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Article ; Online: Spent Lithium-Ion Batteries Derived Co

Zhao, Xinhui / Kuang, Cheng / Liu, Hongshu / An, Chaopeng / Wang, Mingyan / Mu, Tiancheng

ChemSusChem

2024 , Page(s) e202400105

Abstract: Spent lithium-ion batteries (LIBs) are an essential secondary resource containing valuable metal elements. Transforming spent LIBs into efficient catalysts through a simple process presents a promising strategy to address both metal resource scarcity and ...

Abstract	Spent lithium-ion batteries (LIBs) are an essential secondary resource containing valuable metal elements. Transforming spent LIBs into efficient catalysts through a simple process presents a promising strategy to address both metal resource scarcity and clean energy challenges. Herein, a deep eutectic solvent-assisted synthesis of Co
Language	English
Publishing date	2024-03-27
Publishing country	Germany
Document type	Journal Article
ISSN	1864-564X
ISSN (online)	1864-564X
DOI	10.1002/cssc.202400105
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Article: Controllable and facile preparation of Co₉S₈–Ni₃S₂ heterostructures embedded with N,S,O-tri-doped carbon for electrocatalytic oxidation of 5-hydroxymethylfurfural

Zhang, Yibin / Xue, Zhimin / Zhao, Xinhui / Zhang, Baolong / Mu, Tiancheng

Green chemistry. 2022 Feb. 21, v. 24, no. 4

2022

Abstract: Electrochemical oxidation of 5-hydroxymethylfurfural (HMF) into 2,5-furandicarboxylic acid (FDCA) is a highly promising strategy for producing biomass-based valuable chemicals. Exploration of robust and cost-effective electrocatalysts for HMF oxidation ... ...

Abstract	Electrochemical oxidation of 5-hydroxymethylfurfural (HMF) into 2,5-furandicarboxylic acid (FDCA) is a highly promising strategy for producing biomass-based valuable chemicals. Exploration of robust and cost-effective electrocatalysts for HMF oxidation is of significant importance. Here, we proposed a facile and controllable strategy for the preparation of carbon-based heterostructures by direct pyrolysis of rationally designed precursor deep eutectic solvents. The as-prepared Co₉S₈–Ni₃S₂@N,S,O-tri-doped carbon (NSOC) heterostructures exhibit an excellent HMF electrooxidation performance with a conversion of nearly 100%, a Faraday efficiency of 98.6% and a selectivity of 98.8% owing to the unique hollow structure and ternary heterogeneous interface. X-ray photoelectron spectroscopy analysis and theoretical calculations confirm the electron transfer from Ni₃S₂ to NSOC and Co₉S₈ at the heterogeneous interfaces, where hole accumulation on Ni₃S₂ is beneficial for optimizing the HMF electrooxidation reaction (HMF EOR).
Keywords	X-ray photoelectron spectroscopy ; carbon ; cost effectiveness ; electrochemistry ; electron transfer ; green chemistry ; hydroxymethylfurfural ; oxidation ; pyrolysis
Language	English
Dates of publication	2022-0221
Size	p. 1721-1731.
Publishing place	The Royal Society of Chemistry
Document type	Article
ZDB-ID	2006274-6
ISSN	1463-9270 ; 1463-9262
ISSN (online)	1463-9270
ISSN	1463-9262
DOI	10.1039/d1gc04499k
Database	NAL-Catalogue (AGRICOLA)

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Article: Seismic Response Evaluation of High-Steep Slopes Supported by Anti-Slide Piles with Different Initial Damage Based on Shaking Table Test.

Chen, Hongyu / Jiang, Guanlu / Zhao, Xinhui / Zhu, Dan / Liu, Yong / Tian, Hongcheng

Materials (Basel, Switzerland)

2022 Volume 15, Issue 11

Abstract: In order to study the instability development process of the slope reinforced by anti-slide piles under earthquake conditions, the dynamic response characteristics of the slope are usually taken as the main characteristics, and the model test and ... ...

Abstract	In order to study the instability development process of the slope reinforced by anti-slide piles under earthquake conditions, the dynamic response characteristics of the slope are usually taken as the main characteristics, and the model test and numerical simulation are the main research methods. In this paper, a shaking table model test is designed and completed to investigate the influence of anti-slide piles with different initial damage on the failure mode of high and steep slope under earthquake conditions. The changes in velocity, strain and natural frequency during slope vibration are tested in combination with cloud maps when sinusoidal waves of different accelerations with a peak value of 5 Hz are applied. Thus, the differences of slope failure development process and dynamic response characteristics are obtained. The experimental results show that the anti-slide pile with different initial damage has obvious influence on the slope instability process. Under the condition of good anti-slide pile quality, the failure development of the slope behind the pile is limited to soil sliding on top of the slope, slope sliding and overburden sliding; the front slope foot of pile mainly forms shear belt and local sliding. With the decrease in the initial mass of the anti-slide pile, the slope failure develops into topsoil sliding, slope sliding and deep integral sliding; analogously, the failure of the slope in front of the pile develops into a whole slip along the slip belt. The natural frequency cloud map can directly reflect the damage location of the slope, and the frequency change rate is positively correlated with the cumulative shear strain. It shows that the macro-failure characteristics of the model slope change well when the natural frequency is used as the sensitive index to measure the influence of vibration on the model slope. The threshold value of the natural frequency change rate can distinguish different development stages of the slope; 1% is the threshold value of stage II, and 1.5% is the threshold value of stage III.
Language	English
Publishing date	2022-06-03
Publishing country	Switzerland
Document type	Journal Article
ZDB-ID	2487261-1
ISSN	1996-1944
ISSN	1996-1944
DOI	10.3390/ma15113982
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Article ; Online: Comparative Analysis of Efficacy and Prognosis of Hemodialysis and Peritoneal Dialysis for End-Stage Renal Disease: A Meta-analysis.

Lu, Jingyuan / Shi, Danye / Zhao, Xinhui / Xi, Minhui / Qi, Hualin / He, Qiang

publication RETRACTED

Computational and mathematical methods in medicine

2022 Volume 2022, Page(s) 6007698

Abstract: Objective: This meta-analysis is aimed at systematically assessing the efficacy and prognosis of hemodialysis (HD) and peritoneal dialysis (PD) in the treatment of end-stage renal disease (ESRD).: Methods: China National Knowledge Infrastructure, VIP, ...

Abstract	Objective: This meta-analysis is aimed at systematically assessing the efficacy and prognosis of hemodialysis (HD) and peritoneal dialysis (PD) in the treatment of end-stage renal disease (ESRD). Methods: China National Knowledge Infrastructure, VIP, SinoMed, Cochrane Library, PubMed, and Embase databases were searched for relevant studies to evaluate the two different dialysis methods for ESRD. The search time was set from 2010 to 2021. Meta-analysis was performed using Stata16.0. The treatment group received PD, while the control group was given HD. Results: Out of 317 articles initially retrieved, 14 studies were finally included in our meta-analysis. The analysis results showed that there was no marked difference in the 1-year survival rate between the two groups (RR = 1.05; 95% CI: 1.00, 1.10; Conclusion: In summary, both PD and HD can improve renal function in uremic patients, but PD is superior to HD in reducing the incidence of adverse reactions, improving the nutritional status, and therefore improving the quality of life of patients.
MeSH term(s)	Humans ; Kidney Failure, Chronic/therapy ; Peritoneal Dialysis/adverse effects ; Prognosis ; Quality of Life ; Renal Dialysis/adverse effects
Language	English
Publishing date	2022-03-19
Publishing country	United States
Document type	Journal Article ; Meta-Analysis ; Retracted Publication
ZDB-ID	2252430-7
ISSN	1748-6718 ; 1748-670X ; 1027-3662
ISSN (online)	1748-6718
ISSN	1748-670X ; 1027-3662
DOI	10.1155/2022/6007698
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Article ; Online: EZH2-H3K27me3-mediated silencing of mir-139-5p inhibits cellular senescence in hepatocellular carcinoma by activating TOP2A.

Wang, Ke / Jiang, Xunliang / Jiang, Yu / Liu, Jun / Du, Yongtao / Zhang, Zecheng / Li, Yunlong / Zhao, Xinhui / Li, Jipeng / Zhang, Rui

Journal of experimental & clinical cancer research : CR

2023 Volume 42, Issue 1, Page(s) 320

Abstract: Background: Epigenetic alterations play an important role in hepatocellular carcinoma (HCC) development. Enhancer of zeste homolog 2 (EZH2) is a well-known epigenetic modifier that functions as an oncogene in tumors by promoting the H3K27me3-mediated ... ...

Abstract	Background: Epigenetic alterations play an important role in hepatocellular carcinoma (HCC) development. Enhancer of zeste homolog 2 (EZH2) is a well-known epigenetic modifier that functions as an oncogene in tumors by promoting the H3K27me3-mediated transcriptional repression of tumor suppressor genes. "Senescent cells" has been proposed as a possible core component of the hallmarks of cancer conceptualization. Induction of cell senescence and targeted elimination of these senescent tumor cells are new strategies for tumor therapy. However, the role of EZH2 in regulating cellular senescence remains poorly understood. Methods: Bioinformatics analyses suggested that EZH2 and DNA topoisomerase II alpha (TOP2A) are coexpressed in tumors, including HCC. Kyoto Encyclopedia of Genes and Genome (KEGG) pathway enrichment analyses and gene set enrichment analyses (GSEA) suggests a correlation of EZH2 and TOP2A expression with cellular senescence in HCC. MicroRNA (miRNA) inhibitor and mimics, siRNA, PLKO-shRNA, and plenti6.3-miR-139 were used to upregulate or downregulate the expression of target genes. CCK8, EdU, clone formation, and senescence-associated β-galactosidase (SA-β-gal) staining assays were performed to assess cell proliferation and cellular senescence phenotypes. Dual-luciferase reporter and chromatin immunoprecipitation assays were performed to investigate the targeted binding and inhibition of TOP2A 3' untranslated region (UTR) by miR-139-5p and the DNA enrichment of miR139-5p by EZH2 and H3K27me3. BALB/c nude mice were used to establish a xenograft tumor model and verify the phenotypes upon EZH2 and TOP2A silencing and miR-139 overexpression in vivo. In addition, tissue microarrays were used to analyze the expression patterns and correlations among EZH2, TOP2A, and miR-139-5p expression in HCC. Results: Bioinformatics analysis revealed that EZH2 and TOP2A are coexpressed in HCC. In vitro gain- and loss-of-function experiments showed that inhibition of EZH2 and TOP2A induces cellular senescence and inhibits proliferation of HCC cells. In vivo tumorigenesis assays indicated that EZH2 and TOP2A knockdown inhibits tumorigenesis by inducing cellular senescence. Mechanistically, EZH2 promotes TOP2A expression by regulating the H3K27me3-mediated epigenetic silencing of miR-139-5p. TOP2A is a direct target of miR-139-5p, and inhibition of miR-139-5p can reverse the promotion by EZH2 of TOP2A expression. The overexpression of miR-139-5p induces cellular senescence and inhibits proliferation of HCC cells both in vitro and in vivo. Clinically, expression of EZH2 and TOP2A are higher in HCC tissues than in normal tissues, and this high coexpression indicates a worse outcome of patients with HCC. Moreover, expression of EZH2 and TOP2A is significantly correlated with tumor differentiation grade, tumor invasion, and TNM stage in HCC. miR-139-5p expression is lower in HCC tumors than in normal tissues and is correlated with better prognosis of HCC patients. Conclusions: Our study revealed the role of the EZH2/miR-139-5p/TOP2A axis in regulating cellular senescence and cell proliferation in HCC, enriching the molecular mechanisms of EZH2-mediated epigenetic regulation in HCC. Therefore, our results provide insight into the therapeutic potential of targeting EZH2 to induce cellular senescence and then destroy senescent cells for HCC.
MeSH term(s)	Animals ; Humans ; Mice ; Carcinogenesis/genetics ; Carcinoma, Hepatocellular/pathology ; Cell Line, Tumor ; Cell Proliferation/genetics ; Cellular Senescence/genetics ; DNA Topoisomerases, Type II/genetics ; DNA Topoisomerases, Type II/metabolism ; Enhancer of Zeste Homolog 2 Protein/genetics ; Enhancer of Zeste Homolog 2 Protein/metabolism ; Epigenesis, Genetic ; Gene Expression Regulation, Neoplastic ; Histones/metabolism ; Liver Neoplasms/pathology ; Mice, Nude ; MicroRNAs/genetics ; MicroRNAs/metabolism
Chemical Substances	DNA Topoisomerases, Type II (EC 5.99.1.3) ; Enhancer of Zeste Homolog 2 Protein (EC 2.1.1.43) ; EZH2 protein, human (EC 2.1.1.43) ; Histones ; MicroRNAs ; MIRN139 microRNA, human ; TOP2A protein, human (EC 5.99.1.3)
Language	English
Publishing date	2023-11-27
Publishing country	England
Document type	Journal Article
ZDB-ID	803138-1
ISSN	1756-9966 ; 0392-9078
ISSN (online)	1756-9966
ISSN	0392-9078
DOI	10.1186/s13046-023-02855-2
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Zs.A 2065: Show issues

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Jg. 1995 - 2021: Lesesall (1.OG)
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Article ; Online: Enhanced sensitivity and durability in photodetector of Ag/nanocellulose/Si via plasma-assisted synthesis.

Su, Nan / Xu, Kun / Yu, Xinna / Liu, Shuai / Zhao, Xinhui / Hu, Su / Bao, Peng / Niu, Yiru / Wang, Hui

Optics letters

2023 Volume 48, Issue 13, Page(s) 3531–3534

Abstract: Position-sensitive detectors (PSDs) based on the lateral photovoltaic effect (LPE) are widely used for precision displacement and angle measurement. However, high temperatures can lead to the thermal decomposition or oxidation of nanomaterials frequently ...

Abstract	Position-sensitive detectors (PSDs) based on the lateral photovoltaic effect (LPE) are widely used for precision displacement and angle measurement. However, high temperatures can lead to the thermal decomposition or oxidation of nanomaterials frequently utilized in PSDs, and can ultimately affect the performance. In this study, we present a PSD based on Ag/nanocellulose/Si that maintains a maximum sensitivity of 416.52 mV/mm, even at elevated temperatures. By encapsulating nanosilver in a nanocellulose matrix, the device demonstrates excellent stability and performance over a wide temperature range from 300 to 450 K. Its performance can be comparable to that of room temperature PSDs. An approach that uses nanometals to regulate optical absorption and the local electric field overcomes carrier recombination due to nanocellulose, enabling a breakthrough in sensitivity for organic PSDs. The results indicate that the LPE in this structure is dominated by local surface plasmon resonance, presenting opportunities for expanding optoelectronics in high-temperature industrial environments and monitoring applications. The proposed PSD offers a simple, fast, and cost-effective solution for real-time laser beam monitoring, and its high-temperature stability makes it ideal for a wide range of industrial applications.
MeSH term(s)	Electricity ; Nanostructures ; Surface Plasmon Resonance
Language	English
Publishing date	2023-06-30
Publishing country	United States
Document type	Journal Article
ISSN	1539-4794
ISSN (online)	1539-4794
DOI	10.1364/OL.494776
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Article ; Online: Photoinduced Nonvolatile Resistive Switching Behavior in Oxygen-Doped MoS

Chang, Ke / Zhao, Xinhui / Yu, Xinna / Gan, Zhikai / Wang, Renzhi / Dong, Anhua / Zhao, Zhuyikang / Zhang, Yafei / Wang, Hui

Nano letters

2023 Volume 23, Issue 17, Page(s) 8288–8294

Abstract: Controlling resistance by external fields provides fascinating opportunities for the development of novel devices and circuits, such as temperature-field-induced superconductors, magnetic-field-triggered giant magnetoresistance devices, and electric- ... ...

Abstract	Controlling resistance by external fields provides fascinating opportunities for the development of novel devices and circuits, such as temperature-field-induced superconductors, magnetic-field-triggered giant magnetoresistance devices, and electric-field-operated flash memories. In this work, we demonstrate a light-triggered nonvolatile resistive switching behavior in oxygen-doped MoS
Language	English
Publishing date	2023-08-23
Publishing country	United States
Document type	Journal Article
ISSN	1530-6992
ISSN (online)	1530-6992
DOI	10.1021/acs.nanolett.3c02499
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Article: Upgrading of levulinic acid into diverse N-containing functional chemicals

Xue, Zhimin / Mu, Tiancheng / Yu, Dongkun / Zhao, Xinhui

Green chemistry. 2019 Oct. 14, v. 21, no. 20

2019

Abstract: Levulinic acid (LA), one of the top 10 most promising biomass-derived platform molecules, is a versatile compound, and can be transformed into diverse value-added chemicals. In the valorization of LA to various valuable chemicals, conversion of LA into N- ...

Abstract	Levulinic acid (LA), one of the top 10 most promising biomass-derived platform molecules, is a versatile compound, and can be transformed into diverse value-added chemicals. In the valorization of LA to various valuable chemicals, conversion of LA into N-containing functional chemicals is an emerging and rapidly developing topic. For the synthesis of N-containing functional chemicals using LA as the building block, significant progress had been achieved in recent years and further progress would be achieved in the near future. This review article focused on the selective conversion of LA into a series of N-containing chemicals by fully considering the molecular structure of LA. A reasonable outlook is provided in the last section to highlight the challenges and opportunities for upgrading of LA to various N-containing functional chemicals.
Keywords	chemical structure ; green chemistry ; levulinic acid ; value added
Language	English
Dates of publication	2019-1014
Size	p. 5449-5468.
Publishing place	The Royal Society of Chemistry
Document type	Article
ZDB-ID	2006274-6
ISSN	1463-9270 ; 1463-9262
ISSN (online)	1463-9270
ISSN	1463-9262
DOI	10.1039/c9gc02415h
Database	NAL-Catalogue (AGRICOLA)

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Article ; Online: Eutectic Synthesis of High-Entropy Metal Phosphides for Electrocatalytic Water Splitting.

Zhao, Xinhui / Xue, Zhimin / Chen, Wenjun / Wang, Yaqing / Mu, Tiancheng

ChemSusChem

2020 Volume 13, Issue 8, Page(s) 2038–2042

Abstract: High-entropy materials, a new class of alloys that incorporate five or more principal elements into single-phase crystal structures, have received considerable interest in materials science and engineering. Considering the tailored composition and ... ...

Abstract	High-entropy materials, a new class of alloys that incorporate five or more principal elements into single-phase crystal structures, have received considerable interest in materials science and engineering. Considering the tailored composition and disordered configuration, these high-entropy materials may arouse functional synergism towards electrocatalysis. Here, a new strategy for preparing high-entropy metal phosphides (HEMPs) was developed by a eutectic solvent method. The as-prepared HEMP possessed a single metal phosphide phase with up to five homogenously distributed metal components. The versatile application of high-entropy materials was highlighted by integrating the HEMP catalyst into a two-electrode configuration for electrocatalytic water splitting.
Language	English
Publishing date	2020-03-03
Publishing country	Germany
Document type	Journal Article
ISSN	1864-564X
ISSN (online)	1864-564X
DOI	10.1002/cssc.202000173
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Article ; Online: Eutectic Molecular Liquids Based on Hydrogen Bonding and π-π Interaction for Exfoliating Two-dimensional Materials and Recycling Polymers.

Yu, Dongkun / Mou, Hongyu / Zhao, Xinhui / Wang, Yaqing / Mu, Tiancheng

Chemistry, an Asian journal

2019 Volume 14, Issue 19, Page(s) 3350–3356

Abstract: Eutectic molecular liquids (EMLs) based on hydrogen-bonding interaction and π-π stacking were prepared. We found that the thermodynamic properties like initial decomposition temperature and glass transition temperature of EMLs are mainly dominated by the ...

Abstract	Eutectic molecular liquids (EMLs) based on hydrogen-bonding interaction and π-π stacking were prepared. We found that the thermodynamic properties like initial decomposition temperature and glass transition temperature of EMLs are mainly dominated by the hydrogen bond donor, which is beneficial for designing and preparing new EMLs. These new liquid systems could be applied in the field of environmental and material science.
Language	English
Publishing date	2019-09-05
Publishing country	Germany
Document type	Journal Article
ISSN	1861-471X
ISSN (online)	1861-471X
DOI	10.1002/asia.201900990
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