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  1. Artikel ; Online: Coherence protection of spin qubits in hexagonal boron nitride.

    Ramsay, Andrew J / Hekmati, Reza / Patrickson, Charlie J / Baber, Simon / Arvidsson-Shukur, David R M / Bennett, Anthony J / Luxmoore, Isaac J

    Nature communications

    2023  Band 14, Heft 1, Seite(n) 461

    Abstract: Spin defects in foils of hexagonal boron nitride are an attractive platform for magnetic field imaging, since the probe can be placed in close proximity to the target. However, as a III-V material the electron spin coherence is limited by the nuclear ... ...

    Abstract Spin defects in foils of hexagonal boron nitride are an attractive platform for magnetic field imaging, since the probe can be placed in close proximity to the target. However, as a III-V material the electron spin coherence is limited by the nuclear spin environment, with spin echo coherence times of ∽100 ns at room temperature accessible magnetic fields. We use a strong continuous microwave drive with a modulation in order to stabilize a Rabi oscillation, extending the coherence time up to ∽ 4μs, which is close to the 10 μs electron spin lifetime in our sample. We then define a protected qubit basis, and show full control of the protected qubit. The coherence times of a superposition of the protected qubit can be as high as 0.8 μs. This work establishes that boron vacancies in hexagonal boron nitride can have electron spin coherence times that are competitive with typical nitrogen vacancy centres in small nanodiamonds under ambient conditions.
    Sprache Englisch
    Erscheinungsdatum 2023-01-28
    Erscheinungsland England
    Dokumenttyp Journal Article
    ZDB-ID 2553671-0
    ISSN 2041-1723 ; 2041-1723
    ISSN (online) 2041-1723
    ISSN 2041-1723
    DOI 10.1038/s41467-023-36196-7
    Datenquelle MEDical Literature Analysis and Retrieval System OnLINE

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  2. Buch ; Online: High Frequency Magnetometry with an Ensemble of Spin Qubits in Hexagonal Boron Nitride

    Patrickson, Charlie J. / Baber, Simon / Gaál, Blanka B. / Ramsay, Andrew J. / Luxmoore, Isaac J.

    2023  

    Abstract: Sensors based on spin qubits in 2D crystals offer the prospect of nanoscale sensing volumes, where the close proximity of the sensor and source could provide access to otherwise inaccessible signals. For AC magnetometry, the sensitivity and frequency ... ...

    Abstract Sensors based on spin qubits in 2D crystals offer the prospect of nanoscale sensing volumes, where the close proximity of the sensor and source could provide access to otherwise inaccessible signals. For AC magnetometry, the sensitivity and frequency range is typically limited by the noise spectrum, which determines the qubit coherence time. This poses a problem for III-V materials, as the non-zero spin of the host nuclei introduces a considerable source of magnetic noise. Here, we overcome this with a sensing protocol based on phase modulated continuous concatenated dynamic decoupling, which extends the coherence time towards the $T_1$ limit at room temperature and enables tuneable narrowband AC magnetometry. We demonstrate the protocol with an ensemble of negatively charged boron vacancies in hexagonal boron nitride, detecting in-plane AC fields within $\pm 150~\mathrm{MHz}$ of the electron spin resonance, and out-of-plane fields in the range of $\sim10-150~\mathrm{MHz}$. We measure an AC magnetic field sensitivity of $\sim1~\mathrm{\mu T/\sqrt{Hz}}$ at $\sim2.5~\mathrm{GHz}$, for a sensor volume of $\sim0.1~\mathrm{\mu m^3}$, and demonstrate that the sensor can reconstruct the AC magnetic field from a wire loop antenna. This work establishes the viability of spin defects in 2D materials for high frequency magnetometry, demonstrating sensitivities that are comparable to nitrogen vacancy centres in diamond for microscopic sensing volumes, and with wide-ranging applications across science and technology.
    Schlagwörter Condensed Matter - Materials Science
    Thema/Rubrik (Code) 530
    Erscheinungsdatum 2023-06-15
    Erscheinungsland us
    Dokumenttyp Buch ; Online
    Datenquelle BASE - Bielefeld Academic Search Engine (Lebenswissenschaftliche Auswahl)

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  3. Artikel ; Online: Excited State Spectroscopy of Boron Vacancy Defects in Hexagonal Boron Nitride Using Time-Resolved Optically Detected Magnetic Resonance.

    Baber, Simon / Malein, Ralph Nicholas Edward / Khatri, Prince / Keatley, Paul Steven / Guo, Shi / Withers, Freddie / Ramsay, Andrew J / Luxmoore, Isaac J

    Nano letters

    2021  Band 22, Heft 1, Seite(n) 461–467

    Abstract: We report optically detected magnetic resonance (ODMR) measurements of an ensemble of spin-1 negatively charged boron vacancies in hexagonal boron nitride. The photoluminescence decay rates are spin-dependent, with intersystem crossing rates of 1.02 ... ...

    Abstract We report optically detected magnetic resonance (ODMR) measurements of an ensemble of spin-1 negatively charged boron vacancies in hexagonal boron nitride. The photoluminescence decay rates are spin-dependent, with intersystem crossing rates of 1.02 ns
    Sprache Englisch
    Erscheinungsdatum 2021-12-27
    Erscheinungsland United States
    Dokumenttyp Journal Article
    ISSN 1530-6992
    ISSN (online) 1530-6992
    DOI 10.1021/acs.nanolett.1c04366
    Datenquelle MEDical Literature Analysis and Retrieval System OnLINE

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  4. Buch ; Online: Room temperature coherent control of protected qubit in hexagonal boron nitride

    Ramsay, Andrew J. / Hekmati, Reza / Patrickson, Charlie J. / Baber, Simon / Arvidsson-Shukur, David R. M. / Bennett, Anthony J. / Luxmoore, Isaac J.

    2022  

    Abstract: Spin defects in foils of hexagonal boron nitride are an attractive platform for magnetic field imaging, since the probe can be placed in close proximity to the target. However, as a III-V material the electron spin coherence is limited by the nuclear ... ...

    Abstract Spin defects in foils of hexagonal boron nitride are an attractive platform for magnetic field imaging, since the probe can be placed in close proximity to the target. However, as a III-V material the electron spin coherence is limited by the nuclear spin environment, with spin echo coherence time of $\sim100~\mathrm{ns}$ at room temperature accessible magnetic fields. We use a strong continuous microwave drive with a modulation in order to stabilize a Rabi oscillation, extending the coherence time up to $\sim4~\mathrm{\mu s}$, which is close to the 10-$\mathrm{\mu s}$ electron spin lifetime in our sample. We then define a protected qubit basis, and show full control of the protected qubit. The coherence times of a superposition of the protected qubit can be as high as $0.8~\mathrm{\mu s}$. This work establishes that boron vacancies in hexagonal boron nitride can have electron spin coherence times that are competitive with typical NV-centers in small nanodiamonds under ambient conditions.
    Schlagwörter Condensed Matter - Materials Science
    Thema/Rubrik (Code) 530
    Erscheinungsdatum 2022-05-25
    Erscheinungsland us
    Dokumenttyp Buch ; Online
    Datenquelle BASE - Bielefeld Academic Search Engine (Lebenswissenschaftliche Auswahl)

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