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  1. Article ; Online: Solvent-Free CO

    Legrand, L / Schaetzle, O / de Kler, R C F / Hamelers, H V M

    Environmental science & technology

    2018  Volume 52, Issue 16, Page(s) 9478–9485

    Abstract: Capture of ... ...

    Abstract Capture of CO
    MeSH term(s) Adsorption ; Carbon Dioxide ; Electrodes ; Ions ; Water Purification
    Chemical Substances Ions ; Carbon Dioxide (142M471B3J)
    Language English
    Publishing date 2018-08-10
    Publishing country United States
    Document type Journal Article ; Research Support, Non-U.S. Gov't
    ISSN 1520-5851
    ISSN (online) 1520-5851
    DOI 10.1021/acs.est.8b00980
    Database MEDical Literature Analysis and Retrieval System OnLINE

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  2. Article ; Online: Solvent-Free CO2 Capture Using Membrane Capacitive Deionization

    Legrand, L. / Schaetzle, O. / De Kler, R.C.F. / Hamelers, H.V.M.

    Environmental Science and Technology

    2018  Volume 52, Issue 16

    Abstract: Capture of CO2, originating from both fossil fuels, such as coal combustion, and from renewables, such as biogas, appears to be one of the greatest technological challenges of this century. In this study, we show that membrane capacitive deionization ( ... ...

    Abstract Capture of CO2, originating from both fossil fuels, such as coal combustion, and from renewables, such as biogas, appears to be one of the greatest technological challenges of this century. In this study, we show that membrane capacitive deionization (MCDI) can be used to capture CO2 as bicarbonate and carbonate ions produced from the reaction of CO2 with water. This novel approach allows capturing CO2 at room temperature and atmospheric pressure without the use of chemicals. In this process, the adsorption and desorption of bicarbonate ions from the deionized water solution drive the CO2(g) absorption-desorption from the gas phase. In this work, the effects of the current density and the CO2 partial pressure were studied. We found that between 55 and 75% of the electrical charge of the capacitive electrodes can be directly used to absorb CO2 gas. The energy requirement of such a system was found to be ∼40 kJ mol-1 at 15% CO2 and could be further improved by reducing the ohmic and non-ohmic energy losses of the MCDI cell.
    Keywords Life Science
    Subject code 660
    Language English
    Publishing country nl
    Document type Article ; Online
    ISSN 0013-936X
    Database BASE - Bielefeld Academic Search Engine (life sciences selection)

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    Order via subito

    This service is chargeable due to the Delivery terms set by subito. Orders including an article and supplementary material will be classified as separate orders. In these cases, fees will be demanded for each order.

    Inter-library loan at ZB MED

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