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  1. Artikel ; Online: Oxidation of tetracycline hydrochloride with a photoenhanced MIL-101(Fe)/g-C3N4/PMS system

    Jianjun Song / Xiaoying Yuan / Meikun Sun / Zuchen Wang / Gege Cao / Kangqi Gao / Chuanxi Yang / Fengmei Zhang / Feng Dang / Weiliang Wang

    Ecotoxicology and Environmental Safety, Vol 251, Iss , Pp 114524- (2023)

    Synergetic effects and radical/nonradical pathways

    2023  

    Abstract: MIL-101(Fe)-based catalysts have been widely used for degradation of organic pollutants based on peroxymonosulfate (PMS) activation. Hence, a facile calcination and hydrothermal method was used in this study to prepare a MIL-101(Fe)/g-C3N4 composite ... ...

    Abstract MIL-101(Fe)-based catalysts have been widely used for degradation of organic pollutants based on peroxymonosulfate (PMS) activation. Hence, a facile calcination and hydrothermal method was used in this study to prepare a MIL-101(Fe)/g-C3N4 composite catalyst with high activity and high stability for PMS activation to degrade tetracycline hydrochloride (TC) under visible-light irradiation. We clearly elucidated the mechanism involved in the MIL-101(Fe)/g-C3N4 photo Fenton-catalyzed PMS activation process by separating the PMS activation and pollutant oxidation processes. The synergetic effects of MIL-101(Fe) and g-C3N4 involved MIL-101(Fe) acting as an electron shuttle mediating electron transfer from the organic substrate to PMS, accompanied by redox cycling of the surface Fe(II)/Fe(III). Multiple experimental results indicated that PMS was bound to the surface of MIL-101(Fe)/g-C3N4 during visible irradiation and generation of sulfate radicals (SO4•-), hydroxyl radicals (•OH) and superoxide anion free radicals (•O2-) for the radical pathway and singlet oxygen (1O2) and holes (h+) for the nonradical pathway. The major degradation pathways for TC can be described as demethylation, deamination, deamidation and carbonylation. This work provides valuable information and advances the fundamental understanding needed for design and syntheses of metal-free conjugated polymers modified by metal-organic frameworks for heterogeneous photo-Fenton reactions.
    Schlagwörter Photo-Fenton process ; MIL-101(Fe)/g-C3N4 catalyst ; Peroxymonosulfate activation ; Water treatment ; Environmental pollution ; TD172-193.5 ; Environmental sciences ; GE1-350
    Thema/Rubrik (Code) 540
    Sprache Englisch
    Erscheinungsdatum 2023-02-01T00:00:00Z
    Verlag Elsevier
    Dokumenttyp Artikel ; Online
    Datenquelle BASE - Bielefeld Academic Search Engine (Lebenswissenschaftliche Auswahl)

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  2. Artikel ; Online: Nuclear import of Mas-related G protein-coupled receptor member D induces pathological cardiac remodeling

    Kun Zhao / Dongxu Hua / Chuanxi Yang / Xiaoguang Wu / Yukang Mao / Yanhui Sheng / Wei Sun / Yong Li / Xiangqing Kong / Peng Li

    Cell Communication and Signaling, Vol 21, Iss 1, Pp 1-

    2023  Band 19

    Abstract: Abstract Alamandine (Ala), a ligand of Mas-related G protein-coupled receptor, member D (MrgD), alleviates angiotensin II (AngII)-induced cardiac hypertrophy. However, the specific physiological and pathological role of MrgD is not yet elucidated. Here, ... ...

    Abstract Abstract Alamandine (Ala), a ligand of Mas-related G protein-coupled receptor, member D (MrgD), alleviates angiotensin II (AngII)-induced cardiac hypertrophy. However, the specific physiological and pathological role of MrgD is not yet elucidated. Here, we found that MrgD expression increased under various pathological conditions. Then, MrgD knockdown prevented AngII-induced cardiac hypertrophy and fibrosis via inactivating Gαi-mediacted downstream signaling pathways, including the phosphorylation of p38 (p-P38), while MrgD overexpression induced pathological cardiac remodeling. Next, Ala, like silencing MrgD, exerted its cardioprotective effects by inhibiting Ang II-induced nuclear import of MrgD. MrgD interacted with p-P38 and promoted its entry into the nucleus under Ang II stimulation. Our results indicated that Ala was a blocking ligand of MrgD that inhibited downstream signaling pathway, which unveiled the promising cardioprotective effect of silencing MrgD expression on alleviating cardiac remodeling. Video Abstract
    Schlagwörter Cardiac remodeling ; Alamandine ; Mas-related G protein-coupled receptor ; Member D ; Nuclear import ; Gαi subunit ; Medicine ; R ; Cytology ; QH573-671
    Sprache Englisch
    Erscheinungsdatum 2023-07-01T00:00:00Z
    Verlag BMC
    Dokumenttyp Artikel ; Online
    Datenquelle BASE - Bielefeld Academic Search Engine (Lebenswissenschaftliche Auswahl)

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  3. Artikel ; Online: A Set of Global Metabolomic Biomarker Candidates to Predict the Risk of Dry Eye Disease

    Yaping Jiang / Chuanxi Yang / Yuxiang Zheng / Yining Liu / Yihui Chen

    Frontiers in Cell and Developmental Biology, Vol

    2020  Band 8

    Abstract: PurposeWe used ultraperformance liquid chromatography coupled with quadrupole/time-of-flight tandem mass spectrometry (UPLC-Q/TOF-MS/MS) to analyze the metabolic profile of reflex tears obtained from patients with dry eye disorders.MethodsWe performed a ... ...

    Abstract PurposeWe used ultraperformance liquid chromatography coupled with quadrupole/time-of-flight tandem mass spectrometry (UPLC-Q/TOF-MS/MS) to analyze the metabolic profile of reflex tears obtained from patients with dry eye disorders.MethodsWe performed a cross-sectional study involving 113 subjects: 85 patients diagnosed with dry eye syndrome (dry eye group) and 28 healthy volunteers (control group). Reflex tears (20–30 μl) were collected from the tear meniscus of both eyes of each subject using a Schirmer I test strip. MS data were acquired with a standard workflow by UPLC-Q/TOF-MS/MS. Metabolites were quantitatively analyzed and matched with entries in the Metlin, Massbank, and HMDB databases. Least absolute shrinkage and selection operator (LASSO) regression was conducted to detect important metabolites. Multiple logistic regression was used to identify the significant metabolic biomarker candidates for dry eye syndrome. Open database sources, including the Kyoto Encyclopedia of Genes and Genomes and MetaboAnalyst, were used to identify metabolic pathways.ResultsAfter the LASSO regression and multiple logistic regression analysis, 4 of 20 metabolic biomarker candidates were significantly correlated with Ocular Surface Disease Index score, 42 of 57 with fluorescein breakup time, and 26 of 57 with fluorescein staining. By focusing on the overlap of these three sets, 48 of 51 metabolites contributed to the incidence of dry eye and there were obvious changes in different age groups. Metabolic pathway analysis revealed that the main pathways were glucose metabolism, amino acid metabolism, and glutathione metabolism.ConclusionDry eye syndrome induces changes in the metabolic profile of tears, and the trend differs with age. This evidence reveals the relationship between changes in metabolites, symptoms of dry eye syndrome, and age.
    Schlagwörter metabolomic ; dry eye disease ; least absolute shrinkage and selection operator (LASSO) regression ; tear profile ; glucose metabolism ; Glutathione metabolism ; Biology (General) ; QH301-705.5
    Thema/Rubrik (Code) 570
    Sprache Englisch
    Erscheinungsdatum 2020-06-01T00:00:00Z
    Verlag Frontiers Media S.A.
    Dokumenttyp Artikel ; Online
    Datenquelle BASE - Bielefeld Academic Search Engine (Lebenswissenschaftliche Auswahl)

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  4. Artikel ; Online: Comprehensive Analysis of the Transcriptome-Wide m6A Methylome in Pterygium by MeRIP Sequencing

    Yaping Jiang / Xin Zhang / Xiaoyan Zhang / Kun Zhao / Jing Zhang / Chuanxi Yang / Yihui Chen

    Frontiers in Cell and Developmental Biology, Vol

    2021  Band 9

    Abstract: AimPterygium is a common ocular surface disease, which is affected by a variety of factors. Invasion of the cornea can cause severe vision loss. N6-methyladenosine (m6A) is a common post-transcriptional modification of eukaryotic mRNA, which can regulate ...

    Abstract AimPterygium is a common ocular surface disease, which is affected by a variety of factors. Invasion of the cornea can cause severe vision loss. N6-methyladenosine (m6A) is a common post-transcriptional modification of eukaryotic mRNA, which can regulate mRNA splicing, stability, nuclear transport, and translation. To our best knowledge, there is no current research on the mechanism of m6A in pterygium.MethodsWe obtained 24 pterygium tissues and 24 conjunctival tissues from each of 24 pterygium patients recruited from Shanghai Yangpu Hospital, and the level of m6A modification was detected using an m6A RNA Methylation Quantification Kit. Expression and location of METTL3, a key m6A methyltransferase, were identified by immunostaining. Then we used m6A-modified RNA immunoprecipitation sequencing (MeRIP-seq), RNA sequencing (RNA-seq), and bioinformatics analyses to compare the differential expression of m6A methylation in pterygium and normal conjunctival tissue.ResultsWe identified 2,949 dysregulated m6A peaks in pterygium tissue, of which 2,145 were significantly upregulated and 804 were significantly downregulated. The altered m6A peak of genes were found to play a key role in the Hippo signaling pathway and endocytosis. Joint analyses of MeRIP-seq and RNA-seq data identified 72 hypermethylated m6A peaks and 15 hypomethylated m6A peaks in mRNA. After analyzing the differentially methylated m6A peaks and synchronously differentially expressed genes, we searched the Gene Expression Omnibus database and identified five genes related to the development of pterygium (DSP, MXRA5, ARHGAP35, TMEM43, and OLFML2A).ConclusionOur research shows that m6A modification plays an important role in the development of pterygium and can be used as a potential new target for the treatment of pterygium in the future.
    Schlagwörter pterygium ; m6A ; MeRIP sequencing ; methyltransferase 3 ; Hippo signaling pathway ; GEO ; Biology (General) ; QH301-705.5
    Thema/Rubrik (Code) 570
    Sprache Englisch
    Erscheinungsdatum 2021-06-01T00:00:00Z
    Verlag Frontiers Media S.A.
    Dokumenttyp Artikel ; Online
    Datenquelle BASE - Bielefeld Academic Search Engine (Lebenswissenschaftliche Auswahl)

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  5. Artikel ; Online: Highly efficient UV/H2O2 technology for the removal of nifedipine antibiotics

    Wenping Dong / Chuanxi Yang / Lingli Zhang / Qiang Su / Xiaofeng Zou / Wenfeng Xu / Xingang Gao / Kang Xie / Weiliang Wang

    PLoS ONE, Vol 16, Iss

    Kinetics, co-existing anions and degradation pathways

    2021  Band 10

    Abstract: This study investigates the degradation of nifedipine (NIF) by using a novel and highly efficient ultraviolet light combined with hydrogen peroxide (UV/H2O2). The degradation rate and degradation kinetics of NIF first increased and then remained constant ...

    Abstract This study investigates the degradation of nifedipine (NIF) by using a novel and highly efficient ultraviolet light combined with hydrogen peroxide (UV/H2O2). The degradation rate and degradation kinetics of NIF first increased and then remained constant as the H2O2 dose increased, and the quasi-percolation threshold was an H2O2 dose of 0.378 mmol/L. An increase in the initial pH and divalent anions (SO42- and CO32-) resulted in a linear decrease of NIF (the R2 of the initial pH, SO42- and CO32- was 0.6884, 0.9939 and 0.8589, respectively). The effect of monovalent anions was complex; Cl- and NO3- had opposite effects: low Cl- or high NO3- promoted degradation, and high Cl- or low NO3- inhibited the degradation of NIF. The degradation rate and kinetics constant of NIF via UV/H2O2 were 99.94% and 1.45569 min-1, respectively, and the NIF concentration = 5 mg/L, pH = 7, the H2O2 dose = 0.52 mmol/L, T = 20 ℃ and the reaction time = 5 min. The ·OH was the primary key reactive oxygen species (ROS) and ·O2- was the secondary key ROS. There were 11 intermediate products (P345, P329, P329-2, P315, P301, P274, P271, P241, P200, P181 and P158) and 2 degradation pathways (dehydrogenation of NIF → P345 → P274 and dehydration of NIF → P329 → P315).
    Schlagwörter Medicine ; R ; Science ; Q
    Sprache Englisch
    Erscheinungsdatum 2021-01-01T00:00:00Z
    Verlag Public Library of Science (PLoS)
    Dokumenttyp Artikel ; Online
    Datenquelle BASE - Bielefeld Academic Search Engine (Lebenswissenschaftliche Auswahl)

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  6. Artikel ; Online: Highly efficient UV/H2O2 technology for the removal of nifedipine antibiotics

    Wenping Dong / Chuanxi Yang / Lingli Zhang / Qiang Su / Xiaofeng Zou / Wenfeng Xu / Xingang Gao / Kang Xie / Weiliang Wang

    PLoS ONE, Vol 16, Iss 10, p e

    Kinetics, co-existing anions and degradation pathways.

    2021  Band 0258483

    Abstract: This study investigates the degradation of nifedipine (NIF) by using a novel and highly efficient ultraviolet light combined with hydrogen peroxide (UV/H2O2). The degradation rate and degradation kinetics of NIF first increased and then remained constant ...

    Abstract This study investigates the degradation of nifedipine (NIF) by using a novel and highly efficient ultraviolet light combined with hydrogen peroxide (UV/H2O2). The degradation rate and degradation kinetics of NIF first increased and then remained constant as the H2O2 dose increased, and the quasi-percolation threshold was an H2O2 dose of 0.378 mmol/L. An increase in the initial pH and divalent anions (SO42- and CO32-) resulted in a linear decrease of NIF (the R2 of the initial pH, SO42- and CO32- was 0.6884, 0.9939 and 0.8589, respectively). The effect of monovalent anions was complex; Cl- and NO3- had opposite effects: low Cl- or high NO3- promoted degradation, and high Cl- or low NO3- inhibited the degradation of NIF. The degradation rate and kinetics constant of NIF via UV/H2O2 were 99.94% and 1.45569 min-1, respectively, and the NIF concentration = 5 mg/L, pH = 7, the H2O2 dose = 0.52 mmol/L, T = 20 ℃ and the reaction time = 5 min. The ·OH was the primary key reactive oxygen species (ROS) and ·O2- was the secondary key ROS. There were 11 intermediate products (P345, P329, P329-2, P315, P301, P274, P271, P241, P200, P181 and P158) and 2 degradation pathways (dehydrogenation of NIF → P345 → P274 and dehydration of NIF → P329 → P315).
    Schlagwörter Medicine ; R ; Science ; Q
    Sprache Englisch
    Erscheinungsdatum 2021-01-01T00:00:00Z
    Verlag Public Library of Science (PLoS)
    Dokumenttyp Artikel ; Online
    Datenquelle BASE - Bielefeld Academic Search Engine (Lebenswissenschaftliche Auswahl)

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  7. Artikel ; Online: Perirenal adipose afferent nerves sustain pathological high blood pressure in rats

    Peng Li / Boxun Liu / Xiaoguang Wu / Yan Lu / Ming Qiu / Yihui Shen / Yunfan Tian / Chi Liu / Xiru Chen / Chuanxi Yang / Mengqing Deng / Yaqing Wang / Jia Gu / Zhongping Su / Xuguan Chen / Kun Zhao / Yanhui Sheng / Shijiang Zhang / Wei Sun /
    Xiangqing Kong

    Nature Communications, Vol 13, Iss 1, Pp 1-

    2022  Band 13

    Abstract: The sympathetic nervous system can contribute to the development of hypertension, but the neurogenic mechanisms involved are incompletely understood. Here the authors report that afferent nerves in the perirenal adipose tissue (PRAT) contribute to the ... ...

    Abstract The sympathetic nervous system can contribute to the development of hypertension, but the neurogenic mechanisms involved are incompletely understood. Here the authors report that afferent nerves in the perirenal adipose tissue (PRAT) contribute to the maintenance of high blood pressure, and PRAT ablation, denervation or upregulation of calcitonin gene-related peptide reduce blood pressure in hypertensive rats.
    Schlagwörter Science ; Q
    Sprache Englisch
    Erscheinungsdatum 2022-06-01T00:00:00Z
    Verlag Nature Portfolio
    Dokumenttyp Artikel ; Online
    Datenquelle BASE - Bielefeld Academic Search Engine (Lebenswissenschaftliche Auswahl)

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  8. Artikel ; Online: Highly efficient photocatalytic degradation of methylene blue by PoPD/TiO2 nanocomposite.

    Chuanxi Yang / Ming Zhang / Wenping Dong / Guanwei Cui / Zongming Ren / Weiliang Wang

    PLoS ONE, Vol 12, Iss 3, p e

    2017  Band 0174104

    Abstract: The poly-o-phenylenediamine (PoPD)/TiO2 nanocomposite was successfully synthesized via 'in situ' oxidative polymerization method. The modified photocatalysts were characterized by BET, scanning electron microscopy (SEM), transmission electron microscopy ( ...

    Abstract The poly-o-phenylenediamine (PoPD)/TiO2 nanocomposite was successfully synthesized via 'in situ' oxidative polymerization method. The modified photocatalysts were characterized by BET, scanning electron microscopy (SEM), transmission electron microscopy (TEM), X-ray diffraction (XRD), Fourier-transform infrarad spectra (FT-IR), thermogravimrtic analysis (TGA), X-ray photoelectron spectroscopy (XPS), Ultraviolet-visible diffuse reflectance spectrum (UV-Vis DRS) and Photocurrent Test. The results showed that the PoPD exists on the surface of TiO2, the presence of PoPD does not impact on the lattice structure and grain size of TiO2, and the presence of PoPD enhances the visible response and photoelectric property. The photocatalytic degradation of methylene blue (MB) was chosen as a model reaction to evaluate the photocatalytic activities of TiO2 and PoPD/TiO2. The optimal preparation condition was the molar ratio of oPD to TiO2 = 3:1, HCl concentration = 1.2 mol/L, the molar ratio of APS to oPD = 1:1. The apparent first-order rate constant kapp of PoPD/TiO2 nanocomposite was 0.0098 min-1, which is 6 times higher than TiO2 (0.0016 min-1). Meanwhile, the PoPD/TiO2 nanocomposites showed excellent photocatalytic stability, and the photocatalytic stability was depended on the stability of structure. At last, the photocatalytic mechanism of POPD/TiO2 nanocomposites was also proposed based on the synergetic effect between TiO2 and PoPD.
    Schlagwörter Medicine ; R ; Science ; Q
    Thema/Rubrik (Code) 620
    Sprache Englisch
    Erscheinungsdatum 2017-01-01T00:00:00Z
    Verlag Public Library of Science (PLoS)
    Dokumenttyp Artikel ; Online
    Datenquelle BASE - Bielefeld Academic Search Engine (Lebenswissenschaftliche Auswahl)

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  9. Artikel ; Online: A novel screening strategy of anti-SARS-CoV-2 drugs via blocking interaction between Spike RBD and ACE2

    Xiaoning Wang / Chuanxi Yang / Yangyang Sun / Xin Sui / Tong Zhu / Qian Wang / Shuai Wang / Jun Yang / Weijie Yang / Fengying Liu / Minmin Zhang / Yongan Wang / Yuan Luo

    Environment International, Vol 147, Iss , Pp 106361- (2021)

    2021  

    Abstract: Corona virus disease 2019 has spread worldwide, and appropriate drug design and screening activities are required to overcome the associated pandemic. Using computational simulation, blockade mechanism of SARS-CoV-2 spike receptor binding domain (S RBD) ... ...

    Abstract Corona virus disease 2019 has spread worldwide, and appropriate drug design and screening activities are required to overcome the associated pandemic. Using computational simulation, blockade mechanism of SARS-CoV-2 spike receptor binding domain (S RBD) and human angiotensin converting enzyme 2 (hACE2) was clarified based on interactions between RBD and hesperidin. Interactions between anti-SARS-CoV-2 drugs and therapy were investigated based on the binding energy and druggability of the compounds, and they exhibited negative correlations; the compounds were classified into eight common types of structures with highest activity. An anti-SARS-CoV-2 drug screening strategy based on blocking S RBD/hACE2 binding was established according to the first key change (interactions between hesperidin and S RBD/hACE2) vs the second key change (interactions between anti-SARS-CoV-2 drugs and RBD/hACE2) trends. Our findings provide valuable information on the mechanism of RBD/hACE2 binding and on the associated screening strategies for anti-SARS-CoV-2 drugs based on blocking mechanisms of pockets.
    Schlagwörter SARS-CoV-2 Spike RBD ; hACE2 ; Blockade mechanism ; Structure-activity relationship ; Anti-SARS-CoV-2 drugs screening strategy ; Environmental sciences ; GE1-350
    Thema/Rubrik (Code) 540
    Sprache Englisch
    Erscheinungsdatum 2021-02-01T00:00:00Z
    Verlag Elsevier
    Dokumenttyp Artikel ; Online
    Datenquelle BASE - Bielefeld Academic Search Engine (Lebenswissenschaftliche Auswahl)

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  10. Artikel: The design and implementation of risk assessment model for hazard installations based on AHP–FCE method: A case study of Nansi Lake Basin

    Wang, Weiliang / Chuanxi Yang / Chunling Dong / Lihui Huang / Tiantian Ju / Wenping Dong / Zongming Ren

    Ecological informatics. 2016 Nov., v. 36

    2016  

    Abstract: In this paper, the combined analytical hierarchy process–fuzzy comprehensive evaluation (AHP–FCE) model was built to assess the risk for hazard installations of the Nansi Lake Basin. A detailed analysis was carried out showing the relationships between ... ...

    Abstract In this paper, the combined analytical hierarchy process–fuzzy comprehensive evaluation (AHP–FCE) model was built to assess the risk for hazard installations of the Nansi Lake Basin. A detailed analysis was carried out showing the relationships between the risk index and risk factors in the Nansi Lake Basin of China. To enhance the accuracy and applicability of assessing the risk, which could be influenced by the sampled human factor, an analytical mathematic method was used to show the relationship between the statistic law and the comprehensive index. The AHP–FCE model combined AHP's capabilities of multi-object and multi-rule decision with FCE's advantages in uncertainty processing. The fuzzy treatment scheme and fuzzy operation strategy were both optimized and ameliorated, so that the model could achieve the flexibility and reliability to identify and dynamically evaluate hazard installations. In this paper, the analysis of the survey data taken from the Nansi Lake Basin, scientific theory, validity in scheme, and operating feasibility of the model were validated. It is the hope that the combined AHP–FCE model will provide valuable information pertaining to environment and hazard installation risk assessments for basin systems.
    Schlagwörter basins ; case studies ; humans ; models ; risk assessment ; risk factors ; surveys ; uncertainty ; watersheds ; China
    Sprache Englisch
    Erscheinungsverlauf 2016-11
    Umfang p. 162-171.
    Erscheinungsort Elsevier B.V.
    Dokumenttyp Artikel
    ZDB-ID 2212016-6
    ISSN 1878-0512 ; 1574-9541
    ISSN (online) 1878-0512
    ISSN 1574-9541
    DOI 10.1016/j.ecoinf.2015.11.010
    Datenquelle NAL Katalog (AGRICOLA)

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