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Article: Direct Synthesis of MoS

Wu, Zhikang / Li, Feifei / Li, Xiya / Yang, Yang / Huang, Xiao / Li, Hai

2022 Volume 12, Issue 9

Abstract: Due to their unique tubular and spiral structure, graphene and graphene oxide nanoscrolls (GONS) have shown extensive applications in various fields. However, it is still a challenge to improve the optoelectronic application of graphene and GONS because ... ...

Abstract	Due to their unique tubular and spiral structure, graphene and graphene oxide nanoscrolls (GONS) have shown extensive applications in various fields. However, it is still a challenge to improve the optoelectronic application of graphene and GONS because of the zero bandgap of graphene. Herein, ammonium tetrathiomolybdate ((NH
Language	English
Publishing date	2022-05-06
Publishing country	Switzerland
Document type	Journal Article
ZDB-ID	2662255-5
ISSN	2079-4991
ISSN	2079-4991
DOI	10.3390/nano12091581
Database	MEDical Literature Analysis and Retrieval System OnLINE

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Article: Transition Metal Dichalcogenides Nanoscrolls: Preparation and Applications.

Yu, Shilong / Wang, Pinyi / Ye, Huihui / Tang, Hailun / Wang, Siyuan / Wu, Zhikang / Pei, Chengjie / Lu, Junhui / Li, Hai

Nanomaterials (Basel, Switzerland)

2023 Volume 13, Issue 17

Abstract: Two-dimensional (2D) transition metal dichalcogenides (TMDCs) nanosheets have shown extensive applications due to their excellent physical and chemical properties. However, the low light absorption efficiency limits their application in optoelectronics. ... ...

Abstract	Two-dimensional (2D) transition metal dichalcogenides (TMDCs) nanosheets have shown extensive applications due to their excellent physical and chemical properties. However, the low light absorption efficiency limits their application in optoelectronics. By rolling up 2D TMDCs nanosheets, the one-dimensional (1D) TMDCs nanoscrolls are formed with spiral tubular structure, tunable interlayer spacing, and opening ends. Due to the increased thickness of the scroll structure, the light absorption is enhanced. Meanwhile, the rapid electron transportation is confined along the 1D structure. Therefore, the TMDCs nanoscrolls show improved optoelectronic performance compared to 2D nanosheets. In addition, the high specific surface area and active edge site from the bending strain of the basal plane make them promising materials for catalytic reaction. Thus, the TMDCs nanoscrolls have attracted intensive attention in recent years. In this review, the structure of TMDCs nanoscrolls is first demonstrated and followed by various preparation methods of the TMDCs nanoscrolls. Afterwards, the applications of TMDCs nanoscrolls in the fields of photodetection, hydrogen evolution reaction, and gas sensing are discussed.
Language	English
Publishing date	2023-08-27
Publishing country	Switzerland
Document type	Journal Article ; Review
ZDB-ID	2662255-5
ISSN	2079-4991
ISSN	2079-4991
DOI	10.3390/nano13172433
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Article: Comprehensive Analysis of the Differential Expression and Prognostic Value of Histone Deacetylases in Glioma.

Li, Jinwei / Yan, Xianlei / Liang, Cong / Chen, Hongmou / Liu, Meimei / Wu, Zhikang / Zheng, Jiemin / Dang, Junsun / La, Xiaojin / Liu, Quan

Frontiers in cell and developmental biology

2022 Volume 10, Page(s) 840759

Abstract: Gliomas are the most common and aggressive malignancies of the central nervous system. Histone deacetylases (HDACs) are important targets in cancer treatment. They regulate complex cellular mechanisms that influence tumor biology and immunogenicity. ... ...

Abstract	Gliomas are the most common and aggressive malignancies of the central nervous system. Histone deacetylases (HDACs) are important targets in cancer treatment. They regulate complex cellular mechanisms that influence tumor biology and immunogenicity. However, little is known about the function of HDACs in glioma. The Oncomine, Human Protein Atlas, Gene Expression Profiling Interactive Analysis, Broad Institute Cancer Cell Line Encyclopedia, Chinese Glioma Genome Atlas, OmicShare, cBioPortal, GeneMANIA, STRING, and TIMER databases were utilized to analyze the differential expression, prognostic value, and genetic alteration of HDAC and immune cell infiltration in patients with glioma.
Language	English
Publishing date	2022-03-10
Publishing country	Switzerland
Document type	Journal Article
ZDB-ID	2737824-X
ISSN	2296-634X
ISSN	2296-634X
DOI	10.3389/fcell.2022.840759
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Article ; Online: Metallic phase enabling MoS

Chen, Huizhi / He, Xiaojun / Zhou, Zhan / Wu, Zhikang / Li, Hai / Peng, Xinsheng / Zhou, Yubin / Tan, Chaoliang / Shen, Jianliang

Journal of nanobiotechnology

2022 Volume 20, Issue 1, Page(s) 136

Abstract: Two-dimensional (2D) transition metal dichalcogenide (TMD) nanosheets (e.g., ... ...

Abstract	Two-dimensional (2D) transition metal dichalcogenide (TMD) nanosheets (e.g., MoS
MeSH term(s)	Anti-Bacterial Agents/pharmacology ; Bacteria ; Molybdenum/chemistry ; Molybdenum/pharmacology ; Povidone
Chemical Substances	Anti-Bacterial Agents ; Molybdenum (81AH48963U) ; Povidone (FZ989GH94E)
Language	English
Publishing date	2022-03-15
Publishing country	England
Document type	Journal Article
ZDB-ID	2100022-0
ISSN	1477-3155 ; 1477-3155
ISSN (online)	1477-3155
ISSN	1477-3155
DOI	10.1186/s12951-022-01344-6
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Article ; Online: A Novel Necroptosis-Related lncRNA Signature for Predicting Prognosis and Immune Response of Glioma.

Wu, Zhikang / Liu, Meimei / Fu, Jinlong / Li, Jinwei / Qin, Lingyao / Wu, Liuying / Chen, Hongmou / Yan, Xianlei / Liu, Quan / Zheng, Jiemin

BioMed research international

2022 Volume 2022, Page(s) 3742447

Abstract: Glioma is one of the most common intracranial malignancies that plagues people around the world. Despite current improvements in treatment, the prognosis of glioma is often unsatisfactory. Necroptosis is a form of programmed cell death. As research ... ...

Abstract	Glioma is one of the most common intracranial malignancies that plagues people around the world. Despite current improvements in treatment, the prognosis of glioma is often unsatisfactory. Necroptosis is a form of programmed cell death. As research progresses, the role of necroptosis in tumors has gradually attracted the attention of researchers. And lncRNA is regarded as a critical role in the development of cancer. Therefore, this study is aimed at establishing a prognostic model based on necroptosis-associated lncRNAs to accurately assess the prognosis and immune response of patients with glioma. The RNA sequences of glioma patients and normal brain samples were downloaded from The Cancer Genome Atlas (TCGA) and GTEx databases, respectively. The coexpression analysis was performed to identify the necroptosis-related lncRNAs. Then, we utilized LASSO analysis following univariate Cox analysis to construct a prognostic model. Subsequently, we applied the Kaplan-Meier curve, time-dependent receiver operating characteristics (ROC), and univariate and multivariate Cox regression analyses to assess the effectiveness of this model. And the functional enrichment analyses and immune-related analyses were employed to investigate the potential biological functions. A validation set was obtained from the Chinese Glioma Genome Atlas (CGGA) database. And qRT-PCR was employed to further validate the expression levels of selected necroptosis-associated lncRNAs. Seven necroptosis-related lncRNAs (FAM13A-AS1, JMJD1C-AS1, LBX2-AS1, ZBTB20-AS4, HAR1A, SNHG14, and LINC00900) were determined to construct a prognostic model. The area under the ROC curve (AUC) was 0.871, 0.901, and 0.911 at 1, 2, and 3 years, respectively. The risk score was shown to be an important independent predictor in both univariate and multivariate Cox regression analyses. Through functional enrichment analyses, we found that the differentially expressed genes (DEGs) were mainly enriched in protein binding and signaling-related biological functions and immune-associated pathways. In conclusion, we established and validated a novel necroptosis-related lncRNA signature, which could accurately predict the overall survival of glioma patients and serve as potential therapeutic targets.
MeSH term(s)	Biomarkers, Tumor/genetics ; GTPase-Activating Proteins/genetics ; Gene Expression Regulation, Neoplastic ; Glioma/genetics ; Humans ; Immunity ; Jumonji Domain-Containing Histone Demethylases/genetics ; Kaplan-Meier Estimate ; Necroptosis/genetics ; Oxidoreductases, N-Demethylating/genetics ; Oxidoreductases, N-Demethylating/metabolism ; Prognosis ; RNA, Long Noncoding/metabolism
Chemical Substances	Biomarkers, Tumor ; FAM13A protein, human ; GTPase-Activating Proteins ; RNA, Long Noncoding ; JMJD1C protein, human (EC 1.14.11.-) ; Jumonji Domain-Containing Histone Demethylases (EC 1.14.11.-) ; Oxidoreductases, N-Demethylating (EC 1.5.-)
Language	English
Publishing date	2022-06-16
Publishing country	United States
Document type	Journal Article
ZDB-ID	2698540-8
ISSN	2314-6141 ; 2314-6133
ISSN (online)	2314-6141
ISSN	2314-6133
DOI	10.1155/2022/3742447
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Article: An efficient way for the N-formylation of amines by inorganic-ligand supported iron catalysis

Wu, Zhikang / Han, Sheng / Wei, Yongge / Wei, Zheyu / Yu, Han / Zhai, Yongyan / Zhao, Wenshu

Green chemistry. 2020 Feb. 10, v. 22, no. 3

2020

Abstract: The first example of an inorganic-ligand supported iron(iii) catalysed coupling of formic acid and amines to form formamides is reported. The pure inorganic catalyst (NH4)3[FeMo6O18(OH)6] (1), which consists of a central FeIII single-atomic core ... ...

Abstract	The first example of an inorganic-ligand supported iron(iii) catalysed coupling of formic acid and amines to form formamides is reported. The pure inorganic catalyst (NH4)3[FeMo6O18(OH)6] (1), which consists of a central FeIII single-atomic core supported within a cycle-shaped inorganic ligand consisting of six MoVIO6 octahedra, shows excellent activity and selectivity, and avoids the use of complicated/commercially unavailable organic ligands. Various primary amines and secondary amines have been successfully transformed into the corresponding formamides under mild conditions, and the formylation of primary diamines has also been achieved for the first time. The Fe catalyst 1 can be reused several times without appreciable loss of activity.
Keywords	ammonium compounds ; catalysts ; catalytic activity ; diamines ; formic acid ; geometry ; green chemistry ; iron ; ligands ; primary amines ; secondary amines
Language	English
Dates of publication	2020-0210
Size	p. 737-741.
Publishing place	The Royal Society of Chemistry
Document type	Article
ZDB-ID	2006274-6
ISSN	1463-9270 ; 1463-9262
ISSN (online)	1463-9270
ISSN	1463-9262
DOI	10.1039/c9gc03564h
Database	NAL-Catalogue (AGRICOLA)

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Article ; Online: Iron-catalyzed oxidative functionalization of C(sp

Yu, Han / Zhao, Qixin / Wei, Zheyu / Wu, Zhikang / Li, Qi / Han, Sheng / Wei, Yongge

Chemical communications (Cambridge, England)

2019 Volume 55, Issue 54, Page(s) 7840–7843

Abstract: An efficient oxidation and functionalization of C-H bonds with an inorganic-ligand supported iron catalyst and hydrogen peroxide to prepare the corresponding ketones was achieved using the bromide ion as a promoter. Preliminary mechanistic investigations ...

Abstract	An efficient oxidation and functionalization of C-H bonds with an inorganic-ligand supported iron catalyst and hydrogen peroxide to prepare the corresponding ketones was achieved using the bromide ion as a promoter. Preliminary mechanistic investigations indicated that the bromide ion can bind to FeMo
Language	English
Publishing date	2019-06-19
Publishing country	England
Document type	Journal Article
ZDB-ID	1472881-3
ISSN	1364-548X ; 1359-7345 ; 0009-241X
ISSN (online)	1364-548X
ISSN	1359-7345 ; 0009-241X
DOI	10.1039/c9cc03939b
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Article ; Online: Identification of diagnostic genes for both Alzheimer's disease and Metabolic syndrome by the machine learning algorithm.

Li, Jinwei / Zhang, Yang / Lu, Tanli / Liang, Rui / Wu, Zhikang / Liu, Meimei / Qin, Linyao / Chen, Hongmou / Yan, Xianlei / Deng, Shan / Zheng, Jiemin / Liu, Quan

Frontiers in immunology

2022 Volume 13, Page(s) 1037318

Abstract: Background: Alzheimer's disease is the most common neurodegenerative disease worldwide. Metabolic syndrome is the most common metabolic and endocrine disease in the elderly. Some studies have suggested a possible association between MetS and AD, but few ...

Abstract	Background: Alzheimer's disease is the most common neurodegenerative disease worldwide. Metabolic syndrome is the most common metabolic and endocrine disease in the elderly. Some studies have suggested a possible association between MetS and AD, but few studied genes that have a co-diagnostic role in both diseases. Methods: The microarray data of AD (GSE63060 and GSE63061 were merged after the batch effect was removed) and MetS (GSE98895) in the GEO database were downloaded. The WGCNA was used to identify the co-expression modules related to AD and MetS. RF and LASSO were used to identify the candidate genes. Machine learning XGBoost improves the diagnostic effect of hub gene in AD and MetS. The CIBERSORT algorithm was performed to assess immune cell infiltration MetS and AD samples and to investigate the relationship between biomarkers and infiltrating immune cells. The peripheral blood mononuclear cells (PBMCs) single-cell RNA (scRNA) sequencing data from patients with AD and normal individuals were visualized with the Seurat standard flow dimension reduction clustering the metabolic pathway activity changes each cell with ssGSEA. Results: The brown module was identified as the significant module with AD and MetS. GO analysis of shared genes showed that intracellular transport and establishment of localization in cell and organelle organization were enriched in the pathophysiology of AD and MetS. By using RF and Lasso learning methods, we finally obtained eight diagnostic genes, namely Conclusion: We identified genes with common diagnostic effects on both MetS and AD, and found genes involved in multiple metabolic pathways associated with various immune cells.
MeSH term(s)	Humans ; Aged ; Alzheimer Disease/genetics ; Alzheimer Disease/metabolism ; Metabolic Syndrome/genetics ; Neurodegenerative Diseases ; Leukocytes, Mononuclear/metabolism ; Algorithms ; Machine Learning ; Biomarkers ; snRNP Core Proteins
Chemical Substances	Biomarkers ; SNRPG protein, human ; snRNP Core Proteins
Language	English
Publishing date	2022-11-02
Publishing country	Switzerland
Document type	Journal Article ; Research Support, Non-U.S. Gov't
ZDB-ID	2606827-8
ISSN	1664-3224 ; 1664-3224
ISSN (online)	1664-3224
ISSN	1664-3224
DOI	10.3389/fimmu.2022.1037318
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Article ; Online: Defect engineering of layered double hydroxide nanosheets as inorganic photosensitizers for NIR-III photodynamic cancer therapy.

Shen, Weicheng / Hu, Tingting / Liu, Xueyan / Zha, Jiajia / Meng, Fanqi / Wu, Zhikang / Cui, Zhuolin / Yang, Yu / Li, Hai / Zhang, Qinghua / Gu, Lin / Liang, Ruizheng / Tan, Chaoliang

Nature communications

2022 Volume 13, Issue 1, Page(s) 3384

Abstract: Although two-dimensional (2D) layered double hydroxides (LDHs) have been widely used as efficient nanoagents for biological diagnosis and treatment, they have been found to be inert as photosensitizers (PSs) for photodynamic therapy (PDT). Herein, we ... ...

Abstract	Although two-dimensional (2D) layered double hydroxides (LDHs) have been widely used as efficient nanoagents for biological diagnosis and treatment, they have been found to be inert as photosensitizers (PSs) for photodynamic therapy (PDT). Herein, we report the defect engineering of ultrathin 2D CoMo-LDH and NiMo-LDH nanosheets as highly active inorganic PSs for PDT in the third near-infrared (NIR-III) window. Hydrothermal-synthesized 2D CoMo-LDH and NiMo-LDH nanosheets are etched via a simple acid treatment to obtain defect-rich CoMo-LDH and NiMo-LDH nanosheets. Importantly, the defect-rich CoMo-LDH nanosheets exhibit much higher activity (~97 times) for generation of reactive oxygen species than that of the pristine CoMo-LDH nanosheets under a NIR-III 1567 nm laser irradiation. Therefore, after modification with polyethylene glycol, the defect-rich CoMo-LDH nanosheets can be used as an efficient inorganic PS for PDT to efficiently induce cancer cells apoptosis in vitro and eradicate tumors in vivo under 1567 nm laser irradiation.
MeSH term(s)	Humans ; Hydroxides ; Light ; Neoplasms/drug therapy ; Photochemotherapy/methods ; Photosensitizing Agents/pharmacology
Chemical Substances	Hydroxides ; Photosensitizing Agents
Language	English
Publishing date	2022-06-13
Publishing country	England
Document type	Journal Article ; Research Support, Non-U.S. Gov't
ZDB-ID	2553671-0
ISSN	2041-1723 ; 2041-1723
ISSN (online)	2041-1723
ISSN	2041-1723
DOI	10.1038/s41467-022-31106-9
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Article ; Online: Growth of Cu

Zhao, Xinshuo / He, Xiaojun / Hou, Aidi / Cheng, Chunhua / Wang, Xingnan / Yue, Yuanjing / Wu, Zhikang / Wu, Haixia / Liu, Baozhong / Li, Hai / Shen, Jianliang / Tan, Chaoliang / Zhou, Zhan / Ma, Lufang

Inorganic chemistry

2022 Volume 61, Issue 24, Page(s) 9328–9338

Abstract: Two-dimensional (2D) metal-organic framework (MOF) nanosheets have been demonstrated to be promising templates for the growth of various kinds of nanomaterials on their surfaces to construct novel 2D composites, thus realizing enhanced performance in ... ...

Abstract	Two-dimensional (2D) metal-organic framework (MOF) nanosheets have been demonstrated to be promising templates for the growth of various kinds of nanomaterials on their surfaces to construct novel 2D composites, thus realizing enhanced performance in various applications. Herein, we report the growth of Cu
MeSH term(s)	Anti-Bacterial Agents/pharmacology ; Metal-Organic Frameworks/pharmacology ; Metallocenes/pharmacology ; Nanoparticles ; Nanostructures
Chemical Substances	Anti-Bacterial Agents ; Metal-Organic Frameworks ; Metallocenes
Language	English
Publishing date	2022-06-06
Publishing country	United States
Document type	Journal Article
ZDB-ID	1484438-2
ISSN	1520-510X ; 0020-1669
ISSN (online)	1520-510X
ISSN	0020-1669
DOI	10.1021/acs.inorgchem.2c01091
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