene epoxides with water dominated over that with sulfate in the polluted urban air. A simple set of reaction rate constant could not fully describe iOS and iOT formation everywhere. We also found that the IEPOX pathway was dominant over the HMML pathway over urban regions. Using the kinetic data of IEPOX to estimate the reaction parameters of HMML will cause significant underestimation in the importance of HMML pathway. All these findings provide insights into iSOA formation over polluted areas.
    Keywords Lewis bases ; aerosols ; air ; environmental science ; epoxides ; isoprene ; sulfates ; technology ; China
    Language English
    Dates of publication 2022-0302
    Size p. 4795-4805.
    Publishing place American Chemical Society
    Document type Article
    ISSN 1520-5851
    DOI 10.1021/acs.est.1c06974
    Database NAL-Catalogue (AGRICOLA)

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